Search results for "Concentration."

showing 10 items of 1849 documents

Investigation of pH-Responsiveness inside Lipid Nanoparticles for Parenteral mRNA Application Using Small-Angle X-ray Scattering.

2020

Messenger ribonucleic acid (mRNA)-based nanomedicines have shown to be a promising new lead in a broad field of potential applications such as tumor immunotherapy. Of these nanomedicines, lipid-based mRNA nanoparticles comprising ionizable lipids are gaining increasing attention as versatile technologies for fine-tuning toward a given application, with proven potential for successful development up to clinical practice. Still, several hurdles have to be overcome to obtain a drug product that shows adequate mRNA delivery and clinical efficacy. In this study, pH-induced changes in internal molecular organization and overall physicochemical characteristics of lipoplexes comprising ionizable li…

In situPhospholipidNanoparticle02 engineering and technology010402 general chemistry01 natural sciencesDegree of ionizationchemistry.chemical_compoundElectrochemistryGeneral Materials ScienceRNA MessengerParticle SizeSpectroscopyChemistrySmall-angle X-ray scatteringX-RaysRNASurfaces and InterfacesHydrogen-Ion Concentration021001 nanoscience & nanotechnologyCondensed Matter PhysicsFluorescence0104 chemical sciencesMembraneBiophysicsNanoparticles0210 nano-technologyLangmuir : the ACS journal of surfaces and colloids
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Synthesis and antiproliferative activity of triazenoindazoles and triazenopyrazoles: a comparative study.

2003

Several triazenoindazoles and triazenopyrazoles were prepared transforming the appropriate aminoindazoles and aminopyrazoles in the corresponding diazonium salts which were reacted with dimethylamine, diethylamine and pyrrolidine. All the triazenes were tested for their antiproliferative activity against K562, HL60, L1210 and MCF7 cell lines. The biological data showed that the benzocondensation plays a positive role on the antiproliferative activity. The (1)H-NMR spectra showed that the rotational barrier around the N(2)-N(3) bond in the triazene group can be influenced both by the position of this group in the indazole nucleus and by the substitution pattern in the benzene moiety.

IndazolesMagnetic Resonance SpectroscopyHL60StereochemistryAntineoplastic AgentsMedicinal chemistryChemical synthesisPyrrolidinechemistry.chemical_compoundInhibitory Concentration 50Structure-Activity RelationshipDrug DiscoveryTumor Cells CulturedMoietyHumansTriazeneBenzeneDimethylaminePharmacologyDiethylamineIndazoleBicyclic moleculeMolecular StructureOrganic ChemistryGeneral MedicineSettore CHIM/08 - Chimica FarmaceuticachemistryPyrazolesTriazenoindazoles Triazenopyrazoles Antiproliferative activity Hindered rotationDrug Screening Assays AntitumorTriazenesCell DivisionEuropean journal of medicinal chemistry
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Validation of Dissolution Testing with Biorelevant Media: An OrBiTo Study.

2017

Dissolution testing with biorelevant media has become widespread in the pharmaceutical industry as a means of better understanding how drugs and formulations behave in the gastrointestinal tract. Until now, however, there have been few attempts to gauge the reproducibility of results obtained with these methods. The aim of this study was to determine the interlaboratory reproducibility of biorelevant dissolution testing, using the paddle apparatus (USP 2). Thirteen industrial and three academic laboratories participated in this study. All laboratories were provided with standard protocols for running the tests: dissolution in FaSSGF to simulate release in the stomach, dissolution in a singl…

IndolesInterlaboratory reproducibilityChemistry PharmaceuticalPhenylcarbamatesPharmaceutical ScienceIbuprofen02 engineering and technologyPharmacology030226 pharmacology & pharmacyBiopharmaceuticsTosyl Compounds03 medical and health sciences0302 clinical medicineDrug DiscoveryIntestine SmallDissolution testingTransfer modelDissolutionSulfonamidesChromatographyChemistryReproducibility of ResultsHydrogen-Ion Concentration021001 nanoscience & nanotechnologyDrug LiberationSolubilityGastric MucosaMolecular Medicine0210 nano-technologyTabletsMolecular pharmaceutics
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THIOPYRANO[2,3-E]INDOL-2-ONES: ANGELICIN HETEROANALOGUES WITH POTENT PHOTOANTIPROLIFERATIVE ACTIVITY

2008

A new class of compounds, the thiopyrano[2,3-e]indol-2-ones, bioisosters of the angular furocoumarin angelicin, was synthesized with the aim of obtaining new photochemotherapeutic agents. In particular 7,8-dimethyl-thiopyranoindolone 6c s showed a remarkable phototoxicity and a great dose UVA dependence reaching IC(50) values at submicromolar level. This latter photoinduced a massive apoptosis and a remarkable photodamage to lipids and proteins. Although it did not intercalate DNA, it was able to cause photooxidation of DNA bases.

IndolesStereochemistryDNA damageUltraviolet RaysAngelicinThiopyrano[23-e ]indol-2-oneClinical BiochemistryPharmaceutical ScienceHL-60 CellsApoptosisThiopyrano[2Antiproliferative activityBiochemistryChemical synthesischemistry.chemical_compoundInhibitory Concentration 50Jurkat CellsAngelicinPhotochemotherapeutic agentsFurocoumarinsDrug DiscoveryThiolactoneTumor Cells CulturedHumansPhotosensitizer3-e ]indol-2-onesMolecular BiologyPhotosensitizing AgentsFurocoumarinOrganic ChemistryProteinsBiological activityThiopyrano[2; 3-e ]indol-2-ones; Angelicin; Antiproliferative activity; Photochemotherapeutic agents; ApoptosisDNASettore CHIM/08 - Chimica FarmaceuticaMitochondriachemistryPhotochemotherapeutic agentMolecular MedicineLipid PeroxidationPhototoxicityDNA Damage
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Diacylglycerols containing Omega 3 and Omega 6 fatty acids bind to RasGRP and modulate MAP kinase activation.

2003

We elucidated the effects of different diacylglycerols (DAGs), i.e. 1-stearoyl-2-arachidonoyl-sn-glycerol (SAG), 1-stearoyl-2-docosahexaenoyl-sn-glycerol (SDG), and 1-stearoyl-2-eicosapentaenoyl-sn-glycerol (SEG), on [3H]PDBu binding to RasGRP. The competition studies with these DAGs on [3H]PDBu binding to RasGRP revealed different Ki values for these DAG molecular species. Furthermore, we transfected human Jurkat T cells by a plasmid containing RasGRP and assessed the implication of endogenous DAGs on activation of MAP kinases ERK1/ERK2, induced by phorbol-12-myristate-13-acetate (PMA). In control cells, GF109203X, a protein kinase C inhibitor, inhibited ERK1/ERK2 activation. However, this…

IndolesTime FactorsBiochemistryJurkat cellsMaleimideschemistry.chemical_compoundJurkat CellsGuanine Nucleotide Exchange FactorsEnzyme InhibitorsMitogen-Activated Protein Kinase 1Mitogen-Activated Protein Kinase 3KinaseFatty AcidsBrainTransfectionCell biologyDNA-Binding ProteinsBiochemistryEicosapentaenoic AcidDocosahexaenoic acidMitogen-activated protein kinasePhosphorylationTetradecanoylphorbol Acetatelipids (amino acids peptides and proteins)Arachidonic acidMitogen-Activated Protein KinasesPlasmidsProtein BindingDNA ComplementaryDocosahexaenoic AcidsMAP Kinase Signaling SystemImmunoblottingBiologyTransfectionBinding CompetitiveDiglyceridesInhibitory Concentration 50Fatty Acids Omega-6Fatty Acids Omega-3Escherichia coliAnimalsHumansCalphostinMolecular BiologyDose-Response Relationship Drugurogenital systemCell BiologyRatsEnzyme ActivationKineticschemistrybiology.proteinThe Journal of biological chemistry
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Industrial application of selected lactic acid bacteria isolated from local semolinas for typical sourdough bread production

2016

Abstract Four obligate heterofermentative lactic acid bacteria (LAB) strains (Weissella cibaria PON10030 and PON10032 and Leuconostoc citreum PON 10079 and PON10080) were tested as single strain starters, mono-species dual strain starters, and multiple strain starter for the preparation and propagation of sourdoughs for the production of a typical bread at industrial level. The kinetics of pH and TTA during the daily sourdough refreshments indicated a correct acidification process for all trials. The concentration of lactic and acetic acid increased consistently during fermentation. The resulting molar ratios between these two organic acids in the experimental trials were lower than those o…

Industrial application Leuconostoc citreum Sourdough Starter culture Typical bread Weissella cibaria0301 basic medicineFlour030106 microbiologyBiologymedicine.disease_causeMicrobiologySingle strainIndustrial Microbiology03 medical and health scienceschemistry.chemical_compoundAcetic acid0404 agricultural biotechnologyStarterLeuconostoc citreumIndustrial application Leuconostoc citreum Sourdough Starter culture Typical bread Weissella cibariamedicineLactic AcidFood scienceWeissella cibariaAcetic AcidPolymorphism Geneticdigestive oral and skin physiologyfood and beveragesBread04 agricultural and veterinary sciencesSettore AGR/15 - Scienze E Tecnologie AlimentariHydrogen-Ion Concentrationbiology.organism_classification040401 food scienceLactic acidchemistryWeissellaFermentationFood MicrobiologyFermentationLeuconostocBacteriaFood ScienceSettore AGR/16 - Microbiologia Agraria
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Clinical and Biological Characterization of Patients with Low/Intermediate-1 Risk Myelodysplastic Syndrome and Iron Overload

2012

Abstract Abstract 4956 Introduction. Patients with Myelodysplastic Syndrome (MDS) are susceptible to developing iron overload as a response to the red blood cell (RBC) transfusions and ineffective hematopoiesis. This iron overload (IOL) is characterized by an increase in oxygen-reactive species accompanied by a decrease in antioxidants, and results in hepatic, cardiac and endocrine disorders, as well as an increased risk of infection. Ineffective hematopoiesis promotes iron absorption at intestinal level. This process is enhanced by the presence of mutations in the hereditary hemochromatosis gene (HFE). This study aims to define the features that accompany patients with iron overload, compa…

Ineffective Hematopoiesismedicine.medical_specialtyPathologyLiver Iron Concentrationeducation.field_of_studybiologybusiness.industryImmunologyPopulationCell BiologyHematologyBiochemistryGastroenterologyRed blood cellmedicine.anatomical_structureAlanine transaminaseRefractory sideroblastic anemiaInternal medicineHereditary hemochromatosismedicinebiology.proteinChelation therapybusinesseducation
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Small angle neutron scattering study of the quaternary structure of haemocyanin of Rapana thomasiana

1996

Abstract Small angle neutron scattering (SANS) experiments were performed on a series of solutions of haemocyanin (Hc) of Rapana thomasiana . In a first series of solutions, by changing the external contrast a model of the molecule that is apparently in disagreement with electron microscopy (EM) measurements was obtained. The apparent disagreement was resolved by performing experiments on a series of variable protein concentration solutions in D 2 O. The physical parameters of the model, extrapolated to zero concentration, are in excellent agreement with the EM results obtained on samples more dilute than those examined with SANS.

Inorganic ChemistryCrystallographyRapana thomasianaSeries (mathematics)ChemistryOrganic ChemistryAnalytical chemistryMoleculeProtein quaternary structureSmall-angle neutron scatteringProtein concentrationSpectroscopyAnalytical ChemistryJournal of Molecular Structure
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Acid Titrations of poly(dG-dC).poly(dG-dC) in Aqueous Solution and in a w/o Microemulsion

2005

The model polynucleotide poly(dG-dC).poly(dG-dC) (polyGC) was titrated with a strong acid (HCl) in aqueous unbuffered solutions and in the quaternary w/o microemulsion CTAB/n-pentanol/n-hexane/water. The titrations, performed at several concentrations of NaCl in the range 0.005 to 0.600 M, were followed by recording the modifications of the electronic absorption and of the CD spectra (210or = lambdaor =350 nm) upon addition of the acid. In solution, the polynucleotide undergoes two acid-induced transitions, neither of which corresponds to denaturation of the duplex to single coil. The first transition leads to the Hoogsteen type synG.C+ duplex, while the second leads to the C+.C duplex. The…

Inorganic chemistryAnalytical chemistrySalt (chemistry)Sodium ChloridePolydeoxyribonucleotidesStructural BiologyMicroemulsionDenaturation (biochemistry)Molecular Biologychemistry.chemical_classificationAqueous solutionChemistryCircular Dichroismacid titrationWaterGeneral MedicineHydrogen-Ion ConcentrationmicroemulsionSolutionsIonic strengthPolynucleotideNucleic Acid ConformationEmulsionsSpectrophotometry UltravioletTitrationPolyGCAbsorption (chemistry)aqueous solutionJournal of Biomolecular Structure and Dynamics
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Alkaline titrations of poly(dG-dC).poly(dG-dC): microemulsion versus solution behaviour

2007

PolyGC was titrated with a strong base in the presence of increasing concentrations of NaCl (from 0.00 to 0.60M) either in water solution or with the polynucleotide solubilized in the aqueous core of reverse micelles, i.e., the cationic quaternary water-in-oil microemulsion CTAB/n-hexane/n-pentanol/water. The results for matched samples in the two media were compared. CD and UV spectroscopies and, for the solution experiments, pH measurements were used to follow the course of deprotonation. In both media the primary effect of the addition of base was denaturation of the polynucleotide, reversible by back-titration with a strong acid. In solution, the apparent pK(a) of the transition decreas…

Inorganic chemistryPolynucleotidesPolynucleotides; Alkaline titration; Reverse micelles; SpectroscopiesMicellepolynucleotideDeprotonationPolydeoxyribonucleotidesStructural Biologyalkaline titrationDenaturation (biochemistry)MicroemulsionMolecular BiologyAqueous solutionChemistryCetrimoniumCircular DichroismspectroscopiesGeneral MedicineHydrogen-Ion ConcentrationSolutionsFreeze Dryingreverse micelleIonic strengthPolynucleotideCetrimonium CompoundsNucleic Acid ConformationTitrationEmulsionsReverse micelles
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