Search results for "RADIOCHEMISTRY"
showing 10 items of 273 documents
Neutron–gamma mixed field measurements by means of MCP–TLD600 dosimeter pair
2007
Abstract In this paper, we compared the TL response of three types of thermoluminescence dosimeters, TLD600 (6LiF:Mg,Ti), TLD700 (7LiF:Mg,Ti) and MCP (LiF:Mg,Cu,P) after exposure to a n–γ mixed field in the fluence range of radiotherapeutic applications. Since a dosimeter pair is required to discriminate the two components of the mixed field, we analyzed the ability of each dosimeter pair to provide the fluence value in the mixed field. At this aim we performed a 60Co–γ calibration and a neutron calibration for all three dosimeter types. Finally, a blind test was performed in order to analyze the accuracy of each dosimeter pair and we found that in this mixed field the fluence value obtaine…
Production of radioactive Ag ion beams with a chemically selective laser ion source
1997
Abstract We have developed a chemically selective laser ion source at the CERN-ISOLDE facility in order to study neutron-rich Ag nuclides. A pulsed laser system with high repetition rate has been used based on high-power coppe-vapour pump lasers and dye lasers. With this source significant reductions of the isobaric background has been achieved.
Separation of fission products by the ion guide fed isotope separator, IGISOL
1987
Abstract The performance of the ion guide method in the on-line mass separation of fission products has been investigated. Activity was produced by bombarding nat. U targets with a beam of 20 MeV protons. All the mass chains from A = 95 through A = 120 have been scanned using conventional methods of nuclear spectroscopy. No chemical selectivity in the separation was observed; isotopes of highly nonvolatile elements from yttrium to palladium were produced with efficiencies equal to those for the more volatile ones. The boundary of known neutron-rich nuclides was reached throughout the mass region from A = 106 to A = 118. During the course of this preliminary study the new isotope 116 Rh was …
Tritium release from beryllium articles for use in fusion devices
2009
Abstract Results obtained on radiation and magnetic field (MF) effects on tritium release at annealing of the beryllium pebbles from the EXOTIC-8-3/13 irradiation are presented in this study and compared with those for other irradiated beryllium materials. Abundance ratios of chemical forms of tritium in the EXOTIC-8-3/13 beryllium pebbles were determined: T 2 – 65%, T 0 – 23%, T + – 12%. A complete detritiation of these pebbles was achieved at 1123 K for 240 min; MF of 2.35 T had no appreciable effect on the tritium release. At 991 K for 240 min, the degree of detritiation was 96.6% without MF; MF of 2.35 T decreased it to 86.7%. At 940 K for 47 min, the degree of detritiation was 60%, 5 M…
Very high specific activity erbium 169Er production for potential receptor-targeted radiotherapy
2019
Erbium 169Er is one of the most interesting radiolanthanides for new potential receptor-targeted β− therapy applications due to its low energy β− emissions, very low intensity ɣ rays and the possibility to use 68Ga or 44Sc as companion for diagnostic in a theranostics approach. Currently it can be produced in reactors through the neutron activation of highly enriched 168Er. The low specific activity of the produced carrier-added 169Er is limiting its use for receptor-targeted therapy. Nonetheless it is used for radiosynoviorthesis of small joints. The aim of this work is to develop a new large-scale production method for the supply of very high specific activity 169Er. Highly enriched 168Er…
Ion beam analysis and alpha spectrometry of sources electrodeposited on several backings
1998
Abstract Alpha sources of several activities were prepared by electrodeposition of natural uranium onto four different backings: stainless steel, Ni, Mo and Ti. The influence of the activity, the type of backing, and the process of heating the source on the energy resolution of the spectra were investigated using alpha spectrometry and Rutherford Backscattering Spectrometry (RBS) techniques. Diffusion profiles of the radioactive deposits in the backings were obtained from RBS and related to the results using alpha spectrometry
First intense isotopic titanium-50 beam using MIVOC method
2012
Abstract An organometallic compound isotopically enriched in titanium-50 has been successfully used for the first time to produce intense ion beams with an ECR ion source by means of the MIVOC method. After some fruitful tests performed with compounds produced at IPHC Strasbourg with natural titanium, enriched organometallic titanium compound was produced successfully, beam extracted from ECR ion sources and accelerated through a K = 130 MeV cyclotron to an energy of 242 MeV. This isotopic 50 Ti 11 + beam was used for the first time in three week-experiment with typical MIVOC stable operating conditions. After optimization, up to 19.4 μA of titanium-50 in charge state 11 + could be extracte…
Production of neutron-rich surface-ionized nuclides at PARRNe
2002
Yields of neutron-rich isotopes produced by fast neutron induced fission of 238 U were measured at the ISOL set-up Production dAtomes Radioactifs Riches en Neutrons. A surface ion source was used to ionize selectively elements with low ionization potentials. In order to observe also the most n-rich isotopes, the identification was achieved by a combined measurement of b- and c-rays and b-delayed neutrons. The flux of fast neutrons inducing fission was generated by a 1 lA beam of 26 MeV deuterons stopped in a graphite converter. The target was a standard ISOLDE type 238 UC
A new pulsed release method for element selective production of neutron rich isotopes near 208Pb
1998
Abstract A new method to reduce the isobaric contamination problem for the production of neutron rich Bi, Pb and Tl nuclei at on-line mass separators, based on the pulsed release of these radioactive species, is presented. The results of a feasibility study are reported.
On-line yields obtained with the ISOLDE RILIS
2003
The ISOLDE resonance ionization laser ion source (RILIS) allows to ionize efficiently and selectively many metallic elements. In recent yield surveys and on-line experiments with the ISOLDE RILIS we observed 23–34 Mg, 26–34 Al, 98–132 Cd, 149 Tb, 155–177 Yb, 179–200 Tl, 183–215 Pb and 188–218 Bi. The obtained yields are presented together with measured release parameters which allow to extrapolate the release efficiency towards more exotic (short-lived) nuclides of the same elements. 2002 Elsevier Science B.V. All rights reserved.