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RESEARCH PRODUCT
Second-order Raman scattering in CuO
Alexander P. LitvinchukAlexander P. LitvinchukPeter KrügerL. DebbichiMarin GospodinovAngela MöllerAngela MöllerMilko IlievMilko Ilievsubject
Quasielastic scatteringCondensed matter physicsPhonon scatteringScatteringChemistryInelastic scatteringMott scatteringCondensed Matter PhysicsMolecular physicsLight scatteringX-ray Raman scatteringCondensed Matter::SuperconductivityGeneral Materials ScienceBiological small-angle scatteringdescription
Polarized second-order Raman scattering spectra of CuO single crystals are reported. It is shown that for some scattering geometries the second-order processes dominate the inelastic light scattering spectra. Group-theoretical symmetry analysis of the selection rules for the first- and second-order scattering processes is performed and phonon dispersion relations are calculated within density functional theory. The main spectral features of the two-phonon spectra are assigned to overtones of the vibrational branches at various special points across the Brillouin zone.
year | journal | country | edition | language |
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2013-02-08 | Journal of Physics: Condensed Matter |