Search results for "Nonlinear optic"
showing 10 items of 530 documents
Solution-processed transparent ferroelectric nylon thin films
2019
We have developed a method to solution process strongly hydrogen-bonded odd nylons into ferroelectric thin films.
Unusual response to environmental polarity in a nonlinear-optical benzylidene-type chromophore containing a 1,3-bis(dicyanomethylidene)indane accepto…
2017
One of the strongest known electron-accepting fragments used in the synthesis of organic dyes for applications in nonlinear optics (NLO) is 1,3-bis(dicyanomethylidene)indane (BDMI). By studying a benzylidene-type push-pull chromophore bearing a 5-carboxy-BDMI electron-acceptor and 4-(dimethylamino)aniline donor fragment, we demonstrate that this class of compounds can show unusual response to the polarity of the surrounding medium. The combined results of UV-Vis absorption spectrometry, NMR experiments and computational modeling indicate that the studied compound undergoes a geometrical transformation that involves an increase in the torsion angle ω between the aniline and indane ring syste…
Modulating the polarization of broadband terahertz pulses from a spintronic emitter at rates up to 10 kHz
2021
Reliable modulation of terahertz electromagnetic waveforms is important for many applications. Here, we rapidly modulate the direction of the electric field of linearly polarized terahertz electromagnetic pulses with 1–30 THz bandwidth by applying time-dependent magnetic fields to a spintronic terahertz emitter. Polarity modulation of the terahertz field with more than 99% contrast at a rate of 10 kHz is achieved using a harmonic magnetic field. By adding a static magnetic field, we modulate the direction of the terahertz field between angles of, for instance, −53° and 53° at kilohertz rates. We believe our approach makes spintronic terahertz emitters a promising source for low-noise modula…
Influence of Ag, Cu dopants on the second and third harmonic response of ZnO films
2009
International audience; Silver- and copper-doped ZnO films were prepared by radio-frequency (RF)-magnetron sputtering on glass and quartz substrates. The influence of dopants content on the microstructural evolution and optical as well as nonlinear optical (NLO) properties were investigated. It has been found that the grain sizes were enlarged with increasing of Ag, Cu dopants amount in ZnO films. The Ag or Cu doping leads to the optical band gap narrowing. Besides, the second-order NLO response of Ag- and Cu-doped ZnO films is lower than that of undoped ZnO film. The second harmonic generation (SHG) efficiency of the ZnO:Ag film was found to be higher than that of the ZnO:Cu film at the si…
Non-critically phase-matched cascaded THG at 440 nm in KTiOP1−yAsyO4 crystals
1995
Abstract We report the relative nonlinear optical properties of flux-grown KTiOP 1− y As y O 4 crystals ( y =0, y =0.03 and y =0.12). The non-critical phase-matching temperatures along the x -axis for blue generation by type II indirect third harmonic generation from 1318.8 nm and 1320 nm are measured. The phosphorus-arsenic substitution allows a “chemical tuning” of the phase-matching properties, through a birefringence variation, so that non-critical phase-matching at room temperature is possible for the previous interactions. Type II frequency doubling from 1064 nm is briefly considered.
Temperature dependence of refractive index and absorption coefficient of GaSe at 633 nm
1995
Abstract Measurements of the ordinary refractive index and the absorption coefficient ( E /t] to c axis ) of gallium selenide at 633 nm, in the temperature range [20,100] °C, are reported. Useful analytical approximations obtained after a least squares fitting process are provided, as well. These results are basic for any theoretical model of nonlinear and bistable optical devices based on GaSe.
Chalcogenide Glasses Based on Germanium Disulfide for Second Harmonic Generation
2007
International audience; High second-order susceptibilities are created by thermal poling in bulk germanium disulfide based chalcogenide glasses. Experimental conditions of the poling treatment (temperature, voltage, time) were optimized for each glass composition. The second-order nonlinear signals were recorded by using the Maker fringes experiment and a second-order coefficient χ(2) up to 8 pm V-1 was measured in the Ge25Sb10S65 glass. This value is obtained using a simulation based on accurate knowledge of the thickness of the nonlinear layer. Two mechanisms are proposed to explain the creation of a nonlinear layer under the anode: the formation and the migration of charged defects towar…
Nonlinear Disorder Mapping via Three Wave Mixing in Poled Lithium Tantalate
2010
We introduce and test a simple approach for the characterization of domain distribution in bulk quadratic ferroelectric crystals, such as periodically poled Lithium Tantalate with random mark-to space ratio.
Three-Dimensional Printing of Nonlinear Optical Lenses.
2018
In the current paper, a series of nonlinear optical (NLO) active devices was prepared by utilizing stereolithographic three-dimensional printing technique. Microcrystalline NLO active component, urea, or potassium dihydrogen phosphate was dispersed in a simple photopolymerizable polyacrylate-based resin and used as the printing material to fabricate highly efficient transparent NLO lenses. The nonlinear activity of the printed lenses was confirmed by second-harmonic generation measurements using a femtosecond laser-pumped optical parametric amplifier operating at a wavelength of 1195 nm. The three-dimensional printing provides a simple method to utilize a range of NLO active compounds witho…
<title>Effects of light polarization and crystal orientation on the holographic recording efficiency in doped LiNbO<formula><inf>&l…
2008
The holographic recording efficiency in doped LiNbO3 crystals has been studied both experimentally and theoretically depending on the type of dope, on the recording geometry and on the polarizations of the recording and readout light.. The studied crystals can be arranged in the following order by their efficiency: LiNbO3:Cu, LiNbO3:Fe (yet having a smaller thickness and donor concentration than LiNbO3:Cu), LiNbO3:Fe+Cu, LiNbO3:Fe+Ti, LiNbO3:Ti. It was found that the recording geometry with the holographic grating vector along the optical axis is much more efficient than in the perpendicular configuration.This fact is in accordance with the photorefraction theory based on photogalvanic and …