Search results for " Soft"
showing 10 items of 1710 documents
Experimental Evidence for a Structural-Dynamical Transition in Trajectory Space.
2016
Among the key insights into the glass transition has been the identification of a non-equilibrium phase transition in trajectory space which reveals phase coexistence between the normal supercooled liquid (active phase) and a glassy state (inactive phase). Here we present evidence that such a transition occurs in experiment. In colloidal hard spheres we find a non-Gaussian distribution of trajectories leaning towards those rich in locally favoured structures (LFS), associated with the emergence of slow dynamics. This we interpret as evidence for an non-equilibrium transition to an inactive LFS-rich phase. Reweighting trajectories reveals a first-order phase transition in trajectory space be…
Microscopic Dynamics of Hard Ellipsoids in their Liquid and Glassy Phase
2001
To investigate the influence of orientational degrees of freedom onto the dynamics of molecular systems in its supercooled and glassy regime we have solved numerically the mode-coupling equations for hard ellipsoids of revolution. For a wide range of volume fractions $\phi$ and aspect ratios $x_{0}$ we find an orientational peak in the center of mass spectra $\chi_{000}^{''}(q,\omega)$ and $\phi_{000}^{''} (q,\omega)$ about one decade below a high frequency peak. This orientational peak is the counterpart of a peak appearing in the quadrupolar spectra $\chi_{22m}^{''}(q,\omega)$ and $\phi_{22m}^{''}(q,\omega)$. The latter peak is almost insensitive on $\phi$ for $x_{0}$ close to one, i.e. f…
Dynamical precursor of nematic order in a dense fluid of hard ellipsoids of revolution
2004
We investigate hard ellipsoids of revolution in a parameter regime where no long range nematic order is present but already finite size domains are formed which show orientational order. Domain formation leads to a substantial slowing down of a collective rotational mode which separates well from the usual microscopic frequency regime. A dynamic coupling of this particular mode into all other modes provides a general mechanism which explains an excess peak in spectra of molecular fluids. Using molecular dynamics simulation on up to 4096 particles and on solving the molecular mode coupling equation we investigate dynamic properties of the peak and prove its orientational origin.
Magnetic micro-droplet in rotating field: numerical simulation and comparison with experiment
2017
Magnetic droplets obtained by induced phase separation in a magnetic colloid show a large variety of shapes when exposed to an external field. However, the description of shapes is often limited. Here we formulate an algorithm based on three dimensional boundary-integral equations for strongly magnetic droplets in a high-frequency rotating magnetic field, allowing us to find their figures of equilibrium in three dimensions. The algorithm is justified by a series of comparisons with known analytical results. We compare the calculated equilibrium shapes with experimental observations and find a good agreement. The main features of these observations are the oblate-prolate transition, the flat…
3D motion of flexible ferromagnetic filaments under a rotating magnetic field.
2020
Ferromagnetic filaments in a rotating magnetic field are studied both numerically and experimentally. The filaments are made from micron-sized ferromagnetic particles linked with DNA strands. It is found that at low frequencies of the rotating field a filament rotates synchronously with the field and beyond a critical frequency it undergoes a transition to a three dimensional regime. In this regime the tips of the filament rotate synchronously with the field on circular trajectories in the plane parallel to the plane of the rotating field. The characteristics of this motion found numerically match the experimental data and allow us to obtain the physical properties of such filaments. We als…
Diffusion in active magnetic colloids
2013
Abstract Properties of active colloids of circle swimmers are reviewed. As a particular example of active magnetic colloids the magnetotactic bacteria under the action of a rotating magnetic field is considered. The relation for a diffusion coefficient due to the random switching of the direction of rotation of their rotary motors is derived on the basis of the master equation. The obtained relation is confirmed by the direct numerical simulation of random trajectory of a magnetotactic bacterium under the action of the Poisson type internal noise due to the random switching of rotary motors. The results obtained are in qualitative and quantitative agreement with the available experimental r…
Dynamics of Uniaxial Hard Ellipsoids
2007
We study the dynamics of monodisperse hard ellipsoids via a new event-driven molecular dynamics algorithm as a function of volume fraction $\phi$ and aspect ratio $X_0$. We evaluate the translational $D_{trans}$ and the rotational $D_{rot}$ diffusion coefficient and the associated isodiffusivity lines in the $\phi-X_0$ plane. We observe a decoupling of the translational and rotational dynamics which generates an almost perpendicular crossing of the $D_{trans}$ and $D_{rot}$ isodiffusivity lines. While the self intermediate scattering function exhibits stretched relaxation, i.e. glassy dynamics, only for large $\phi$ and $X_0 \approx 1$, the second order orientational correlator $C_2(t)$ sho…
Neutron scattering and molecular correlations in a supercooled liquid
1999
We show that the intermediate scattering function $S_n(q,t)$ for neutron scattering (ns) can be expanded naturely with respect to a set of molecular correlation functions that give a complete description of the translational and orientational two-point correlations in the liquid. The general properties of this expansion are discussed with special focus on the $q$-dependence and hints for a (partial) determination of the molecular correlation functions from neutron scattering results are given. The resulting representation of the static structure factor $S_n(q)$ is studied in detail for a model system using data from a molecular dynamics simulation of a supercooled liquid of rigid diatomic m…
Transport coefficients of self-propelled particles: Reverse perturbations and transverse current correlations
2019
The reverse perturbation method [Phys. Rev. E 59, 4894 (1999)] for shearing simple liquids and measuring their viscosity is extended to the Vicsek model (VM) of active particles [Phys. Rev. Lett. 75, 1226 (1995)] and its metric-free version. The sheared systems exhibit a phenomenon that is similar to the skin effect of an alternating electric current: Momentum that is fed into the boundaries of a layer decays mostly exponentially toward the center of the layer. It is shown how two transport coefficients, i.e., the shear viscosity $\ensuremath{\nu}$ and the momentum amplification coefficient $\ensuremath{\lambda}$, can be obtained by fitting this decay with an analytical solution of the hydr…
JEM-X: three years in space
2006
We report on the technical and scientific performance of JEM-X, the X-ray monitor on ESA's INTEGRAL mission. INTEGRAL has now been in orbit for more than three years, and the mission is foreseen to be extended until the end of 2010. Overall, JEM-X performs very well, and can be expected to continue to do so for the duration of the mission. We discuss in some detail the operational experiences and the problems encountered with the microstrip detectors caused by the space environment and give one example of the interesting scientific results obtained. The analysis software is still being improved on, and we discuss briefly the significance of these improvements.