6533b884fe1ef96bd12dfd1a

RESEARCH PRODUCT

Multistep spin switching in orthogonally-twisted ferromagnetic monolayers

Carla Boix-constantSamuel Mañas-valeroEugenio Coronado

subject

Mesoscale and Nanoscale Physics (cond-mat.mes-hall)Materials Science (cond-mat.mtrl-sci)FOS: Physical sciences

description

The advent of twisting-engineering in two-dimensional (2D) crystals enables the design of van der Waals (vdW) heterostructures exhibiting emergent properties. In the case of magnets, this approach can afford artificial magnets with tailored spin arrangements that do not exist in nature. Here, we fabricate an artificial magnet by twisting 90 degrees two CrSBr ferromagnetic monolayers with an easy-axis in-plane anisotropy, thus forming an "orthogonally-twisted bilayer". The magneto-transport properties reveal multistep spin switching with a magnetic hysteresis opening, which is absent in the pristine case. By tuning the magnetic field, we modulate the remanent state and coercivity and select between hysteretic and non-hysteretic magneto-resistance scenarios. This complexity is fundamentally different from that achieved in Moiré superlattices. Our results highlight the control over the magnetic properties in vdW heterostructures, leading to a variety of field-induced phenomena and opening a fruitful playground for creating artificial magnetic symmetries and manipulating non-collinear magnetic textures.

10.48550/arxiv.2301.05647https://doi.org/10.48550/arxiv.2301.05647