6533b839fe1ef96bd12a6e04

RESEARCH PRODUCT

Oscillation Phenomena Leading to Chaos in a Stochastic Surface Reaction Model

W. Von NiessenV. N. KuzovkovV. N. KuzovkovO. Kortlüke

subject

PhysicsOscillationLattice (order)Monte Carlo methodGeneral Physics and AstronomyStatistical physicsSurface reaction

description

A microscopic lattice gas model for the $\mathrm{CO}+\mathrm{NO}$ reaction on Pt(100) is studied by means of Monte Carlo simulations. It shows different kinetical phenomena such as steady state reaction, damped, regular, and irregular oscillations, as well as a transition into chaotical behavior via the Feigenbaum route. Because of its small number of parameters, each with a specific physical meaning, it enables the investigation of the whole parameter regime leading to a deeper insight to the mechanisms which create the oscillations and chaotical behavior.

https://doi.org/10.1103/physrevlett.81.2164