Search results for "DIPOLE"

Coherent control of stimulated emission inside one-dimensional photonic crystals

2004

In this paper, the quasinormal mode (QNM) theory is applied to discuss the quantum problem of an atom embedded inside a one-dimensional (1D) photonic band gap (PBG) cavity pumped by two counterpropagating laser beams. The e.m. field is quantized in terms of the QNMs in the 1D PBG and the atom modeled as a two-level system is assumed to be weakly coupled to just one of the QNMs. The main result of the paper is that the decay time depends on the position of the dipole inside the cavity, and can be controlled by the phase difference of the two laser beams.

2011

Evidence for Pygmy and Giant Dipole Resonances inSn130andSn132

2005

The dipole strength distribution above the one-neutron separation energy was measured in the unstable $^{130}\mathrm{Sn}$ and the double-magic $^{132}\mathrm{Sn}$ isotopes. The results were deduced from Coulomb dissociation of secondary Sn beams with energies around $500\text{ }\text{ }\mathrm{MeV}/\mathrm{\text{nucleon}}$, produced by in-flight fission of a primary $^{238}\mathrm{U}$ beam. In addition to the giant dipole resonance, a resonancelike structure (``pygmy resonance'') is observed at a lower excitation energy around 10 MeV exhausting a few percent of the isovector $E1$ energy-weighted sum rule. The results are discussed in the context of a predicted new dipole mode of excess neut…

Sum Frequency Generation Spectra from Velocity-Velocity Correlation Functions: New Developments and Applications

2018

At the interface, the properties of water can be rather different from those observed in the bulk. In this chapter we present an overview of our computational approach to understand water structure and dynamics at the interface including atomistic and electronic structure details. In particular we show how Density Functional Theory-based molecular dynamics simulations (DFT-MD) of water interfaces can provide a microscopic interpretation of recent experimental results from surface sensitive vibrational Sum Frequency Generation spectroscopy (SFG). In our recent work we developed an expression for the calculation of the SFG spectra of water interfaces which is based on the projection of the at…

Finite perturbation calculations for the static dipole polarizabilities of the first-row atoms

1976

Static dipole polarizabilities are calculated from self-consistent-field and highly correlated wave functions for the ground states of the atoms Li through Ne. The correlation contributions to the polarizabilities are found to vary between -16% for Be and + 14% for F. The polarizabilities as obtained from the coupled-electron-pair approximation are expected to be accurate to about 2%.

Transition from Prolate to Oblate to Triaxial Shapes in158Yb

1983

The decay of the entry states in ISIYb populated in the reactions of 149 MeV ,oNe with ,44Nd and lUNd has been investigated with a 4" multidetector system gated by a Ge counter. The average excitation energy, the ,.-ray spectra and the angular distribu tions as a function of multiplicity show several changes in the ,.-ray decay. These changes suggest a transition from prolate to particle aligned oblate connguration at low spin. At 1- 38-48 collective transitions with dipole and quad­ rupole component possibly built on high K single particle states are observed. Furthennore, above 1- 48 the dipole component disappears suggesting a further change toward more triaxial shape.

Evidence for Three Microscopically Different Kinds of E1 Transitions in Lead-Region Nuclei

1986

One outstanding feature of the shell model in heavy nuclei is that within a main shell the single-particle transitions of electric dipole (E1) character are forbidden. This leads to the experimentally observed fact that the E1 transitions are usually hindered by a factor of about 10 with respect to the Weisskopf estimate. But since there is a dispersion of about two or three orders of magnitude among these hindrance factors, the isomeric E1 transitions have not been used to elucidate the mocroscopic properties of the involved states, as has been done for the E3 transitions of this nuclear region [1]. The E3 transitions often proceed via admixtures of the low-lying collective octupole state,…

Phase Transitions in Classical Fluids and Fluids with Internal Quantum States in Two Dimensions: Computer Simulations and Theory

1993

1)We investigate the properties of a model fluid whose molecules have classical degrees of freedom in two dimensions and two internal quantum states. The attractive interactions are “turned on” when the internal states are hybridized, corresponding to the molecules acquiring a “dipole” moment. The phase diagram of this system in the temperature- density plane is investigated by a combination of path integral Monte Carlo and block size analysis techniques. The results are compared with mean- field—theory predictions. 2) We present molecular dynamics simulation results of quenches into the unstable region of a two-dimensional Lennard-Jones system. The evolution of the system from the non-equi…

Residual fluctuations in the microwave background at large angular scales: Revision of the Sachs-Wolfe effect

1993

In this paper we revise the Sachs-Wolfe (SW) computation of large-scale an isotropies of the microwave background temperature, taking into account the properties of the metrics admitting an isotropic distribution of collisionless photons. We show that the metric used by SW belongs to the aforementioned class, and conclude that the microwave background (once the dipolar anisotropy has been subtracted) should now be isotropic at large angular scales, provided that it was isotropic on the last scattering surface and assuming that the growing mode of a pressureless Einstein-de Sitter perturbation is a good description of the metric.

Origin invariant calculation of optical rotation without recourse to London orbitals

2004

We propose an inherently origin invariant formulation of specific optical rotation obtained from the conventional velocity gauge expression by subtracting the static limit from the electric dipole-magnetic dipole polarizability: 〈〈p→,L→〉〉ω→〈〈p→,L→〉〉ω-〈〈p→,L→〉〉0. London (gauge including) atomic orbitals are therefore not needed to ensure origin invariance and, consequently, this modified velocity gauge formulation may be employed in conjunction with variational and non-variational quantum chemical methods alike. Sample calculations on S-propylene oxide and 3,4- methylenedioxymethamphetamine using self-consistent field and coupled cluster wave functions…