Search results for "ELECTRONIC STRUCTURE"

Measurement of the total width, the electronic width, and the mass of theΥ(10580)resonance

2005

We present a measurement of the parameters of the Υ(10580) resonance based on a dataset collected with the BABAR detector at the SLAC PEP-II asymmetric B factory. We measure the total width Γtot=(20.7±1.6±2.5)  MeV, the electronic partial width Γee=(0.321±0.017±0.029)  keV and the mass M=(10579.3±0.4±1.2)  MeV/c2.

A two-detector spectrometer for measurements of Doppler broadened positron annihilation spectra

2004

Abstract A two-detector spectrometer for measurements of Doppler broadened positron annihilation spectra has been constructed and tested. The energy difference of the annihilation quanta is measured in the analogue, not in the digital manner. The peak to background ratio in the measured spectra is of the order of 10 6 , the FWHM representing the energy resolution, equals to 1.1 keV , thus enabling the very subtle physical effects to be revealed. Some information on electronic structure of the investigated 3-d metals (Ti, V, Cr, Fe, Ni, Cu and Zn) has been determined using this spectrometer. It has been shown that the apparatus permits to detect the impurity-vacancy pairs in dilute nickel al…

Hard X-ray resonant electronic spectroscopy in transition metal oxides

2005

K-edge X-ray absorption and 2p-XPS spectra of 3d-element oxides present spectral features which cannot be explained within a simple one-electron model. These features reveal the fine electronic structure of transition metal (TM) oxides valence states resulting from hybridized TM-3d and O-2p states, and the correlations between these valence electrons. In this paper, we show how resonant electronic spectroscopy (resonant Auger or resonant photoelectron spectroscopy) around the TM K-edge can be used to interpret the structures of the threshold and, with the help of theoretical calculation, to determine the electronic configuration of the excited ion. Quadrupolar transitions towards localized …

Prospects for laser spectroscopy, ion chemistry and mobility measurements of superheavy elements in buffer-gas traps

2015

Abstract Laser spectroscopic methods are reviewed which are of potential interest for the investigation of atomic and ionic level structures of superheavy elements. The latter are defined here as the trans-fermium elements with Z > 100 for which no experimental atomic or ionic level structure information is known so far, and which cannot be bred in high flux nuclear power reactors via successive neutron capture. The principles of suitable laser spectroscopic methods are described, and illustrated by examples of real experiments. The addressed methods include single-ion spectroscopy in Paul traps, laser-induced fluorescence spectroscopy (LIF), radiation-detected optical pumping (RADOP), radi…

Hyperfine structure studies in the 6s 6p3P2-level of barium

1991

The hfs of the3P2 state of the 6s 6p configuration of atomic barium has been determined for137Ba, applying the collinear fast-beam laser spectroscopy. The data fill the last gap in the experimental information on low lying 6s2, 6s 6p, 6s 5d and 6p 5d configurations of this alcaline earth system. The results are analyzed in terms for the existing semi-empirical modified Breit-Wills theory (MBWT), working with two basic wave functions, as well as by an extension to six-component wave functions of inclusion of configuration interaction. The semi-empirical approaches lead to a consistent description of the different hyperfine structures; they are compared with the results from recent ab initio …

Average charge states of heavy and superheavy ions passing through a rarified gas: Theory and experiment

2013

The average charge states $\overline{q}$ of heavy and superheavy ions (atomic numbers $Z=80$--114) passing through He gas are studied experimentally and theoretically. Experimental data were measured at the gas-filled recoil separator, i.e., the TransActinide Separator and Chemistry Apparatus (TASCA) at GSI Darmstadt, for ion energies of a few hundred keV/u at gas pressures of 0.2 to 2.0 mbar. An attempt is made to describe experimental $\overline{q}$ values by means of atomic calculations of the binding energies and electron-loss and electron-capture cross sections. The influence of the gas-density effect is included in the calculations. The calculated $\overline{q}$ reproduce the experime…

Aluminum cluster anions: Photoelectron spectroscopy andab initiosimulations

2000

Atomic structures and geometries, electronic structure, and temperature-dependent photoelectron spectra of ${\mathrm{Al}}_{N}^{\ensuremath{-}} (N=19\ensuremath{-}102)$ clusters are studied both theoretically via ab initio local-density-functional simulations, and experimentally with high-resolution measurements. The use of a theoretically well-defined energy shift in conjunction with a generalized Koopmans' theorem enables direct comparisons between the calculated density of states and the experimental photoelectron spectrum. Such comparisons, using photoelectron spectra calculated for various relaxed cluster geometries, enables a determination of the optimal structures of the clusters. The…

2014

N-type CdO is a transparent conducting oxide (TCO) which has promise in a number of areas including solar cell applications. In order to realize this potential a detailed knowledge of the electronic structure of the material is essential. In particular, standard density functional theory (DFT) methods struggle to accurately predict fundamental material properties such as the band gap. This is largely due to the underestimation of the Cd 4d binding energy, which results in a strong hybridization with the valence-band (VB) states. In order to test theoretical approaches, comparisons to experiment need to be made. Here, synchrotron-radiation photoelectron spectroscopy (SR-PES) measurements are…

Electronic structure and positron states at vacancies in Si and GaAs

1986

Topological Signatures in the Electronic Structure of Graphene Spirals

2013

Topology is familiar mostly from mathematics, but also natural sciences have found its concepts useful. Those concepts have been used to explain several natural phenomena in biology and physics, and they are particularly relevant for the electronic structure description of topological insulators and graphene systems. Here, we introduce topologically distinct graphene forms - graphene spirals - and employ density-functional theory to investigate their geometric and electronic properties. We found that the spiral topology gives rise to an intrinsic Rashba spin-orbit splitting. Through a Hamiltonian constrained by space curvature, graphene spirals have topologically protected states due to tim…