6533b862fe1ef96bd12c654f

RESEARCH PRODUCT

Singlet-groundstate magnetism in TbP

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Elastic neutron scattering and magnetic susceptibility data are reported for temperatures around the Neel-point,TN=7.3 K, and for zero magnetic field. AboveTN, the temperature dependence of the magnetic central peak intensity can adequately be described within the RPA assuming isotropic exchange between nearest and next-nearest neighbours as the only parameters. This two-parameter model is quantitatively confirmed by the susceptibility data. AtTN, magnetic Bragg-intensities arise almost discontinuously (reaching 70% of the saturation within 0.1 K) accompanied by thermal hysteresis. For all temperatures belowTN the sublattice magnetic moment is explained by solutions of meanfield equations, if an effective quadrupole-quadrupole interaction is included. The quadrupolar coupling parameter is fully consistent with a value determined recently from the softening of thec44-mode. These results show, that earlier suggestions of renormalization group results upon the origin of the first order phase transition in TbP are not needed.