Search results for "Consistent"

showing 10 items of 56 documents

Multi-scale multireference configuration interaction calculations for large systems using localized orbitals: Partition in zones

2012

A new multireference configuration interaction method using localised orbitals is proposed, in which a molecular system is divided into regions of unequal importance. The advantage of dealing with local orbitals, i.e., the possibility to neglect long range interaction is enhanced. Indeed, while in the zone of the molecule where the important phenomena occur, the interaction cut off may be as small as necessary to get relevant results, in the most part of the system it can be taken rather large, so that results of good quality may be obtained at a lower cost. The method is tested on several systems. In one of them, the definition of the various regions is not based on topological considerati…

010304 chemical physicsChemistryGeneral Physics and AstronomyMultireference configuration interactionMolecular orbital theory010402 general chemistry01 natural sciences0104 chemical sciencesLinear combination of atomic orbitalsMulti-configurational self-consistent field0103 physical sciencesMolecular orbitalComplete active spaceStatistical physicsPhysical and Theoretical ChemistryAtomic physicsBasis setNatural bond orbital
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Solution of the Skyrme-Hartree–Fock–Bogolyubovequations in the Cartesian deformed harmonic-oscillator basis. (VIII) hfodd (v2.73y): A new version of …

2017

We describe the new version (v2.73y) of the code HFODD which solves the nuclear Skyrme Hartree-Fock or Skyrme Hartree-Fock-Bogolyubov problem by using the Cartesian deformed harmonic-oscillator basis. In the new version, we have implemented the following new features: (i) full proton-neutron mixing in the particle-hole channel for Skyrme functionals, (ii) the Gogny force in both particle-hole and particle-particle channels, (iii) linear multi-constraint method at finite temperature, (iv) fission toolkit including the constraint on the number of particles in the neck between two fragments, calculation of the interaction energy between fragments, and calculation of the nuclear and Coulomb ene…

Angular momentumNuclear Theory[PHYS.NUCL]Physics [physics]/Nuclear Theory [nucl-th]SYMMETRYNuclear TheoryHartree–Fock methodGeneral Physics and AstronomyFOS: Physical sciencesGogny forceSkyrme interactionNuclear density functional theorySelf-consistent mean-field01 natural sciences114 Physical sciencesNuclear Theory (nucl-th)Energy density functional theorySYSTEMSQuantum mechanics0103 physical sciences010306 general physicsHarmonic oscillator[ PHYS.NUCL ] Physics [physics]/Nuclear Theory [nucl-th]PhysicsHartree–Fock–Bogolyubovta114010308 nuclear & particles physicsAugmented Lagrangian methodInteraction energyAngular-momentum projection113 Computer and information sciencesHardware and ArchitecturePairingIsospintheoretical nuclear physicsSelf-consistent mean fieldHartree-Fock-BogolyubovPairing correlations
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Linear scaling exchange gradients for Hartree–Fock and hybrid density functional theory

2000

Abstract A new method is introduced which allows to form the exchange part of self-consistent field energy gradients in a way which scales linearly with molecular size for molecules with a non-vanishing HOMO–LUMO gap. This is not only important for Hartree–Fock but as well for the popular hybrid density functional theory methods. The method preserves the optimized integral-driven structure of conventional direct methods. Efficiency and scaling behavior of the new method are illustrated for DNA fragments.

ChemistryMulti-configurational self-consistent fieldQuantum mechanicsHartree–Fock methodRestricted open-shell Hartree–FockGeneral Physics and AstronomyUnrestricted Hartree–FockDensity functional theoryStatistical physicsPhysical and Theoretical ChemistryScalingPost-Hartree–FockHybrid functionalChemical Physics Letters
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General occurrence of polar twisted minima in the ionic singlet excited surfaces of polyenes

1982

Except for a few cases, the lowest closed shell SCF solutions for the twisted geometries of polyenes involves delocalized nonpolarized MO’s, and represents a meaningless mixture of radicalar gound state and ionic excited states. Higher (quasi) solutions allow a realistic approach of the polarized ionic states. Orthogonality to the radicalar ground state may be imposed without important loss of energy. Further extensive CI does not modify significantly the situation. These statements are illustrated through ab initio calculations of butadiene and hexatriene. This approach allows us to show that slight distortions stablize polar minima even in ’’homosymmetric’’ molecules such as all‐trans hex…

ChemistryUNESCO::FÍSICAGeneral Physics and AstronomyIonic bondingElectronic structurePolyenesExcited StatesSelf−Consistent FieldDelocalized electronElectronic StructureAb initio quantum chemistry methods:FÍSICA [UNESCO]Polyenes ; Self−Consistent Field ; Electronic Structure ; Excited StatesExcited statePhysics::Atomic and Molecular ClustersSinglet statePhysical and Theoretical ChemistryAtomic physicsPhysics::Chemical PhysicsGround stateOpen shell
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Determination of single crystal elastic constants in textured polycrystalline materials: inverse approach coupling x-ray diffraction and self consist…

2004

La diffraction des rayons X couplee a l'utilisation d'un modele polycristallin (modele auto-coherent) est utilisee pour determiner les constantes d'elasticite monocristallines d'un materiau polycristallin texture. En effet, la connaissance du tenseur de rigidite elastique cijkl d'un solide est fondamentale pour les etudes s'attachant a la comprehension des proprietes mecaniques de la matiere (approches theoriques ou experimentales). Si, d'autres techniques permettent de determiner le tenseur d'elasticite d'un materiau (ultrasons par exemple), elles necessitent souvent l'utilisation d'un monocristal. Ceci n'est pas toujours realisable, en particulier pour des alliages de concentrations varia…

ChemistryX-ray crystallographyPhysical chemistrychemistry.chemical_elementMineralogyGeneral Materials ScienceCrystalliteSelf consistentSingle crystalCopperMatériaux & Techniques
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On the Efficiency of Affine Invariant Multivariate Rank Tests

1998

AbstractIn this paper the asymptotic Pitman efficiencies of the affine invariant multivariate analogues of the rank tests based on the generalized median of Oja are considered. Formulae for asymptotic relative efficiencies are found and, under multivariate normal and multivariatetdistributions, relative efficiencies with respect to Hotelling'sT2test are calculated.

CombinatoricsStatistics and ProbabilityMultivariate statisticsNumerical AnalysisRank (linear algebra)Consistent estimatorAffine invariantStatistics::MethodologyMultivariate normal distributionStatistics Probability and UncertaintyAsymptotic efficiency Oja median multivariate signed-rank test multivariate-rank test Pitman efficiencyMathematicsJournal of Multivariate Analysis
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On Contextuality in Behavioral Data

2015

Dzhafarov, Zhang, and Kujala (Phil. Trans. Roy. Soc. A 374, 20150099) reviewed several behavioral data sets imitating the formal design of the quantum-mechanical contextuality experiments. The conclusion was that none of these data sets exhibited contextuality if understood in the generalized sense proposed in Dzhafarov, Kujala, and Larsson (Found. Phys. 7, 762-782, 2015), while the traditional definition of contextuality does not apply to these data because they violate the condition of consistent connectedness (also known as marginal selectivity, no-signaling condition, no-disturbance principle, etc.). In this paper we clarify the relationship between (in)consistent connectedness and (non…

Computer scienceGeneral MathematicsFOS: Physical sciencesGeneral Physics and Astronomy01 natural sciences050105 experimental psychology0103 physical sciences0501 psychology and cognitive sciencescontextuality010306 general physicsta515Cognitive scienceQuantum Physics05 social sciencesta111General Engineeringcyclic systemsArticlesKochen–Specker theorem81P13 81Q99 60A99 81P13 81Q99 60A99 81P13 81Q99 60A99Formal designFOS: Biological sciencesQuantitative Biology - Neurons and Cognitionconsistent connectednessNeurons and Cognition (q-bio.NC)Quantum Physics (quant-ph)
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Shear Modulus of an Irreversible Diblock Copolymer Network from Self-Consistent Field Theory

2019

Using self-consistent field theory, we investigate the stretching-induced microphase separation in an irreversibly cross-linked polymer network composed of diblock copolymer chains and estimate its...

Condensed Matter::Soft Condensed MatterInorganic ChemistryShear modulusQuantitative Biology::BiomoleculesMaterials sciencePolymers and PlasticsPolymer networkOrganic ChemistryMaterials ChemistryCopolymerField theory (psychology)Composite materialSelf consistentMacromolecules
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The Relationship between the Italian Constitution and the European Convention on Human Rights

2016

The present paper deals with the Italian Constitutional Court approach to the application of the European Court of Human Rights decisions in the domestic legal order.

Consistent Interpretation Article 117.1 of the Italian Constitution Confiscation without condemnationSettore IUS/13 - Diritto Internazionale
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The Stackelberg equilibrium as a consistent conjectural equilibrium

2011

International audience; We consider a static game with conjectural variations where some firms make conjectures while others do not. Two propositions are proved. We first show that there exists a continuum of conjectural variations such that the conjectural equilibrium locally coincides with the Stackelberg equilibrium (Proposition 1). Second, we define the conditions under which a conjectural equilibrium is a locally consistent equilibrium (i.e. such that conjectures are fulfilled). The conceptof (local) consistency is restricted to firms making conjectures. Two conditions on consistency are featured: consistency within a cohort and consistency among cohorts. The Stackelberg equilibrium fu…

Consistent conjectural variations reaction functions Stackelberg competition[ SHS.ECO ] Humanities and Social Sciences/Economies and financesjel:D4[SHS.ECO] Humanities and Social Sciences/Economics and Finance[SHS.ECO]Humanities and Social Sciences/Economics and Financejel:L1Stackelberg Equilibrium
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