6533b833fe1ef96bd129b993
RESEARCH PRODUCT
Cross-stream migration of a Brownian droplet in a polymer solution under Poiseuille flow
Michael P. HowardThomas M. TruskettArash Nikoubashmansubject
Materials scienceFOS: Physical sciences02 engineering and technologyCondensed Matter - Soft Condensed Matter010402 general chemistry01 natural sciencesPhysics::Fluid DynamicsNewtonian fluidPhysics::Atomic and Molecular ClustersBrownian motionchemistry.chemical_classificationMicrochannelDissipative particle dynamicsFluid Dynamics (physics.flu-dyn)General ChemistryPolymerMechanicsPhysics - Fluid Dynamics021001 nanoscience & nanotechnologyCondensed Matter PhysicsHagen–Poiseuille equation0104 chemical sciencesShear rateLift (force)Condensed Matter::Soft Condensed MatterchemistrySoft Condensed Matter (cond-mat.soft)0210 nano-technologydescription
The migration of a Brownian fluid droplet in a parallel-plate microchannel was investigated using dissipative particle dynamics computer simulations. In a Newtonian solvent, the droplet migrated toward the channel walls due to inertial effects at the studied flow conditions, in agreement with theoretical predictions and recent simulations. However, the droplet focused onto the channel centerline when polymer chains were added to the solvent. Focusing was typically enhanced for longer polymers and higher polymer concentrations with a nontrivial flow-rate dependence due to droplet and polymer deformability. Brownian motion caused the droplet position to fluctuate with a distribution that primarily depended on the balance between inertial lift forces pushing the droplet outward and elastic forces from the polymers driving it inward. The droplet shape was controlled by the local shear rate, and so its average shape depended on the droplet distribution.
| year | journal | country | edition | language |
|---|---|---|---|---|
| 2018-12-17 |