Search results for "Metastability"
showing 10 items of 262 documents
K isomerism in Rf255 and total kinetic energy measurements for spontaneous fission of Rf255,256,258
2020
Spontaneous fission properties of the isotopes $^{255}\mathrm{Rf}$, $^{256}\mathrm{Rf}$, and $^{258}\mathrm{Rf}$ produced in the reactions $^{50}\mathrm{Ti}+^{207}\mathrm{Pb}$, $^{50}\mathrm{Ti}+^{208}\mathrm{Pb}$, and $^{50}\mathrm{Ti}+^{209}\mathrm{Bi}$ were studied. The method of time and position correlations was used to identify spontaneous fission events. The correction to the energy deficit in measured total kinetic energy (TKE) determined on the basis of a study of $^{252}\mathrm{No}$ was applied to evaluate the $\overline{\mathrm{TKE}}$ of investigated rutherfordium isotopes. A signature which we assigned tentatively to bimodal fission was observed in TKE distributions of $^{255}\m…
New shape isomer in the self-conjugate nucleus $^{72}$Kr
2003
A new isomeric ${0}^{+}$ state was identified as the first excited state in the self-conjugate ($N=Z$) nucleus $^{\mathrm{72}}\mathrm{K}\mathrm{r}$. By combining for the first time conversion-electron and gamma-ray spectroscopy with the production of metastable states in high-energy fragmentation, the electric-monopole decay of the new isomer to the ground state was established. The new ${0}^{+}$ state is understood as the band head of the known prolate rotational structure, which strongly supports the interpretation that $^{\mathrm{72}}\mathrm{K}\mathrm{r}$ is one of the rare nuclei having an oblate-deformed ground state. This observation gives in fact the first evidence for a shape isomer…
STRUCTURAL INSTABILITY IN FERROELECTRICS: SUPERIMPOSING HAMILTONIAN AND STOCHASTIC DYNAMICS
2008
ABSTRACT Structural instability of ferroelectrics distinguished by appearance of coexisting phases and spatial inhomogeneity is at variance with the predictions of statistics in the canonical ensemble. A more refined description includes ergodicity breaking which become apparent at critical temperature when the system resides in metastable state and its development lead to one of possible minimum energy states. In this study the domain growth and switching is reproduced within the framework of Fokker-Planck approach. The mathematical technique is developed for empiric Landau Hamiltonians and improved for application to first principles effective Hamiltonians with supercells and elementary l…
Theory of radiative recombination from the metastable excited states of quantum dots
1998
The radiative recombination of an exciton ~electron-hole pair! confined in a semiconductor quantum dot is studied within a general model based on the effective-mass approximation. The dependence of the photoluminescence spectrum on the size of the dot and the magnetic field describe well a series of recent experimental results. In particular, a characteristic splitting of the main photoluminescence peak into a doublet or triplet is observed at the critical size and magnetic field, as a consequence of the appearance of metastable states in the exciton spectrum. @S0163-1829~98!06915-X#
Stable and metastable hard-sphere crystals in fundamental measure theory
2013
Using fully minimized fundamental measure functionals, we investigate free energies, vacancy concentrations and density distributions for bcc, fcc and hcp hard-sphere crystals. Results are complemented by an approach due to Stillinger which is based on expanding the crystal partition function in terms of the number n of free particles while the remaining particles are frozen at their ideal lattice positions. The free energies of fcc/hcp and one branch of bcc agree well with Stillinger's approach truncated at n=2. A second branch of bcc solutions features rather spread-out density distributions around lattice sites and large equilibrium vacancy concentrations and is presumably linked to the …
Transitions between metastable states in silica clusters
1999
Relaxation phenomena in glasses can be related to jump processes between different minima of the potential energy in the configuration space. These transitions play a key role in the low temperature regime, giving rise to tunneling systems responsible for the anomalous specific heat and thermal conductivity in disordered solids with respect to crystals. By using a recently developed numerical algorithm, we study the potential energy landscape of silica clusters, taking as a starting point the location of first order saddle points. This allows us to find a great number of adjacent minima. We analyze the degree of cooperativity of these transitions and the connection of physical properties wi…
Inelastic neutron scattering study of the rotational excitations in(KBr)1−x(KCN)xin the paraelastic and structural glass state
1984
The coupled rotational-translational excitations in ${(\mathrm{KBr})}_{1\ensuremath{-}x}{(\mathrm{KCN})}_{x}$ were studied by inelastic neutron scattering for concentrations $0.008\ensuremath{\le}x\ensuremath{\le}0.20$. We followed the ${A}_{1g}\ensuremath{-}{T}_{2g}$ tunneling transition and the ${A}_{1g}\ensuremath{-}{E}_{g}$ librational excitation through the transition from the paraelastic to the structural glass state. We found that these two excitations and their coupling to the lattice strains exhibit a very different temperature dependence in the glass state. While the tunneling transition, which triggers reorientations of the ${\mathrm{CN}}^{\ensuremath{-}}$ ions, shows a drastic r…
Intrinsic localized excitations in nonlinear lattices: Heuristic explanation for the nature of polar nanoregions?
2010
The study is addressed to a topical problem of self-localization in condensed state with special emphasis on a class of complex oxides categorized as ferroelectric relaxors. Basically, their anomalous temperature response is associated with the dynamics of microscopic scale polar regions supported by somewhat artificial metastable configurations. A unified approach to the spontaneous emergence and stability of the polar nanoregions is assigned to intrinsic localized excitations in Hamiltonian lattices with nonlinearity and non-Gibbsian statistics as necessary and sufficient ingredients of the theory.
Number of metastable states of a chain with competing and anharmonicΦ4−like interactions
1993
We investigate the number of metastable configurations of a Φ 4 -like model with competing and anharmonic interactions as a function of an effective coupling constant η. The model has piecewise harmonic nearest-neighbor and harmonic next-nearerst-neighbor interactions. The number M of metastable states in the configuration space increases exponentially with the number N of particles: M∞exp(vN). It is shown numerically that, outside the previously considered range |η|<1/3, v is approximately linearly decreasing with η for |η|<1 and that v=0 for η≥1. These findings can be understood by describing the metastable configurations as an arrangement of kink solitons whose width creases with η
CONSTRUCTION OF METASTABLE STATES IN QUANTUM ELECTRODYNAMICS
2004
In this paper, we construct metastable states of atoms interacting with the quantized radiation field. These states emerge from the excited bound states of the non-interacting system. We prove that these states obey an exponential time-decay law. In detail, we show that their decay is given by an exponential function in time, predicted by Fermi's Golden Rule, plus a small remainder term. The latter is proportional to the (4+β)th power of the coupling constant and decays algebraically in time. As a result, though it is small, it dominates the decay for large times. A central point of the paper is that our remainder term is significantly smaller than the one previously obtained in [1] and as…