Search results for "Coulomb barrier"
showing 10 items of 54 documents
Trianionic gold clusters
2001
Using Penning-trap experiments and a shell-correction method incorporating ellipsoidal shape deformations, we investigate the formation and stability patterns of trianionic gold clusters. Theory and ex- periment are in remarkable agreement concerning appearance sizes and electronic shell eects. In contrast to multiply cationic clusters, decay of the trianionic gold clusters occurs primarily via electron autodetach- ment and tunneling through a Coulomb barrier, rather than via ssion. PACS. 36.40.Wa Charged clusters { 36.40.Qv Stability and fragmentation of clusters { 36.40.Cg Electronic and magnetic properties of clusters
Electron Binding in a Superatom with a Repulsive Coulomb Barrier: The Case of [Ag44(SC6H3F2)30]4– in the Gas Phase
2020
The electron binding mechanism in [Ag44(SC6H3F2)30]4- (SC6H3F2 = 3,4-difluorobenzenethiolate) tetra-anion was studied by photoelectron spectroscopy (PES), collision-induced dissociation mass spectrometry (CID-MS), and density functional theory (DFT) computations. PES showed that [Ag44(SC6H3F2)30]4- is energetically metastable with respect to electron autodetachment {[Ag44(SC6H3F2)30]3- + e-} and features a repulsive Coulomb barrier (RCB) with a height of 2.7 eV. However, CID-MS revealed that [Ag44(SC6H3F2)30]4- does not release an electron upon collisional excitation but undergoes dissociation. DFT computations performed on the known structure of [Ag44(SC6H3F2)30]4- confirmed the negative a…
Concept of a high-resolution online mass separator for the Munich fission fragment accelerator
1997
A fission fragment accelerator combined with the Munich high-flux reactor FRM-II is under design for the delivery of intense beams of mass separated very neutron-rich fission fragments with energies at the Coulomb barrier They can be used to produce very heavy neutron-rich nuclei in fusion reactions. The large neutron excess will result in much longer lifetimes of the produced heavy elements, compared to neutron-deficient ones produced in reactions with stable nuclear beams. Thus fast a-chains can no longer be used to identify the heavy reaction products. A new separator will be used consisting of a velocity filter, an ion guide system (IGISOL) and a Penning trap. The velocity filter separa…
Evidence for quasi-fission in40Ar+208Pb collisions near the coulomb-barrier
1987
Fission-fragment angular distributions were measured in the reaction of40Ar with208Pb near the fusion barrier. For nearly symmetric mass-/charge splits we find angular distributions symmetric around θ=90 degrees, however, with unusually large anisotropies. These develop gradually into forward-backward asymmetric distributions as one moves away from mass-/charge symmetry. This indicates that non-compound fission (‘quasi-fission’) competes with true fusion-fission. The relative contribution of quasi-fission to the total fission cross section is somewhere between 51 and 85%. In the framework of the extra-push model this is equivalent to an extra-extra push energy for compound-nucleus formation…
The REX-ISOLDE project
1998
Abstract REX-ISOLDE [1] is an experiment at ISOLDE/CERN with a twofold aim: (i) to demonstrate a novel efficient scheme for the acceleration of radioactive ions from the online mass separator ISOLDE to energies around the Coulomb barrier. (ii) to perform first nuclear physics experiments by studying the structure of the neutron-rich (N = 20, N = 28) nuclei by Coulomb excitation and neutron transfer reactions. An overview on the different components of the radioactive beam accelerator is given with special emphasis on the separation possibilities and ion number capabilities of the system.
Measurement of Evaporation Residue and Fission Cross Sections of the Reaction 30Si + 238U at Subbarrier Energies
2007
Effects of the prolate deformation of 238 U on fusion were studied in the reaction 30 Si + 238 U at bombarding energies close to the Coulomb barrier. The fission (capture) cross sections were measured at the JAEA tandem accelerator to see the enhancement of the cross sections in the subbarrier energy due to the lower Coulomb barrier in the collisions of projectile at the polar sides of 238 U. In order to obtain the direct evidence for complete fusion, evaporation residue cross sections were measured at UNILAC of GSI. At the subbarrier energy of Ec.m. = 133.0 MeV, where only polar collisions to 238 U occur, we measured three spontaneously fissioning nuclei which we assigned to the isotope 26…
Final State Three-Body Coulomb Effects in thePb208(B8,Be7p)Pb208Coulomb Breakup Reaction
2003
We present results of the first calculation of the double differential cross section for the 208Pb(8B,(7)Bep)208Pb Coulomb breakup reaction which treats the postdecay acceleration of the ejectiles within a genuine three-body approach. From this we conclude that, in order to minimize postdecay Coulomb acceleration effects, experiments should be performed at as small as possible scattering angles, not too low 7Be-p relative energies, and high incident energy.
Three-Body Coulomb Effects in the Direct Coulomb Breakup of 8B into 7Be + p in the Field of a 208Pb Ion
1999
The amplitude for the Coulomb breakup of a light nucleus in the field of a highly charged ion is considered in the framework of the distorted wave approach, with particular emphasis being laid on correctly taking into account the three-body Coulomb interactions in the final state. Numerical calculations have been performed for the double differential cross section for the reaction 208Pb(8B, 7Be p)208Pb. They clearly demonstrate the importance of long-range three-body Coulomb correlations in the astrophysically interesting regime when the ejectiles have the extremely small relative energies.
Positron-Electron Angular Correlations in Heavy Ion Collisions
1987
Recent measurements of positrons in coincidence with electrons emitted in U+Th collisions near the Coulomb barrier show sharp line structures in the sum and difference energy spectra of the two leptons (ref. 1). A possible method to clarify the origin of these lines is to study the angular correlation of the leptons. In this short contribution we want to report on a positron-electron coincidence test measurement performed with the TORI spectrometer. This apparatus offers the possibility to measure positrons in coincidence with electrons emitted into the same and opposite hemisphere as well.
Cross sections for nuclear reactions in collisions of238U+238U and238U +197Au near and below the coulomb barrier
1991
Cross sections for nuclear reactions at beam energies near and below the spherical Coulomb barrier V c were measured in the very heavy collision systems238U +238U and238U +197Au. The most probable reaction channel with mass transfer is the one-neutron transfer. Its excitation function is understood in terms of Rutherford trajectories together with the quantal process of neutron tunnelling over large distances. In addition, the exchange of up to 15 nucleons is observed down to 0.90 V c . The excitation functions for the multi-nucleon transfer products have much steeper slopes than that for one-neutron transfer, and are steeper for238U +197Au than for238U +238U, suggesting that nuclear contac…