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RESEARCH PRODUCT

Characterization of the light absorbing properties, chromophores composition and sources of brown carbon aerosol in Xi'an, Northwest China

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Abstract. The impact of brown carbon aerosol (BrC) on the Earth's radiative forcing balance has been widely recognized but remains uncertain, mainly because the relationships among BrC sources, chromophores, and optical properties of aerosol are poorly understood. In this work, the light absorption properties and chromophore composition of BrC were investigated for samples collected in Xi'an, Northwest China from 2015 to 2016. Both absorption Ångström exponent and mass absorption efficiency show distinct seasonal differences, which could be attributed to the differences in sources and chromophore composition of BrC. Three groups of light-absorbing organics were found to be important BrC chromophores, including those show multiple absorption peaks at wavelength > 350 nm (12 polycyclic aromatic hydrocarbons and their derivatives) and those show single absorption peak at wavelength