Search results for "Heterostructure"

showing 10 items of 28 documents

High-Mobility, Wet-Transferred Graphene Grown by Chemical Vapor Deposition

2019

We report high room-temperature mobility in single layer graphene grown by Chemical Vapor Deposition (CVD) after wet transfer on SiO$_2$ and hexagonal boron nitride (hBN) encapsulation. By removing contaminations trapped at the interfaces between single-crystal graphene and hBN, we achieve mobilities up to$\sim70000cm^2 V^{-1} s^{-1}$ at room temperature and$\sim120000cm^2 V^{-1} s^{-1}$ at 9K. These are over twice those of previous wet transferred graphene and comparable to samples prepared by dry transfer. We also investigate the combined approach of thermal annealing and encapsulation in polycrystalline graphene, achieving room temperature mobilities$\sim30000 cm^2 V^{-1} s^{-1}$. These …

Materials scienceFOS: Physical sciencesGeneral Physics and AstronomyHexagonal boron nitride02 engineering and technologyChemical vapor deposition010402 general chemistrySettore ING-INF/01 - Elettronica01 natural scienceslaw.inventionlawMesoscale and Nanoscale Physics (cond-mat.mes-hall)General Materials ScienceDry transferCondensed Matter - Materials ScienceCondensed Matter - Mesoscale and Nanoscale PhysicsCharge carrier mobilityGrapheneSettore FIS/01 - Fisica Sperimentalecharge carrier mobilitygrapheneGeneral EngineeringMaterials Science (cond-mat.mtrl-sci)HeterojunctionheterostructureCVD021001 nanoscience & nanotechnologyCombined approach0104 chemical sciencesheterostructuresChemical engineeringCrystallitecharge carrier mobility; CVD; graphene; heterostructures; transfer;0210 nano-technologytransferACS Nano
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Facile synthesis of magnetically separable CoFe2O4/Ag2O/Ag2CO3 nanoheterostructures with high photocatalytic performance under visible light and enha…

2017

Riga Technical University supported the preparation of this manuscript from the Scientific Research Project Competition for Young Researchers No. ZP-2016/7. The authors wish to kindly acknowledge the financial support of HZB, Estonian Research Council (PUT1096, PUT735 and IUT2-25) and Estonian Centre of Excellence in Research Project “Advanced materials and high-technology devices for sustain-able energetics, sensorics and nanoelectronics” TK141 (2014–2020.4.01.15-0011).

Materials scienceMagneticNanoparticle02 engineering and technologyPhotocatalyticNanoheterostructures010402 general chemistryPhotochemistry01 natural sciencesSilver carbonatechemistry.chemical_compoundX-ray photoelectron spectroscopyPhase (matter):NATURAL SCIENCES:Physics [Research Subject Categories]Chemical Engineering (miscellaneous)PhotodegradationWaste Management and DisposalSilver carbonateta114Process Chemistry and Technology021001 nanoscience & nanotechnologyPollution0104 chemical scienceschemistryPhotocatalysis0210 nano-technologySilver oxideSilver oxideVisible spectrumJournal of Environmental Chemical Engineering
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Fast-Response Single-Nanowire Photodetector Based on ZnO/WS 2 Core/Shell Heterostructures

2018

This work was supported by the Latvian National Research Program IMIS2 and ISSP project for Students and Young Researchers Nr. SJZ/2016/6. S.P. is grateful to the ERA.Net RUS Plus WATERSPLIT project no. 237 for the financial support. S.V. is grateful for partial support by the Estonian Science Foundation grant PUT1689.

Materials scienceNanostructureScanning electron microscopeNanowirePhotodetector02 engineering and technology010402 general chemistry01 natural sciences7. Clean energysymbols.namesake:NATURAL SCIENCES:Physics [Research Subject Categories]General Materials Sciencecore/shell nanowirestransitional metal chalcogenidesvan der Waals epitaxybusiness.industryHeterojunction021001 nanoscience & nanotechnology0104 chemical sciencesTransmission electron microscopy1D/1D heterostructuressymbolsphotodetectorsOptoelectronicsCharge carrier0210 nano-technologybusinessRaman spectroscopyACS Applied Materials & Interfaces
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Strain relaxation, extended defects and doping effects in InxGa1-xN/GaN heterostructures investigated by surface photovoltage

2020

Abstract We have analysed electrical properties of extended defects and interfaces in fully strained and partially relaxed InxGa1-xN/GaN heterostructures by means of Kelvin probe force microscopy and surface photovoltage spectroscopy. The study highlights the role of indium incorporation and Si doping levels on the charge state of extended defects including threading dislocations, V defects and misfit dislocations. Surface potential maps reveal that these defects are associated with a different local work function and thus could remarkably alter electron-hole recombination mechanisms of InxGa1-xN/GaN layers locally. Surface photovoltage spectra clearly demonstrate the role of misfit disloca…

Materials scienceSurface photovoltageGeneral Physics and Astronomychemistry.chemical_element02 engineering and technology010402 general chemistryKelvin probe force microscopy01 natural sciencesSurface photovoltage spectroscopyWork functionSpectroscopyKelvin probe force microscopeCondensed matter physicsInxGa1-xN/GaN heterostructureRelaxation (NMR)DopingHeterojunctionSurfaces and InterfacesGeneral Chemistry021001 nanoscience & nanotechnologyCondensed Matter Physics0104 chemical sciencesSurfaces Coatings and Filmschemistry0210 nano-technologyIndium
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Enhancing triplet superconductivity by the proximity to a singlet superconductor in oxide heterostructures

2016

We show how in principle a coherent coupling between two superconductors of opposite parity can be realized in a three-layer oxide heterostructure. Due to strong intraionic spin-orbit coupling in the middle layer, singlet Cooper pairs are converted into triplet ones and vice versa. This results in a large enhancement of the triplet superconductivity, persisting well above the native triplet critical temperature.

OxideFOS: Physical sciences02 engineering and technology01 natural sciencesSuperconductivity (cond-mat.supr-con)Condensed Matter - Strongly Correlated Electronschemistry.chemical_compound0103 physical sciencesoxide heterostructureSinglet stateTriplet state010306 general physicsPhysicsSuperconductivityStrongly Correlated Electrons (cond-mat.str-el)Condensed matter physicsta114singlet Cooper pairsCondensed Matter - SuperconductivityParity (physics)Heterojunction021001 nanoscience & nanotechnology3. Good healthchemistrySinglet fissiontriplet superconductivityCooper pair0210 nano-technologyphysicsPhysical Review B
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Codeposition of Fe 3 O 4 nanoparticles sandwiched between g-C3N4 and TiO2 nanosheets: Structure, characterization and high photocatalytic activity fo…

2019

Novel ternary nanocomposite photocatalysts based on g-C3N4 /Fe3O4 /TiO2 nanosheet were synthesized using simple solid combustion, hydrothermal and wetness impregnation methods. The g-C3N4 nanosheet (2D)/ Fe3O4 /TiO2 nanosheet (2D) triad-interface nanocomposite arranged in the form of Fe 3 O 4 nanoparticle was sandwiched and effectively dispersed on the surface between g-C3N4 and TiO2 nanosheets. The synthesized composites were characterized by some specific techniques such as X-ray diffraction (XRD), Fourier transform infrared (FT-IR) spectroscopy, field emission scanning electronic microscopy (FE-SEM), transmission electron microscope (TEM), vibrating sample magnetometer (VSM), specific su…

Photocatalytic activitySettore CHIM/03 - Chimica Generale E InorganicaHeterostructurePhotocatalystSettore CHIM/07 - Fondamenti Chimici Delle TecnologieNanosheet
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A facile way to synthesize noble metal free TiO2 based catalysts for glycerol photoreforming

2023

In this work anaerobic heterogeneous photocatalytic solar/UV light reforming of glycerol in aqueous media was performed with Pt-photodeposition and noble metal free modified TiO2 photocatalysts prepared through ball milling, a very simple and cheap coupled catalyst preparation method. Different amounts of Cu2O or 3% CuO were loaded on TiO2 using ball milling and during each run glycerol conversion, hydrogen and CO2 formed in the gas phase and 1,3-dihydroxyacetone (DHA) and glyceraldehyde (GA) in the liquid phase were determined. The results were compared with the aim to verify the effectiveness of Cu2O in replacing Pt. Using noble metal free photocatalysts, 33% glycerol conversion, 10.3% an…

Settore ING-IND/24 - Principi Di Ingegneria ChimicaSettore ING-IND/23 - Chimica Fisica ApplicataHigh added value chemicalsGeneral Chemical EngineeringBall milling heterostructure formationTiO2Settore CHIM/07 - Fondamenti Chimici Delle TecnologieH2 productionPhotocatalytic glycerol partial oxidation
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Photoluminescence Enhancement by Band Alignment Engineering in MoS 2 /FePS 3 van der Waals Heterostructures

2022

Single-layer semiconducting transition metal dichalcogenides (2H-TMDs) display robust excitonic photoluminescence emission, which can be improved by controlled changes to the environment and the chemical potential of the material. However, a drastic emission quench has been generally observed when TMDs are stacked in van der Waals heterostructures, which often favor the nonradiative recombination of photocarriers. Herein, we achieve an enhancement of the photoluminescence of single-layer MoS2 on top of van der Waals FePS3. The optimal energy band alignment of this heterostructure preserves light emission of MoS2 against nonradiative interlayer recombination processes and favors the charge t…

Transition metal dichalcogenide monolayersAlignment engineeringVan der Waals heterostructuresEnhanced photoluminescenceOptoelectronic tunabilityGeneral Materials ScienceMaterialsACS Applied Materials & Interfaces
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Two-Dimensional Crystals and van der Waals Heterostructures based on Inorganic and Molecular Strongly Correlated Layered Materials

2021

“En resumen, toda obra grande es el fruto de la paciencia y de la perseverancia, combinadas con una atención orientada tenazmente durante meses y aun años hacia un objeto particular”. “In summary, all great work is the fruit of patience and perseverance, combined with tenacious concentration on a subject over a period of months or years”. Santiago Ramón y Cajal (Reglas y consejos sobre investigación científica. Madrid: Academia de Ciencias Exactas, Físicas y Naturales, 1897). The present Thesis constitutes a journey –a romance of many dimensions, quoting Edwin Abbot Abbot– from 3D to 2D and, hopefully (we let the curious Reader judge), “Through Flatland to Thoughtland” (citing, again, Abbot…

Two-Dimensional MaterialsSuperconductivityUNESCO::QUÍMICALayered MaterialsUNESCO::FÍSICAMagnetismSolid State ChemistryCondensed Matter Physics:QUÍMICA [UNESCO]Molecular materials:FÍSICA [UNESCO]van der Waals HeterostructuresStrongly Correlated Materials
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Hybrid heterostructures and materials based on transition metal dichalcogenides

2020

La irrupción de los nanomateriales en la vida moderna es un claro indicador del avance científico. El diseño de materiales a la carta permite establecer un control preciso sobre las propiedades finales de estos. El objetivo principal que ha motivado la presente Tesis es la combinación y funcionalización de láminas de MoS2 ultrafinas químicamente exfoliadas (ce-MoS2) con diferentes sistemas de base molecular. La Tesis se divide en los siguientes Capítulos: Capítulo I: En primer lugar, se introducen brevemente los nanomateriales. En segundo lugar, se describen los materiales bidimensionales (2D). A continuación, se detallan algunos aspectos generales de los dicalcogenuros de metales de transi…

UNESCO::QUÍMICAfunctionalizationcompositeheterostructureMoS2:QUÍMICA [UNESCO]
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