Search results for " Phase"

showing 10 items of 1862 documents

On the blue phase structure of hydrogen-bonded liquid crystals via 19F NMR

2018

Abstract 19 F NMR spectra are simulated for blue phase I of FPHG( St 1.5 ∗ Ap 1.5 ) based on a model of a double-twisted substructure inside cylinders that form a body-centred cubic lattice. A kinetic matrix is included to describe jump processes over quarter pitch lengths. Though the lines in the NMR spectra are broad and featureless, changes in the widths and positions with temperature are well described by the blue phase model structure. The spectra in the chiral nematic N∗ phase are also simulated. Dynamics in the BP I are found to be slower than in the N∗ phase.

Materials scienceHydrogenSpectral simulationChemieGeneral Physics and Astronomychemistry.chemical_elementBlue phase IDouble-twisted substructure02 engineering and technologyFluorine-19 NMR010402 general chemistryKinetic energy01 natural sciencesMolecular physicsSpectral lineDiffusion rateLiquid crystalLattice (order)Physical and Theoretical Chemistry021001 nanoscience & nanotechnologyFluorine NMR0104 chemical sciencesNMR spectra databasechemistrySubstructureSettore CHIM/07 - Fondamenti Chimici Delle Tecnologie0210 nano-technologyChiral nematic
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A New Environmentally-Friendly Colorimetric Probe for Formaldehyde Gas Detection under Real Conditions

2018

[EN] A new environmentally-friendly, simple, selective and sensitive probe for detecting formaldehyde, based on naturally-occurring compounds, through either colorimetric or fluorescence changes, is described. The probe is able to detect formaldehyde in both solution and the gas phase with limits of detection of 0.24 mM and 0.7 ppm, respectively. The probe has been tested to study formaldehyde emission in contaminated real atmospheres. The supported probe is easy to use and to dispose, and is safe and suitable as an individual chemodosimeter.

Materials scienceInorganic chemistryFormaldehydePharmaceutical ScienceGas phase010402 general chemistry01 natural sciencesAnalytical ChemistryGas phaselcsh:QD241-441chemistry.chemical_compoundchromogenic sensorlcsh:Organic chemistryLimit of DetectionFormaldehydeDrug DiscoveryPhysical and Theoretical ChemistryDetection limitPictet-Spengler010405 organic chemistryCommunicationOrganic ChemistryEnvironmentally friendlyenvironmentally-friendlyChromogenic sensor0104 chemical sciencesEnvironmentally-friendlySolutionsSpectrometry FluorescencechemistryChemistry (miscellaneous)Molecular MedicineformaldehydeColorimetrygas phaseMolecules
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CVD elaboration and in situ characterization of barium silicate thin films.

2010

International audience; This study is concerned with the elaboration of barium silicate thin films by metal organic chemical vapor deposition (MOCVD) and in situ characterization by X-ray photoemission spectroscopy (XPS) with an apparatus connected to the deposition reactor. The difficulty to find an efficient metal organic precursor for barium is described. After characterizations of the selected reactant, Ba(TMHD)2tetraglyme, the development of an original specific vapor delivering source which allows reactant sublimation in the CVD reactor was performed. In the most optimized cases, including use of oxygen introduction during the deposition, barium silicate films were obtained. Moreover,…

Materials scienceInorganic chemistrychemistry.chemical_element02 engineering and technologyChemical vapor deposition01 natural scienceschemistry.chemical_compound0103 physical sciencesMaterials ChemistryMetalorganic vapour phase epitaxyThin filmSpectroscopyFilms010302 applied physicsBarium oxideBariumSilicate021001 nanoscience & nanotechnologySilicateCarbon filmchemistryBariumCeramics and CompositesSublimation (phase transition)Insulator0210 nano-technology
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Adsorption of CO and N 2 molecules at the surface of solid water. A grand canonical Monte Carlo study

2020

International audience; The adsorption of carbon monoxide and nitrogen molecules at the surface of four forms of solid water is investigated by means of grand canonical Monte Carlo simulations. The trapping ability of crystalline Ih and low-density amorphous ices, along with clathrate hy-drates of structures I and II, are compared at temperatures relevant for astrophysics. It is shown that, when considering a gas phase that contains mixtures of carbon monoxide and nitrogen, the trapping of carbon monoxide is favored with respect to that of nitrogen at the surface of all solids, irrespective of the temperature. The results of the calculations also indicate that some amounts of molecules can …

Materials scienceInterface propertiesClathrate hydrateGeneral Physics and Astronomychemistry.chemical_elementGas phaseTrappingPhysics of gases010402 general chemistryAstrophysics01 natural scienceschemistry.chemical_compoundAmorphous materialsAdsorption0103 physical sciencesCometsMoleculePhysical and Theoretical ChemistryAdsorption isothermCarbon monoxideComputingMilieux_MISCELLANEOUS[PHYS]Physics [physics]010304 chemical physicsMonte Carlo methodsNitrogen0104 chemical sciencesAmorphous solid[CHIM.THEO]Chemical Sciences/Theoretical and/or physical chemistrychemistry13. Climate actionChemical physics[SDU]Sciences of the Universe [physics]Complex solidsSelectivityCarbon monoxide
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Liquid phase exfoliation of carbonate-intercalated layered double hydroxides.

2019

Direct exfoliation of a carbonate layered double hydroxide (LDH) has been achieved by using a novel horn-probe sonic tip, avoiding the development of time-consuming anion-exchange reactions. The most suitable solvents were chosen based on the Hildebrand solubility parameters and the thickness of the exfoliated nanosheets confirmed unambiguously the successful delamination.

Materials scienceLiquid phaseengineering.material010402 general chemistry01 natural sciencesCatalysischemistry.chemical_compoundMaterials Chemistry010405 organic chemistryDelaminationMetals and AlloysLayered double hydroxidesGeneral ChemistryQuímicaExfoliation joint0104 chemical sciencesSurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsHildebrand solubility parameterchemistryChemical engineeringCeramics and CompositesengineeringHydroxideCarbonateChemical communications (Cambridge, England)
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The Effect of Technological Factors on the Synthesis of PbMg 1/3 Nb 2/3 O 3

2003

Conventional technique of solid phase reactions allows one to obtain PbMg 1/3 Nb 2/3 O 3 material with about 20 vol.% of the pyrochlore phase. The latter can be reduced to 5 vol.% by Swartz-Shrout two-stage solid state reaction via MgNb 2 O 6 having the columbite structure. A single-phase perovskite product can be obtained by by the two-stage columbite method from mixtures containing 0.2 mol. parts of overstoichiometric MgO. The best results are obtained by using magnesium carbonate hydroxide pentahydrate (MgCO 3 ) 4 ·Mg(OH) 2 ·5H 2 O as the magnesium source. The modified route yields stoichiometric single-phase PMN.

Materials scienceMagnesiumSolid phase reactionsAnalytical chemistryPyrochlorechemistry.chemical_elementengineering.materialCondensed Matter PhysicsFerroelectricityElectronic Optical and Magnetic MaterialschemistryPhase (matter)engineeringColumbiteStoichiometryPerovskite (structure)Ferroelectrics
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Single-Element Reflective Digital Holographic Microscopy

2021

Digital holographic microscopy (DHM) is a well-known microscopy technique using an interferometric architecture for quantitative phase imaging (QPI) and it has been already implemented utilizing a large number of interferometers. Among them, single-element interferometers are of particular interest due to its simplicity, stability, and low cost. Here, we present an extremely simple common-path interferometric layout based on the use of a single one-dimensional diffraction grating for both illuminating the sample in reflection and generating the digital holograms. The technique, named single-element reflective digital holographic microscopy (SER-DHM), enables QPI and topography analysis of r…

Materials scienceMaterials Science (miscellaneous)BiophysicsHolographyGeneral Physics and Astronomy02 engineering and technologydigital holographic microscopyreflective microscopy01 natural scienceslaw.invention010309 opticsOpticslaw0103 physical sciencesMicroscopyAstronomical interferometerdiffraction gratingPhysical and Theoretical ChemistryReflection (computer graphics)Diffraction gratingMathematical Physicsbusiness.industryphase measurememnt021001 nanoscience & nanotechnologyInterference microscopylcsh:QC1-999interference microscopyInterferometryquantitative phase imaging (QPI)Digital holographic microscopy0210 nano-technologybusinesslcsh:PhysicsFrontiers in Physics
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Synthesis and characterization of copper intercalated ZrTe3

1997

Abstract Electrochemical copper intercalation in ZrTe3 yields the new metallic ternary phase CuxZrTe3 with a maximum stoichiometry of x = 1.9. The charge is balanced by filling the σ∗ antibonding Te p bands, as monitored by XANES spectroscopy. The reaction is accompanied by an increase in the a lattice dimension of 9%. This observation is explained by theoretical calculations.

Materials scienceMechanical EngineeringIntercalation (chemistry)Inorganic chemistryMetals and Alloyschemistry.chemical_elementAntibonding molecular orbitalTernary phaseElectrochemistryCopperMetalCrystallographychemistryMechanics of MaterialsLattice (order)visual_artMaterials Chemistryvisual_art.visual_art_mediumStoichiometry
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Synthesis of Nd:YAG nanopowder using the citrate method with microwave irradiation

2010

Abstract Nd:YAG nanopowders were prepared using the Pechini process with microwave irradiation ( MWs ). A reference sample was also prepared using conventional heating. XRD pattern analysis showed that nanopowder obtained by means of conventional heating and calcination for 1 h at 900 °C has a structure made up of the garnet phase together with the hexagonal phase that disappeared after two additional hours of thermal treatment. The MWs powder calcined for 1 h consists of the single garnet phase. SAXS data analysis indicated that nanoparticles are characterized by a sharp interface. TEM investigation showed crystalline particles with remarkable agglomeration in both samples, although a more…

Materials scienceMechanical EngineeringMetals and AlloysAnalytical chemistryHexagonal phaseNanoparticleThermal treatmentNd:YAG nanopowders microwave irradiation Pechini method SAXS.law.inventionMechanics of MaterialslawPhase (matter)Materials ChemistryCalcinationParticle sizeSelected area diffractionMicrowave
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Melting and multipole deformation of sodium clusters

1999

Melting and multipole deformations of sodium clusters with up to 55 atoms are studied using an ab initio molecular dynamics method. The melting temperature regions for Na20, Na40, and Na 55 + are estimated. The melting temperature region determined here for Na 55 + agrees with the one determined experimentally. The dominating deformation type observed at the liquid phase for Na20 and Na40 is octupole deformation and for Na14 and Na 55 + quadrupole deformation.

Materials scienceMelting temperatureSodiumLiquid phasechemistry.chemical_elementDeformation (meteorology)Molecular physicsAtomic and Molecular Physics and OpticsAb initio molecular dynamicsNuclear magnetic resonancechemistryQuadrupolePhysics::Atomic PhysicsMultipole expansionThe European Physical Journal D
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