Search results for "Mesoscale"
showing 10 items of 776 documents
Derivation of the universal decay cascade distribution
2014
A detailed derivation of the decay cascade probability distribution stated in Eqs. (4)-(6) and (11) of Phys. Rev. Lett. 104, 186805 (2010) [arXiv:0901.4102] by Kashcheyevs and Kaestner is provided. Recurrence relations are solved explicitly and connections between solutions in different limits are demonstrated.
Data mining, dashboard and statistical analysis: a powerful framework for the chemical design of molecular nanomagnets
2021
Three decades of research in molecular nanomagnets have raised their magnetic memories from liquid helium to liquid nitrogen temperature thanks to a wise choice of the magnetic ion and coordination environment. Still, serendipity and chemical intuition played a main role. In order to establish a powerful framework for statistically driven chemical design, we collected chemical and physical data for lanthanide-based nanomagnets, catalogued over 1400 published experiments, developed an interactive dashboard (SIMDAVIS) to visualise the dataset, and applied inferential statistical analysis. Our analysis showed that the Arrhenius energy barrier correlates unexpectedly well with the magnetic memo…
Strong Coupling of Coherent Phonons to Excitons in Semiconducting Monolayer MoTe$_2$
2023
The coupling of the electron system to lattice vibrations and their time-dependent control and detection provides unique insight into the non-equilibrium physics of semiconductors. Here, we investigate the ultrafast transient response of semiconducting monolayer 2$H$-MoTe$_2$ encapsulated with $h$BN using broadband optical pump-probe microscopy. The sub-40-fs pump pulse triggers extremely intense and long-lived coherent oscillations in the spectral region of the A' and B' exciton resonances, up to $\sim$20% of the maximum transient signal, due to the displacive excitation of the out-of-plane $A_{1g}$ phonon. Ab-initio calculations reveal a dramatic rearrangement of the optical absorption of…
Origin of the spin Seebeck effect probed by temperature dependent measurements in Gd$_{3}$Fe$_{5}$O$_{12}$
2014
We probe the spin Seebeck effect in Gd$_{3}$Fe$_{5}$O$_{12}$/Pt hybrid structures as a function of temperature and observe two sign changes of the spin Seebeck signal with decreasing temperature. A first sign change occurs at a temperature close to the Gd$_{3}$Fe$_{5}$O$_{12}$ magnetic compensation point at around 280 K. There the spin Seebeck signal changes sign abruptly with unaltered amplitude, indicating that the spin current is mainly caused by the magnetic Fe sub-lattices, which reorient their directions at this temperature. A second, more gradual sign change takes place around the ordering temperature of the Gd sub-lattice in the range of 65-85 K, showing that the Gd magnetic sub-lat…
Multiorbital exciton formation in an organic semiconductor
2023
Harnessing the optoelectronic response of organic semiconductors requires a thorough understanding of the fundamental light-matter interaction that is dominated by the excitation of correlated electron-hole pairs, i.e. excitons. The nature of these excitons would be fully captured by knowing the quantum-mechanical wavefunction, which, however, is difficult to access both theoretically and experimentally. Here, we use femtosecond photoemission orbital tomography in combination with many-body perturbation theory to gain access to exciton wavefunctions in organic semiconductors. We find that the coherent sum of multiple electron-hole pair contributions that typically make up a single exciton c…
Effective Seiberg-Witten gauge theory of noncollinear magnetism
2020
Smoothly varying magnetization textures such as domain walls, skyrmions or hopfions serve as promising candidates for the information bits of the future. Understanding their physical properties is both a major field of interest and a theoretical challenge, involving the physics on different length scales. Here, we apply the phase space formulation of quantum mechanics to magnetic insulators and metals in the limit of zero temperature to obtain a gradient expansion in terms of real-space derivatives of the magnetization. Our primary focus is the anomalous Hall effect in noncollinear magnets which serves as an important proxy in the detection of localized magnetic structures. We formulate the…
Atlas for the properties of elemental 2D metals
2018
Common two-dimensional (2D) materials have a layered 3D structure with covalently bonded, atomically thin layers held together by weak van der Waals forces. However, in a recent transmission electron microscopy experiment, atomically thin 2D patches of iron were discovered inside a graphene nanopore. Motivated by this discovery, we perform a systematic density-functional study on atomically thin elemental 2D metal films, using 45 metals in three lattice structures. Cohesive energies, equilibrium distances, and bulk moduli in 2D are found to be linearly correlated to the corresponding 3D bulk properties, enabling the quick estimation of these values for a given 2D metal and lattice structure…
Lanthanide molecular nanomagnets as probabilistic bits
2023
Abstract Over the decades, the spin dynamics of a large set of lanthanide complexes have been explored. Lanthanide-based molecular nanomagnets are bistable spin systems, generally conceptualized as classical bits, but many lanthanide complexes have also been presented as candidate quantum bits (qubits). Here we offer a third alternative and model them as probabilistic bits (p-bits), where their stochastic behavior constitutes a computational resource instead of a limitation. We present a modelling tool for molecular spin p-bits, we demonstrate its capability to simulate bulk magnetic relaxation data and ac experiments and to simulate a minimal p-bit network under realistic conditions. Final…
Low-frequency excitation of double quantum dots
2008
We address theoretically adiabatic regime of charge transport for a model of two tunnel-coupled quantum dots connected in series. The energy levels of the two dots are harmonically modulated by an external potential with a constant phase shift between the two. Motivated by recent experiments with surface-acoustic-wave excitation, we consider two situations: (a) pure pumping in the absence of external voltage (also at finite temperature), and (b) adiabatic modulation of the current driven by large external bias. In both cases we derive results consistent with published experimental data. For the case (b) we explicitly derive the adiabatic limit of Tien-Gordon formula for photon-assisted tunn…
Heat transfer across a vacuum gap induced by piezoelectrically mediated acoustic phonon tunneling
2023
In contradictin to the common concept that acoustic phonons can only travel inside a material medium, they can in fact "tunnel" across a vacuum gap with the help of piezoelectricity, transmitting a significantly stronger heat flux than that of blackbody radiation. Here, we present a theoretical formulation for the heat flux of such piezoelectrically mediated heat transfer, applicable to any anisotropic piezoelectric crystals with an arbitrary orientation. A few numerical results are demonstrated and compared to heat transfer driven by other close-range mechanisms, including near-field radiative heat transfer and other acoustic phonon tunneling mechanisms. We find that piezoelectrically medi…