Search results for " Coating"

showing 10 items of 2563 documents

An integrated approach to evaluating the tribo-contact for coated cutting inserts

2000

Abstract The orthogonal machining process when end turning medium carbon and austenitic stainless steels with cemented WC-Co tools coated with single-layer (TiC), two-layer (TiC/TiN), and three-layer (TiC/Al2O3/TiN) hard thin films was investigated. Extensive experimental investigations including the thermal, mechanical and tribological responses of the tribo-contact between the coating–substrate system and the chip, under different cutting conditions, were carried out. The study sheds light on the cutting forces, the interface temperatures and the tribo-contact conditions, including the friction energy dissipated at the tool–chip interface, the frictional heat flux conducting into either t…

AusteniteInsert (composites)Materials scienceMetallurgychemistry.chemical_elementSurfaces and InterfacesTribologyengineering.materialCondensed Matter PhysicsSurfaces Coatings and FilmschemistryCoatingHeat fluxMechanics of MaterialsMaterials ChemistryengineeringThin filmComposite materialContact areaTinWear
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The influence of thin hard coatings on frictional behaviour in the orthogonal cutting process

2000

New knowledge about the tribological response deriving from the interaction of the substrate/coating-chip system, with special attention to the orthogonal cutting process when chatter-free end turning using natural contact tools, is developed. In order to evaluate the frictional behaviour of this process under modified contact conditions, experimental investigations including the contact temperature, the contact loads, friction and the frictional heat flux per unit area were carried out. In contrast to the most obvious approach, the coefficient of sliding friction versus the cutting speed, the contact temperature, the normal pressure and the interface control factor is considered. A number …

AusteniteMaterials scienceMechanical EngineeringMetallurgySurfaces and InterfacesTribologyengineering.materialThermal conductionSurfaces Coatings and FilmsControllabilitySubstrate (building)Heat fluxCoatingMechanics of MaterialsengineeringComposite materialLayer (electronics)Tribology International
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Microstructural evolution of wear-resistant FeCrB and FeCrNiCoB coating alloys during high-energy mechanical attrition

2008

Mechanical milling/attrition provides a convenient scope of simulating the microstructural changes encountered by wear-resistant coating alloys subjected to deformation under high frequency and high-intensity impact loading or accelerated wear condition. In the present study, the microstructural evolution of two commercial coating materials, FeCrB (Armacor M) and FeCrNiCoB (Armacor C), in the course of low- and high-intensity mechanical attrition, was monitored by X-ray diffraction and high-resolution transmission electron microscopy. While low-intensity milling leads to marginal grain refinement but no change in phase-aggregate in FeCrB, similar mechanical attrition causes boride precipita…

AusteniteMaterials scienceMetallurgyAlloySurfaces and Interfacesengineering.materialCondensed Matter PhysicsMicrostructureNanocrystalline materialSurfaces Coatings and FilmsAmorphous solidchemistry.chemical_compoundchemistryCoatingMechanics of MaterialsBorideMaterials ChemistryengineeringSolid solutionWear
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Influence of friction on the local mechanical and electrochemical behaviour of duplex stainless steels.

2006

International audience; The electrochemical behaviour of ferritic and austenitic phases in duplex stainless steel (UNS S32304) and the modifications induced by straining during sliding were studied by potentiodynamic polarisation curves determined at the microscale in a 1MNaCl (pH 3) solution, using an electrochemical microcell. The mechanical properties and stress state of each phase were determined by microhardness and X-ray microdiffraction measurements, before and after straining. The results show that sliding generates elastic straining of the ferrite and plastic deformation of the austenite. The electrochemical behaviour of these phases is dramatically altered, inducing a reduction of…

AusteniteMaterials sciencePassivationFrictionMetallurgyMicrodiffractionSurfaces and InterfacesCondensed Matter PhysicsElectrochemistryStressIndentation hardnessSurfaces Coatings and FilmsCorrosion[SPI]Engineering Sciences [physics]Local electrochemistryMechanics of MaterialsDuplex (building)MicrohardnessFerrite (iron)Duplex steelsMaterials Chemistry[ SPI ] Engineering Sciences [physics]Microscale chemistry
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Inhibitoren der Korrosion 21 (1) - Autoxidationsstudien an Fe2+-Salzen der Tetramethylen-1,4-bis-phosphonsäure, der Hexamethylen-1,6-bis-phosphonsäur…

1978

Die Wirksamkeit der organischen Bisphosphonsauren als Inhibitoren der Korrosion von Eisen ist dadurch bedingt, das die aus der Eisenoberflache auftretenden Fe2+-Ionen direkt am Austrittsort mit den Sauren reagieren und an Ort und Stelle dreidimensional vernetzte Deckschichten aufbauen. Je dichter die Struktur dieser Schichten, je bestandiger das Netzwerk gegen Sauerstoff und je hydrolysebestandiger die FeOP-Bindungen, desto besser ist die Schutzwirkung: Dadurch wird sowohl dem Sauerstoff als auch dem Chloridion der Zugang zur Metalloberflache verwehrt. Die Modellversuche ermoglichen aufgrund der Verteilung des Phosphors in den Niederschlagen Ruckschlusse auf den Vernetzungsgrad. Corrosion I…

AutoxidationChemistryMechanical EngineeringMetals and AlloysGeneral MedicineChlorideMedicinal chemistrySurfaces Coatings and FilmsMetalHydrolysischemistry.chemical_compoundPyrophosphoric acidMechanics of Materialsvisual_artMaterials Chemistrymedicinevisual_art.visual_art_mediumEnvironmental ChemistryPhosphoric acidmedicine.drugMaterials and Corrosion
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Inhibitoren der Korrosion 19 (1). Autoxidationsstudien an Fe2+-Trimethylen-1,3-bis-phosphonat als Modell einer die Korrosion inhibierenden Deckschicht

1976

Die Autoxidationsgeschwindigkeit der Fe2+. Salze ist stark abhangig vom pH und ist bei pH 2 praktisch gleich Null, bei pH 5–7 sehr hoch. Durch Zusatz von Trimethylen-1,3-bis-phosphonsaure wird die Autoxidation etwas verlangsamt und der Sauerstoffverbrauch starker erhoht als es der Stochiometrie der Fe2+-Oxidation entspricht. Dieser Umstand erklart sich durch den oxidativen Abbau der Trimethylen-1,3-bis-phosphonsaure zu Phosphorsaure, wobei Salze des dreiwertigen Eisens als Niederschlag ausfallen. Diese Fe3+-bis-phosphonate sind dreidimensional vernetzt; das Fe:P-Verhaltnis liegt zwischen 0.5 und 0.9 und wird mit abnehmendem pH-Wert geringer. Inhibitors of corrosion 19 (1). Autoxidation stud…

AutoxidationChemistryMechanical EngineeringMetals and Alloyschemistry.chemical_elementGeneral MedicineMedicinal chemistryOxygenSurfaces Coatings and Filmschemistry.chemical_compoundMechanics of MaterialsPolymer chemistryMaterials ChemistryEnvironmental ChemistryPhosphoric acidStoichiometryMaterials and Corrosion/Werkstoffe und Korrosion
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Kinetics of Zn2+ complexation by a ditopic phenanthroline-azamacrocyclic scorpiand-like receptor.

2012

Coordination of Zn(2+) to a ditopic phenanthroline-macrocycle receptor takes place in three steps, the first one being the coordination to the phenanthroline, followed by the slow movement of the metal to the polyamine macrocycle and a final re-arrangement to coordinate the pendent arm.

Aza CompoundsStereochemistryPhenanthrolineKineticsMetals and AlloysGeneral ChemistryHydrogen-Ion ConcentrationCatalysisSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsMetalchemistry.chemical_compoundKineticsZincchemistryCoordination Complexesvisual_artPolymer chemistryMaterials ChemistryCeramics and Compositesvisual_art.visual_art_mediumSlow MovementPolyamineReceptorPhenanthrolinesChemical communications (Cambridge, England)
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The azido ligand: a useful tool in designing chain compounds exhibiting alternating ferro- and antiferro-magnetic interactions

1997

A one-pot reaction of NiII 1, CoII 2, FeII 3 and MnII 4 with 2,2A-bipyridine (bipy) and azide in water leads to [M(bipy)(N3)2]n chains where the metal ion is alternatively bridged by double end-on (EO) and end-to-end (EE) azido bridges; theoretical analysis of the variable-temperature magnetic susceptibility data of 1 and 4 reveals the occurrence of intrachain alternating ferro- (through EO) and antiferro-magnetic (through EE) interactions. Julve Olcina, Miguel, Miguel.Julve@uv.es ; Lloret Pastor, Francisco, Francisco.Lloret@uv.es ; Clemente Juan, Juan Modesto, Juan.M.Clemente@uv.es

Azido ligand ; Ferro-magnetic ; Antiferro-magnetic ; BipyrineStereochemistryUNESCO::QUÍMICABipyrine:QUÍMICA [UNESCO]CatalysisMetalchemistry.chemical_compoundChain (algebraic topology)Ferro-magneticMaterials ChemistryChemistryLigandUNESCO::QUÍMICA::Química inorgánicaMetals and AlloysAzido ligandGeneral Chemistry:QUÍMICA::Química inorgánica [UNESCO]Magnetic susceptibilitySurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsCrystallographyvisual_artAntiferro-magneticCeramics and Compositesvisual_art.visual_art_mediumAzide
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Electron Transfer from Organic Aminophenyl Acid Sensitizers to Titanium Dioxide Nanoparticle Films

2009

Electron transfer from three conjugated amino-phenyl acid dyes to titanium and aluminum oxide nanocrystalline films was studied by using transient absorption spectroscopy with sub 20 fs time-resolution over the visible spectral region. All the dyes attached to TiO2 showed long-lived ground state bleach signals indicative of formation of new species. Global analysis of the transient kinetics of the dyes on TiO2 revealed stimulated emission decays of about 40 fs and less than 300 fs assigned to electron injection. The same dyes on Al2O3 substrates displayed long stimulated emission decays (ns) suggesting that electron transfer is blocked in this high band gap semiconductor. For two of the dye…

Band gapConjugated systemPhotochemistrySurfaces Coatings and FilmsElectronic Optical and Magnetic Materialschemistry.chemical_compoundElectron transferGeneral EnergychemistryTitanium dioxideUltrafast laser spectroscopyDensity functional theoryStimulated emissionPhysical and Theoretical ChemistrySpectroscopyThe Journal of Physical Chemistry C
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Acid–Base Properties and Surface Charge Distribution of the Water-Soluble Au102(pMBA)44 Nanocluster

2016

The pKa of the p-mercaptobenzoic acid (pMBA) ligands in the Au102(pMBA)44 nanocluster was measured by using acid–base and IR titration. The observed macroscopic pKa = 6.18 ± 0.05 is significantly more basic than that of free pMBA (pKa = 4.16), and the protonation behavior is anticooperative according to the Hill coefficient n = 0.64 ± 0.04. The cluster is truly water-soluble when more than 22 and insoluble when fewer than 7 ligands are in the deprotonated state. In order to obtain more insight into the anticooperative character, the cluster was modeled at pH ∼6.2 using constant pH molecular dynamics simulations. The pKa values of the individual pMBAs are in the range of 5.18–7.58, depending…

Base (chemistry)acid–base propertiesInorganic chemistryProtonation02 engineering and technology010402 general chemistry01 natural sciencescharge distributionMolecular dynamicsDeprotonationCluster (physics)Surface chargePhysical and Theoretical Chemistryta116chemistry.chemical_classificationChemistryCharge density021001 nanoscience & nanotechnology0104 chemical sciencesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsGeneral EnergyPhysical chemistryTitration0210 nano-technologygold nanoclustersJournal of Physical Chemistry C
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