Search results for "IONIZATION"
showing 10 items of 1255 documents
First ionization potential of the heaviest actinide lawrencium, element 103
2016
The first ionization potential (IP1 ) of element 103, lawrencium (Lr), has been successfully determined for the first time by using a newly developed method based on a surface ionization process. The measured IP 1 value is 4.9630.08 0.07 eV. This value is the smallest among those of actinide elements and is in excellent agreement with the value of 4.963(15) eV predicted by state-of-the-art relativistic calculations also performed in this work. Our results strongly support that the Lr atom has an electronic configuration of [Rn]7s 2 5f 14 7p 1 1/2 , which is influenced by strong relativistic effects. The present work provides a reliable benchmark for theoretical calculations and also opens t…
Experimental investigation of electron impact onSi2−
2008
A merged beams technique has been used to investigate collisions between electrons and $\text{Si}_{2}{}^{\ensuremath{-}}$ ions over a relative kinetic energy range of 0--210 eV. Absolute cross sections for pure electron detachment, detachment plus dissociation, and dissociation involving atomic and ionic products were measured. The dominant process over the energy range studied is pure electron detachment. A search for a resonance associated with a ${\text{Si}}_{2}$ dianion was made but none was observed.
Nonlinear collective oscillations of an ion cloud in a Paul trap
1997
In an experiment using a Paul trap, we create a ${\mathrm{H}}_{2}^{+}$ ion cloud by electron ionization of the background gas at ${10}^{\ensuremath{-}9}$-mbar residual pressure. Exciting the ions parametrically at twice the frequency of the secular motion of ions in the $r$ or $z$ direction, we observe a narrow resonance at some distance from the motional resonance center if the amplitude of the exciting field exceeds a threshold value. The threshold value decreases with increasing ion number. Since the narrow resonance does not shift with ion number, we interpret it as a collective resonance of the center of mass of the ion cloud. The resonance shape exhibits the typical form of a driven a…
Method for estimating charge breeder ECR ion source plasma parameters with short pulse 1+ injection of metal ions
2020
Abstract A new method for determining plasma parameters from beam current transients resulting from short pulse 1+ injection of metal ions into a charge breeder electron cyclotron resonance ion source has been developed. The proposed method relies on few assumptions, and yields local values for the ionisation times 1 / n e σ v q → q + 1 inz , charge exchange times 1 / n 0 σ v q → q − 1 cx , the ion confinement times τ q , as well as estimates for the minimum plasma energy contents n e E e and the plasma triple products n e E e τ q . The method is based on fitting the current balance equation on the extracted beam currents of high charge state ions, and using the fitting coefficients to dete…
Cross Sections of232Th (p,xn+yp) Reactions at Ep= 6.8 to 20.2 MeV
1981
Cross-sections for the (p, n), (p, 2n), (p, 3n) and (p, pn) + (p, d) reactions on 232Th targets were measured, by comparison with the K-shell ionization cross-section, for proton energies between 6.8 and 20.2 MeV. The results are compared with the predictions of the statistical and the pre-equilibrium model. For the (p, pn) reaction, the "clean knock-out" model is also considered.
Determination of quantum defect for the Rydberg P series of Ca II
2019
We present an experimental investigation of the Rydberg 23 P$_{1/2}$ state of laser-cooled $^{40}$Ca$^+$ ions in a radiofrequency ion trap. Using micromotion sideband spectroscopy on a narrow quadrupole transition, the oscillating electric field at the ion position was precisely characterised, and the modulation of the Rydberg transition due to this field was minimised. From a correlated fit to this P line and previously measured P and F level energies of Ca II, we have determined the ionization energy of 95 751.916(32) $\rm {cm}^{-1}$, in agreement with the accepted value, and the quantum defect for the $n$ P$_{1/2}$ states.
High-field quantum calculation reveals time-dependent negative Kerr contribution
2013
The exact quantum time-dependent optical response of hydrogen under strong field near infrared excitation is investigated and compared to the perturbative model widely used for describing the effective atomic polarization induced by intense laser fields. By solving the full 3D time-dependent Schr\"{o}dinger equation, we exhibit a supplementary, quasi-instantaneous defocusing contribution missing in the weak-field model of polarization. We show that this effect is far from being negligible in particular when closures of ionization channels occur and stems from the interaction of electrons with their parent ions. It provides an interpretation to higher-order Kerr effect recently observed in v…
Photodetachment of F− by short laser pulses. Comparison between experiments and numerical results
2009
Recently, angle-resolved photoelectron spectra have been measured by exposing negative F− ions to linearly or circularly polarized infrared femtosecond laser fields. We compare the experimental results with numerical calculations carried out in the framework of a Keldysh-type theory modified to account for both the time shape and the spatial inhomogeneity of the pulse. In order to account for the finite duration of the laser pulse, our results have been obtained through calculations of photodetachment probabilities. By using the saddle-point method it is possible to show that the transition amplitude may be written as a coherent sum of terms giving rise to interferences. This circumstance s…
CONTROL OF RADIATIVE RECOMBINATION BY A STRONG LASER FIELD
2004
Strong-field laser-assisted radiation recombination is investigated: (a) to explore the control possibilities with two laser fields having commensurable frequencies and (b) to get some insight into the influence of the medium (a plasma) in which recombination occurs. It is found that by varying the relative phase of the two fields it is possible to control enhancement, broadening and symmetry properties of the recombination differential emitted power. In the case of an anisotropic two-temperature plasma, an interesting interplay is found between the shape of the laser-modified electron velocity distribution function and the shape of the emitted X-ray photon power spectrum. The novel feature…
Dynamics of H2 molecule driven by an ultra-short laser field
2004
We describe, using a semiclassical approach, the molecular dynamics of a one-dimensional H2 molecule interacting with a laser, beyond the Born–Oppenheimer approximation. We observe and discuss different molecular behaviors, such as ionization and dissociation.