Search results for "Magnetism"
showing 10 items of 1934 documents
Singlet-groundstate magnetism in TbP
1979
Elastic neutron scattering and magnetic susceptibility data are reported for temperatures around the Neel-point,TN=7.3 K, and for zero magnetic field. AboveTN, the temperature dependence of the magnetic central peak intensity can adequately be described within the RPA assuming isotropic exchange between nearest and next-nearest neighbours as the only parameters. This two-parameter model is quantitatively confirmed by the susceptibility data. AtTN, magnetic Bragg-intensities arise almost discontinuously (reaching 70% of the saturation within 0.1 K) accompanied by thermal hysteresis. For all temperatures belowTN the sublattice magnetic moment is explained by solutions of meanfield equations, …
Parallel implementation of the MAGPACK package for the analysis of high-nuclearity spin clusters
2010
Abstract Molecular clusters are formed by a finite number of exchange-coupled paramagnetic centers and they are model systems between molecules and extended solids. In order to simulate their properties and extrapolate to solids, the size of the systems to be treated should be as large as possible. In this context, the use of efficient parallel codes is essential. We present the parallel programs ParAni and ParIso , for anisotropic and isotropic models, that enable the calculation of large energy matrices in parallel and the subsequent computation of the relevant spectral information. The evaluation of the matrix elements is based on the serial package Magpack that uses the irreducible tens…
Second harmonic generation by an isolated spin
1970
Abstract The second harmonic generation at microwave frequency by a spin S = 1 2 in a cavity has been studied as a function of the external magnetic field using a resolvent technique, and the average transition rates to states with an increased number of double-frequency photons has been calculated. In spite of the crudeness of the model, a good qualitative agreement has been found between the predictions of the present theory and recent experimental results on non-linear behaviour of paramagnetic spin systems in a microwave field.
The Electric Field Gradient and the Quadrupole Interaction
1984
The Mossbauer effect has become a popular method in analytical chemistry. In contrast to other techniques such as x-ray spectroscopy, NMR, EPR, and MCD where highly sophisticated evaluation procedures are applied to obtain reliable information on the chemical compound, the Mossbauer effect is generally used on a low level concerning the evaluation of quadrupole split spectra. This procedure on a low level is favored by the structure of the spectra especially the simple doublet of the 3/2 → 1/2 nuclear transitions in paramagnetic and diamagnetic compounds. The separation of the two absorption lines, the quadrupole splitting ΔE Q and the center of the two lines, the isomer shift, are easily d…
Effects of the magnetodipolar interactions in the alternating magnetic fields
1999
A macroscopic theory for the description of the structure formation in a system of magnetic dipoles under the action of a high-frequency rotating field is presented. Continuum equations for the effective magnetic field strength describing particle interactions are derived. It is shown that, contrary to the case of a constant magnetic field, where the demagnetizing field arising from a concentration fluctuation stabilizes the system with respect to the phase separation, the same concentration fluctuation will be amplified in the case of a rotating magnetic field, leading to the formation of a layered structure. The extensions of the model necessary for the description of the formation of the…
Magnetization changes visualized using photoemission electron microscopy
2004
Abstract Photoemission electron microscopy was used to visualize the motion of magnetic domains on a sub-nanosecond timescale. The technique exploits the imaging of magnetic domains using soft X-ray circular dichroism, with the special feature that the instrument utilizes a fast image acquisition system with intrinsic 125 ps time resolution. The overall time resolution used is about 500 ps. Different domains and domain movements have been observed in lithographically-produced Permalloy structures on a copper microstrip-line. A current pulse of I=0.5 A with rise times of about 300 ps switched the Permalloy islands from a Landau-Lifshitz type domain configuration into metastable s-state domai…
Thermal disorder driven magnetic phases in van der Waals magnet CrI3
2020
Abstract Magnetic phase transitions often occur spontaneously at specific critical temperatures and are instrumental to understand the origin of long-range spin order in condensed matter systems. The presence of more than one critical temperature (Tc) has been observed in several compounds where the coexistence of competing magnetic orders highlights the importance of phase separation driven by different factors such as pressure, temperature and chemical composition. However, it is unknown whether recently discovered two-dimensional (2D) van der Walls (vdW) magnetic materials show such intriguing phenomena that can result in rich phase diagrams with novel magnetic features to be explored. H…
Suppression of carrier induced ferromagnetism by composition and spin fluctuations in diluted magnetic semiconductors
2001
We suggest an approach to account for spatial (composition) and thermal fluctuations in "disordered" magnetic models (e.g. Heisenberg, Ising) with given spatial dependence of magnetic spin-spin interaction. Our approach is based on introduction of fluctuating molecular field (rather than mean field) acting between the spins. The distribution function of the above field is derived self-consistently. In general case this function is not Gaussian, latter asymptotics occurs only at sufficiently large spins (magnetic ions) concentrations $n_i$. Our approach permits to derive the equation for a critical temperature $T_c$ of ferromagnetic phase transition with respect to the above fluctuations. We…
Pressure induced insulator/half-metal/metal transition in a strongly correlatedp-electron system
2012
Mixed-valent Rb${}_{4}$O${}_{6}$ provides an exceptional prototype material for studying the interplay between local correlations (Hubbard $U$) and electron kinetic energy ($W$) in the open $sp$-electron shell. Based on a first-principles calculation we show that depending on $U/W$ ratio, when tuned by external pressure, Rb${}_{4}$O${}_{6}$ exhibits a surprising sequence of phase transitions between strongly correlated antiferromagnetic insulator, ferromagnetic insulator ($U/W\phantom{\rule{-0.16em}{0ex}}\ensuremath{\gg}\phantom{\rule{-0.16em}{0ex}}1$), moderately correlated ferromagnetic half-metal ($U/W\phantom{\rule{-0.16em}{0ex}}\ensuremath{\sim}\phantom{\rule{-0.16em}{0ex}}1$), and fin…
Novel stripe textures in nonchiral hexatic liquid-crystal films
1992
A novel macroscopic stripe texture has been observed in freely suspended films of nonchiral liquid crystal, uniform stripes of alternating molecular orientation form spontaneously at the smectic-C--to--surface-hexatic phase transition and broaden with decreasing temperature. The stripes are identified as splay domains whose formation is attributed to the polar symmetry of the hexatic surface layers. Transverse (director bend) walls, which lead to an additional modulation of the basic one-dimensional pattern, are manifested inside thick circular islands as twelve-armed star defects.