Search results for "RADII"
showing 10 items of 18 documents
Le spine di Afranio: a proposito di Afran. fr. 1 R.3
2022
In fr. I R.3 (Afranius’ Abducta) we can recognise an imagery connected to the rhetorical-philosophical Stoic tradition. Indeed, the adjective senticosus introduces the metaphor of thorns, a stylistic device associated with the Stoic sermo. This interpretation seems to be confirmed by Apuleius’ use of this adjective in Florida 18, which contains the famous ‘sophism of Protagoras’.
Preparation and Characterization of P2 BCh Ring Systems (Ch=S, Se) and Their Reactivity with N-Heterocyclic Carbenes
2018
Four-membered rings with a P2BCh core (Ch = S, Se) have been synthesized via reaction of phosphinidene chalcogenide (Ar*P=Ch) and phosphaborene (Mes*P=BNR2). The mechanistic pathways towards these rings are explained by detailed computational work that confirmed the preference for the formation of P–P, not P–B, bonded systems, which seems counterintuitive given that both phosphorus atoms contain bulky ligands. The reactivity of the newly synthesized heterocycles, as well as that of the known (RPCh)n rings (n = 2, 3), was probed by the addition of Nheterocyclic carbenes, which revealed that all investigated compounds can act as sources of low-coordinate phosphorus species. peerReviewed
Evidence of a sudden increase in the nuclear size of proton-rich silver-96
2021
Understanding the evolution of the nuclear charge radius is one of the long-standing challenges for nuclear theory. Recently, density functional theory calculations utilizing Fayans functionals have successfully reproduced the charge radii of a variety of exotic isotopes. However, difficulties in the isotope production have hindered testing these models in the immediate region of the nuclear chart below the heaviest self-conjugate doubly-magic nucleus 100Sn, where the near-equal number of protons (Z) and neutrons (N) lead to enhanced neutron-proton pairing. Here, we present an optical excursion into this region by crossing the N = 50 magic neutron number in the silver isotopic chain with th…
Analytic response relativistic coupled-cluster theory: the first application to indium isotope shifts
2019
With increasing demand for accurate calculation of isotope shifts of atomic systems for fundamental and nuclear structure research, an analytic energy derivative approach is presented in the relativistic coupled-cluster theory framework to determine the atomic field shift and mass shift factors. This approach allows the determination of expectation values of atomic operators, overcoming fundamental problems that are present in existing atomic physics methods, i.e. it satisfies the Hellmann-Feynman theorem, does not involve any non-terminating series, and is free from choice of any perturbative parameter. As a proof of concept, the developed analytic response relativistic coupled-cluster the…
Proton-neutron pairing correlations in the self-conjugate nucleus 42Sc
2021
Collinear laser spectroscopy of the N=Z=21 self-conjugate nucleus 42Sc has been performed at the JYFL IGISOL IV facility in order to determine the change in nuclear mean-square charge radius between the Iπ=0+ ground state and the Iπ=7+ isomer via the measurement of the 42g,42mSc isomer shift. New multi-configurational Dirac-Fock calculations for the atomic mass shift and field shift factors have enabled a recalibration of the charge radii of the 42−46Sc isotopes which were measured previously. While consistent with the treatment of proton-neutron, proton-proton and neutron-neutron pairing on an equal footing, the reduction in size for the isomer is observed to be of a significantly larger m…
Deformation and mixing of coexisting shapes in neutron-deficient polonium isotopes
2015
Coulomb-excitation experiments are performed with postaccelerated beams of neutron-deficient Po196,198,200,202 isotopes at the REX-ISOLDE facility. A set of matrix elements, coupling the low-lying states in these isotopes, is extracted. In the two heaviest isotopes, Po200,202, the transitional and diagonal matrix elements of the 2+1 state are determined. In Po196,198 multistep Coulomb excitation is observed, populating the 4+1,0+2, and 2+2 states. The experimental results are compared to the results from the measurement of mean-square charge radii in polonium isotopes, confirming the onset of deformation from Po196 onwards. Three model descriptions are used to compare to the data. Calculati…
High precision hyperfine measurements in Bismuth challenge bound-state strong-field QED
2017
Electrons bound in highly charged heavy ions such as hydrogen-like bismuth 209Bi82+ experience electromagnetic fields that are a million times stronger than in light atoms. Measuring the wavelength of light emitted and absorbed by these ions is therefore a sensitive testing ground for quantum electrodynamical (QED) effects and especially the electron–nucleus interaction under such extreme conditions. However, insufficient knowledge of the nuclear structure has prevented a rigorous test of strong-field QED. Here we present a measurement of the so-called specific difference between the hyperfine splittings in hydrogen-like and lithium-like bismuth 209Bi82+,80+ with a precision that is improve…
Testing for goodness rather than lack of fit of an X–chromosomal SNP to the Hardy-Weinberg model
2019
The problem of checking the genotype distribution obtained for some diallelic marker for compatibility with the Hardy-Weinberg equilibrium (HWE) condition arises also for loci on the X chromosome. The possible genotypes depend on the sex of the individual in this case: for females, the genotype distribution is trinomial, as in the case of an autosomal locus, whereas a binomial proportion is observed for males. Like in genetic association studies with autosomal SNPs, interest is typically in establishing approximate compatibility of the observed genotype frequencies with HWE. This requires to replace traditional methods tailored for detecting lack of fit to the model with an equivalence test…
Characterization of Flux-Grown SmxNd1–xVO4 Compounds and High-Pressure Behavior for x = 0.5
2019
The crystal structure and the vibrational and optical characteristics of flux-grown mixed lanthanide vanadate compounds SmxNd1–xVO4 (x = 0, 0.1, 0.25, 0.5, 0.75 and 1) are reported. A linear, monot...
Triplet 12B-12C-12N : Search for States with Halo
2020
Previously in [1] neutron halo was confirmed for the 2¯, 1.67 MeV and 1¯, 2.62 MeV states in 12B on base of Asymptotic Normalization Coefficients (ANC) method analysis of the obtained experimental data. An unexpected result was received for the unbound 3¯, 3.39 MeV state. Its halo radius was found to be increased and equal to ~5.9 fm. This result can be considered as an evidence of the halo-like structure in this 12B state. It should be noted that last neutron in this state has a non-zero orbital momentum (l = 2). So question arises about possible existence of states with halo in other members of the isobaric triplet 12B–12C–12N. We can expect the formation of a proton halo in the 2¯, 1.19 …