Search results for "FOUNDATION"
showing 10 items of 256 documents
Nano-hygroscopicity tandem differential mobility analyzer (nano-HTDMA) for investigating hygroscopic properties of sub-10 nm aerosol nanoparticles
2020
Interactions between water and nanoparticles are relevant for atmospheric multiphase processes, physical chemistry, and materials science. Current knowledge of the hygroscopic and related physicochemical properties of nanoparticles, however, is restricted by the limitations of the available measurement techniques. Here, we present the design and performance of a nano-hygroscopicity tandem differential mobility analyzer (nano-HTDMA) apparatus that enables high accuracy and precision in hygroscopic growth measurements of aerosol nanoparticles with diameters less than 10 nm. Detailed methods of calibration and validation are provided. Besides maintaining accurate and stable sheath and a…
Determination and analysis of in situ spectral aerosol optical properties by a multi-instrumental approach
2014
Continuous in situ measurements of aerosol optical properties were conducted from 29 June to 29 July 2012 in Granada (Spain) with a seven-wavelength Aethalometer, a Multi-Angle Absorption Photometer, and a three-wavelength integrating nephelometer. The aim of this work is to describe a methodology to obtain the absorption coefficients (babs) for the different Aethalometer wavelengths. In this way, data have been compensated using algorithms which best estimate the compensation factors needed. Two empirical factors are used to infer the absorption coefficients from the Aethalometer measurements: C – the parameter describing the enhancement of absorption by particles in the filter matrix due …
In situ detection of atomic and molecular iodine using resonance and off-resonance fluorescence by lamp excitation: ROFLEX
2018
17 pags, 11 figs, 4 tabs
Measurement of low-ppm mixing ratios of water vapor in the upper troposphere and lower stratosphere using chemical ionization mass spectrometry
2018
A chemical ionization mass spectrometer (CIMS) instrument has been developed for the fast, precise, and accurate measurement of water vapor (H2O) at low mixing ratios in the upper troposphere and lower stratosphere (UT/LS). A low-pressure flow of sample air passes through an ionization volume containing an α-particle radiation source, resulting in a cascade of ion-molecule reactions that produce hydronium ions (H3O+) from ambient H2O. The production of H3O+ ions from ambient H2O depends on pressure and flow through the ion source, which were tightly controlled in order to maintain the measurement sensitivity independent of changes in the airborne sampling environment. The instrument w…
Consistency between GRUAN sondes, LBLRTM and IASI
2017
Abstract. Radiosonde soundings from the GCOS Reference Upper-Air Network (GRUAN) data record are shown to be consistent with Infrared Atmospheric Sounding Instrument (IASI)-measured radiances via LBLRTM (Line-By-Line Radiative Transfer Model) in the part of the spectrum that is mostly affected by water vapour absorption in the upper troposphere (from 700 hPa up). This result is key for climate data records, since GRUAN, IASI and LBLRTM constitute reference measurements or a reference radiative transfer model in each of their fields. This is specially the case for night-time radiosonde measurements. Although the sample size is small (16 cases), daytime GRUAN radiosonde measurements seem to h…
A new airborne tandem platform for collocated measurements of microphysical cloud and radiation properties
2009
Abstract. A new airborne tandem measurement platform for cloud-radiation interaction studies is introduced in this paper. It consists of a Learjet 35A research aircraft and the AIRcraft TOwed Sensor Shuttle (AIRTOSS), which is an instrumented drag-body towed by the Learjet. Currently, the AIRTOSS is instrumented with a Cloud Imaging Probe (CIP) for measuring cloud microphysical properties and an Inertial Navigation System (INS) for measurements of flight attitudes. The cable dragging AIRTOSS can be as long as four kilometres. Thus, truly collocated measurements in two altitudes above, in, and below clouds can be obtained. Results from first test flights with Learjet and AIRTOSS are reported…
Determination of alkylamines in atmospheric aerosol particles: a comparison of gas chromatography–mass spectrometry and ion chromatography approaches
2014
Abstract. In recent years low molecular weight alkylamines have been recognized to play an important role in particle formation and growth in the lower atmosphere. However, major uncertainties are associated with their atmospheric processes, sources and sinks, mostly due to the lack of ambient measurements and the difficulties in accurate quantification of alkylamines at trace level. In this study, we present the evaluation and optimization of two analytical approaches, i.e., gas chromatography–mass spectrometry (GC-MS) and ion chromatography (IC), for the determination of alkylamines in aerosol particles. Alkylamines were converted to carbamates through derivatization with isobutyl chlorof…
Potential of airborne lidar measurements for cirrus cloud studies
2014
Abstract. Aerosol and water vapour measurements were performed with the lidar system WALES of Deutsches Zentrum für Luft- und Raumfahrt (DLR) in October and November 2010 during the first mission with the new German research aircraft G55-HALO. Curtains composed of lidar profiles beneath the aircraft show the vertical and horizontal distribution and variability of water vapour mixing ratio and backscatter ratio above Germany. Two missions on 3 and 4 November 2010 were selected to derive the water vapour mixing ratio inside cirrus clouds from the lidar instrument. A good agreement was found with in situ observations performed on a second research aircraft flying below HALO. ECMWF analysis tem…
The Fifth International Workshop on Ice Nucleation phase 2 (FIN-02): Laboratory intercomparison of ice nucleation measurements
2018
The second phase of the Fifth International Ice Nucleation Workshop (FIN-02) involved the gathering of a large number of researchers at the Karlsruhe Institute of Technology's Aerosol Interactions and Dynamics of the Atmosphere (AIDA) facility to promote characterization and understanding of ice nucleation measurements made by a variety of methods used worldwide. Compared to the previous workshop in 2007, participation was doubled, reflecting a vibrant research area. Experimental methods involved sampling of aerosol particles by direct processing ice nucleation measuring systems from the same volume of air in separate experiments using different ice nucleating particle (INP) types, and coll…
3-D imaging and quantification of graupel porosity by synchrotron-based micro-tomography
2011
The air bubble structure is an important parameter to determine the radiation properties of graupel and hailstones. For 3-D imaging of this structure at micron resolution, a cryo-stage was developed. This stage was used at the tomography beamline of the Swiss Light Source (SLS) synchrotron facility. The cryo-stage setup provides for the first time 3-D-data on the individual pore morphology of ice particles down to infrared wavelength resolution. In the present study, both sub-mm size natural and artificial ice particles rimed in a wind tunnel were investigated. In the natural rimed ice particles, Y-shaped air-filled closed pores were found. When kept for half an hour at −8 °C, this morpholo…