Search results for "Exponent"
showing 10 items of 896 documents
Time-Resolved Coherent Anti-Stokes Raman Scattering of Graphene: Dephasing Dynamics of Optical Phonon.
2017
We report dynamics of the G-mode in graphene probed with time-resolved coherent anti-Stokes Raman scattering measurements. By applying BOXCARS excitation geometry with three different excitation wavelengths, various nonlinear processes can be selectively detected due to energy and momentum conservation and temporal sequence of the pulses. The Raman signal due to resonant coherent excitation of the G-mode shows exponential decay with lifetime of ∼325 ± 50 fs. This decay time is shorter than expected based on the line width of the G-mode in the Raman spectrum. We propose that the unexpectedly short dephasing time is a result of dynamic variation of nonadiabatic coupling of the photoexcited el…
Cathodoluminescence mechanism of crystalline Gd2SiO5:Ce
1993
Complex luminescence decay kinetics have been observed in Gd2SiO5:Ce crystals under electron beam irradiation. Absorption and photoluminescence excitation spectra, decay kinetics in various excitation bands over a wide range of photon energies from 3.6 to 7.0 eV in the temperature region from 80 to 400 K as well as the spectra of the glow curve creation efficiency at 80 K are examined. It is shown that the free electronic excitations produced, depending on the absorbed photon energy, have different recombination mechanisms finally leading to the radiative transitions between the 5d2E configuration and the 4f configuration of the Ce3+ ion. At hvexc < 6.1 eV a single exponential decay caused …
Temperature dependence of luminescence decay in Sn-doped silica
2005
We report an experimental study on the temperature dependence, in the range 18-300 K, of the decay kinetics of the emission at 4.1 eV from the first excited electronic state of oxygen deficient centers in a 2000 ppm Sn-doped sol-gel silica. At low temperature, this luminescence decays exponentially with a lifetime of 8.4 ns, whereas, on increasing the temperature, the time decay decreases and cannot be fitted with an exponential function. These results are expected if there is a competition between the radiative and the thermally activated intersystem-crossing decay channels toward the associated triplet state. The comparison with previous data in pure oxygen-deficient and Ge-doped silica g…
Luminescence of dense, octahedral structured crystalline silicon dioxide (stishovite)
2011
Abstract It is obtained that, as grown, non-irradiated stishovite single crystals possess a luminescence center. Three excimer pulsed lasers (KrF, 248 nm; ArF, 193 nm; F 2 , 157 nm) were used for photoluminescence (PL) excitation. Two PL bands were observed. One, in UV range with the maximum at 4.7±0.1 eV with FWHM equal to 0.95±0.1 eV, mainly is seen under ArF laser. Another, in blue range with the maximum at 3±0.2 eV with FWHM equal to 0.8±0.2 eV, is seen under all three lasers. The UV band main fast component of decay is with time constant τ =1.2±0.1 ns for the range of temperatures 16–150 K. The blue band decay possesses fast and slow components. The fast component of the blue band deca…
Sub-band-gap-excited luminescence of localized states in SiO2–Si and SiO2–Al glasses
2010
Abstract Silica glass samples doped with extra silicon (SiO 2 –Si: artificial oxygen deficiency) and with aluminum (SiO 2 –Al: Al-doped without accompanying alkali ions) were studied. The luminescence properties of these two samples are compared in the range of temperature 15–290 K under excitation of ArF excimer laser (193 nm). In both samples the luminescence of oxygen deficient centers (ODCs) is detected, i.e., emission bands in the blue at 440 nm and the UV at 280 nm. Cooling of the both samples led to strong increases of luminescence intensity down to 80 K with much smaller increases for still lower temperatures. At 290 K in SiO 2 –Si a luminescence similar to that of twofold-coordinat…
Effect of quantized conductivity on the anomalous photon emission radiated from atomic-size point contacts
2019
We observe anomalous visible to near-infrared electromagnetic radiation emitted from electrically driven atomic-size point contacts. We show that the number of photons released strongly depends on the quantized conductance steps of the contact. Counter-intuitively, the light intensity features an exponential decay dependence with the injected electrical power. We propose an analytical model for the light emission considering an out-of-equilibrium electron distribution. We treat photon emission as bremsstrahlung process resulting from hot electrons colliding with the metal boundary and a find qualitative accord with the experimental data.
Fracture Processes Observed with A Cryogenic Detector
2006
In the early stages of running of the CRESST dark matter search using sapphire detectors at very low temperature, an unexpectedly high rate of signal pulses appeared. Their origin was finally traced to fracture events in the sapphire due to the very tight clamping of the detectors. During extensive runs the energy and time of each event was recorded, providing large data sets for such phenomena. We believe this is the first time the energy release in fracture has been directly and accurately measured on a microscopic event-by-event basis. The energy threshold corresponds to the breaking of only a few hundred covalent bonds, a sensitivity some orders of magnitude greater than that of previou…
Diffusive behavior and the modeling of characteristic times in limit order executions
2007
We present an empirical study of the first passage time (FPT) of order book prices needed to observe a prescribed price change Delta, the time to fill (TTF) for executed limit orders and the time to cancel (TTC) for canceled ones in a double auction market. We find that the distribution of all three quantities decays asymptotically as a power law, but that of FPT has significantly fatter tails than that of TTF. Thus a simple first passage time model cannot account for the observed TTF of limit orders. We propose that the origin of this difference is the presence of cancellations. We outline a simple model, which assumes that prices are characterized by the empirically observed distribution …
Stringlike Cooperative Motion in a Supercooled Liquid
1998
Extensive molecular dynamics simulations are performed on a glass-forming Lennard-Jones mixture to determine the nature of the cooperative motions occurring in this model fragile liquid. We observe stringlike cooperative molecular motion (``strings'') at temperatures well above the glass transition. The mean length of the strings increases upon cooling, and the string length distribution is found to be nearly exponential.
Dynamics of correlations due to a phase noisy laser
2012
We analyze the dynamics of various kinds of correlations present between two initially entangled independent qubits, each one subject to a local phase noisy laser. We give explicit expressions of the relevant quantifiers of correlations for the general case of single-qubit unital evolution, which includes the case of a phase noisy laser. Although the light field is treated as classical, we find that this model can describe revivals of quantum correlations. Two different dynamical regimes of decay of correlations occur, a Markovian one (exponential decay) and a non-Markovian one (oscillatory decay with revivals) depending on the values of system parameters. In particular, in the non-Markovia…