Realization of time-resolved two-vacuum-ultraviolet-photon ionization

6533b838fe1ef96bd12a479b

RESEARCH PRODUCT

Realization of time-resolved two-vacuum-ultraviolet-photon ionization

Olivier Faucher E. P. Benis J. Kruse D. Charalambidis D. Charalambidis A. Peralta Conde P. Tzallas

subject

spectroscopy attosecond Photon [ PHYS.PHYS.PHYS-ATOM-PH ] Physics [physics]/Physics [physics]/Atomic Physics [physics.atom-ph]Physics::Optics photoionisation nm 01 natural sciences 7. Clean energy Atmospheric-pressure laser ionization 010309 optics Frequency conversion Ionization higher order harmonic generation 0103 physical sciences Physics::Atomic and Molecular Clusters ethylene molecules two-photon processes Physics::Chemical Physics 010306 general physics Ultrafast dynamics Physics [PHYS.PHYS.PHYS-ATOM-PH]Physics [physics]/Physics [physics]/Atomic Physics [physics.atom-ph]photodissociation dynamics VUV Atomic and Molecular Physics and Optics laser-pulses Vacuum ultraviolet Extreme ultraviolet molecule-photon collisions XUX 32.80.Rm 42.65.Re 42.65.Ky HHG Atomic physics ultrafast internal-conversion organic compounds physics Realization (systems)oxygen

description

International audience; Ultrafast dynamics of excited molecules is studied through time-resolved two-vacuum-ultraviolet (vuv)- photon ionization using a nonlinear volume autocorrelator unit. The two-vuv-photon process is induced by the intense ﬁfth harmonic radiation of a femtosecond Ti:sapphire laser. In a proof-of-principle experiment, ultrafast dynamics of excited ethylene and oxygen molecules are investigated. Molecular decay times are deduced by comparing the experimental data with the results of a numerical model that accounts for the spatial and temporal characteristics of the harmonic ﬁeld. The present experiments pave a convenient way for time domain investigations in the vuv-xuv spectral region in all states of matter at few femtosecond to subfemtosecond temporal scales.

year	journal	country	edition	language
2009-06-12

https://hal.archives-ouvertes.fr/hal-00402819

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