Search results for "Excitation"
showing 10 items of 1290 documents
Performance of electro-optical plasmonic ring resonators at telecom wavelengths
2012
International audience; In this work we report on the characteristics of an electro-optical dielectric-loaded surface plasmon polariton waveguide ring resonator. By doping the dielectric host matrix with an electro-optical material and designing an appropriate set of planar electrodes, we measured a 16% relative change of transmission upon application of a controlled electric field. We have analyzed the temporal response of the device and conclude that electrostriction of the host matrix is playing a dominating role in the transmission response.
Efficient excitation of dielectric-loaded surface plasmon-polariton waveguide modes at telecommunication wavelengths
2008
International audience; The excitation of surface plasmon-polariton (SPP) waveguide modes in subwavelength dielectric ridges deposited on a thin gold film has been characterized and optimized at telecommunication wavelengths. The experimental data on the electromagnetic mode structure obtained using scanning near-field optical microscopy have been directly compared to full vectorial three-dimensional finite element method simulations. Two excitation geometries have been investigated where SPPs are excited outside or inside the dielectric tapered region adjoint to the waveguide. The dependence of the efficiency of the SPP guided mode excitation on the taper opening angle has been measured an…
Cylindrical metal-coated optical fibre devices for filters and sensors
1996
Novel fibre-optic components suitable for sensor applications and wavelength filters are reported. The devices consist of a tapered fibre whose uniform waist has been coated with a thin layer of gold. The operation principle is the resonant excitation of a surface plasma mode of the metal film.
Novel synthesis of up-conversion phosphor based on rare-earth doped NaLaF4
2011
In this work Er3+ doped NaLaF4 material has been synthesized Along with the description of the synthesis route, luminescence spectra and decay kinetics of both traditional and up-conversion luminescence of Er3+ will be presented for different Er3+ doping levels. It will be shown that the main mechanisms involved in the creation of the up-conversion luminescence in NaLaF4:Er3+ under excitation at about 975 nm are excited state absorption and energy transfer. Relative impact of either of the mechanisms in NaLaF4:Er3+ depends on both the concentration of Er3+ and on the excitation wavelength: the increase of either the concentration or the excitation wavelength leads to the prevalence of energ…
Efficient Hot Electron Transfer in Quantum Dot-Sensitized Mesoporous Oxides at Room Temperature
2018
Hot carrier cooling processes represent one of the major efficiency losses in solar energy conversion. Losses associated with cooling can in principle be circumvented if hot carrier extraction toward selective contacts is faster than hot carrier cooling in the absorber (in so-called hot carrier solar cells). Previous work has demonstrated the possibility of hot electron extraction in quantum dot (QD)-sensitized systems, in particular, at low temperatures. Here we demonstrate a room-temperature hot electron transfer (HET) with up to unity quantum efficiency in strongly coupled PbS quantum dot-sensitized mesoporous SnO2. We show that the HET efficiency is determined by a kinetic competition b…
EBIT diagnostics using X-ray spectra of highly ionized Ne
2003
We have carried out a detailed analysis of highly ionized neon spectra collected at the NIST EBIT using an NTD germanium X-ray microcalorimeter developed at the Harvard-Smithsonian Center for Astrophysics [Nucl. Instr. and Meth. A 444 (2000) 156]. Our attention was focused especially on the Ne IX He-like triplet to check electron density diagnostics through the intercombination/forbidden line ratio. We have investigated possible effects of the ion dynamics on the plasma emission line intensities, looking at the dependence of the count-rate and the charge state distribution on the electron beam energy and current. The temperature and spatial distribution of the neon ions, and hence the overl…
Ultrafast Dynamics of Dansylated POPAM Dendrimers and Energy Transfer in their Dye Complexes
2009
We have studied internal dynamics of dansylated poly(propyleneamine) dendrimers of different generations in solution and excitation energy transfer from dansyl chromophores to xanthene dyes that form van der Waals complexes with the dendrimers
Energy transfer to xanthene dyes in dansylated POPAM dendrimers
2011
Abstract Excitation energy transfer (EET) in host–guest complexes of dansylated POPAM dendrimers and xanthene dyes have been studied by transient absorption spectroscopy. EET from dansyl periphery to guests: rose bengal, eosin, or fluorescein, showed non-exponential behaviour as a result of distribution of donor–acceptor distances. Time constants range from 100 fs to 8 ps, independent of the dye and the dendrimer generation. Experiments suggested that in dendrimers binding more than one guest, EET among the guests becomes effective. Guest–host and guest–guest interactions induce non-radiative relaxation channels making excitation decays of the guests clearly faster in complexes than in solu…
Acoustic vibrations of metal nanoparticles: high order radial mode detection
2004
The vibrational radial modes of silver nanospheres embedded in a glass matrix are investigated using a high sensitivity femtosecond pump-probe technique. The results yield evidence for coherent launching of the fundamental and higher order radial modes in agreement with a sphere dilation mediated excitation model. The results are consistent with low-frequency Raman scattering experiments.
Hyperfine Paschen-Back regime realized in Rb nanocell
2012
A simple and efficient scheme based on one-dimensional nanometric thin cell filled with Rb and strong permanent ring magnets allowed direct observation of hyperfine Paschen-Back regime on D1 line in 0.5 - 0.7 T magnetic field. Experimental results are perfectly consistent with the theory. In particular, with sigma+ laser excitation, the slopes of B-field dependence of frequency shift for all the 10 individual transitions of 85,87Rb are the same and equal to 18.6 MHz/mT. Possible applications for magnetometry with submicron spatial resolution and tunable atomic frequency references are discussed.