Search results for "SURFACE PLASMON"

Optical response and shapes of charged sodium clusters; an analogue of the nuclear giant dipole response

1995

Collective vibrations of de-localized electrons against the positive charged ionic background in sodium clusters (plasmon resonances) and the collective vibrations of protons against neutrons in nuclei (giant dipole resonances) have several features in common. However, fundamental differences exist due to differences in the two media; the nucleus is a quantum liquid whereas the metallic medium is more like a plasma with classical positive ions and quantized electrons. The similarities and differences are illustrated by results from optical response measurements for charged sodium clusters with 14 to 48 atoms.

2014

We present a unified framework for the description of the interaction of fast electrons with complex nanostructures based on the Green dyadic method. We show that the computation of a generalized field propagator yields the electron energy losses and cathodoluminescence of nano-objects of arbitrary morphologies embedded in complex dielectric media. Spectra and maps for both penetrating and non-penetrating electron trajectories are provided. This numerical approach can be extended to describe complex experiments involving fast electrons and optically excited nanostructures.

Imaging Surface Plasmons

2012

Controlling surface plasmons is at the heart of plasmonics. Advances in this field are to a large extent triggered by our ability to visualize surface plasmons in their different forms. In this chapter, we provide a review of the different techniques capable of imaging and visualizing surface plasmons. We have divided these techniques in three distinct families: proximal probe techniques, far-field microscopies, and electron imaging. We review here their principal characteristics, advantages, and limitations and illustrate the discussion with images taken from the literature.

Selective excitation of bright and dark plasmonic resonances of single gold nanorods.

2015

Plasmonic dark modes are pure near-field resonances since their dipole moments are vanishing in far field. These modes are particularly interesting to enhance nonlinear light-matter interaction at the nanometer scale because radiative losses are mitigated therefore increasing the intrinsic lifetime of the resonances. However, the excitation of dark modes by standard far field approaches is generally inefficient because the symmetry of the electromagnetic near-field distribution has a poor overlap with the excitation field. Here, we demonstrate the selective optical excitation of bright and dark plasmonic modes of single gold nanorods by spatial phase-shaping the excitation beam. Using two-p…

Many-body origin of the plasmon resonance in small metal clusters

1994

The origin of the plasmon excitation in small metal clusters is studied within the jellium model through ab initio electronic-structure calculations based on the nuclear shell model. In the limit of infinite size, the plasmon classically represents pure harmonic motion of the center of mass of the valence electrons. It is shown that this limit is already well approximated by clusters of only eight electrons.

Soliplasmon excitations at metal/dielectric/Kerr structures

2009

We present novel optical phenomena based on the existence of a new type of quasi-particle excitation in metal/dielectric/Kerr structures. We discuss the possibility of excitation of surface plasmon polaritons via spatial solitons in these systems.

Plasmon excitations in chemically heterogeneous nanoarrays

2020

| openaire: EC/H2020/838996/EU//RealNanoPlasmon The capability of collective excitations, such as localized surface plasmon resonances, to produce a versatile spectrum of optical phenomena is governed by the interactions within the collective and single-particle responses in the finite system. In many practical instances, plasmonic metallic nanoparticles and arrays are either topologically or chemically heterogeneous, which affects both the constituent transitions and their interactions. Here, the formation of collective excitations in weakly Cu- and Pd-doped Au nanoarrays is described using time-dependent density functional theory. The additional impurity-induced modes in the optical respo…

Unguided plasmon-mode resonance in optically excited thin film: exact modal description of Kretschmann–Raether experiment

2013

With the aim of studying electromagnetic surface wave resonance, we rigorously solve the homogeneous and inhomogeneous problem associated with an optically excited thin metallic film. We then demonstrate unambiguously that the excited eigenmode engendering plasmonic resonance in the so-called Kretschmann–Raether configuration is an unguided mode (i.e., with an anti-evanescent structure). This result, challenging the classical interpretation of the outgoing wave condition applied to surface waves, permits a quantitative interpretation of the attenuated total reflection curves.

Electron-gas clusters: the ultimate jellium model

1995

The local spin-density approximation is used to calculate ground- and isomeric-state geometries of jellium clusters with 2 to 22 electrons. The positive background charge of the model is completely deformable, both in shape and in density. The model has no input parameters. The resulting shapes of the clusters exhibit breaking of axial and inversion symmetries; in general the shapes are far from ellipsoidal. Those clusters which lack inversion symmetry are extremely soft against odd-multipole deformations. Some clusters can be interpreted as molecules built from magic clusters. The deformation produces a gap at the Fermi level. This results in a regular odd-even staggering of the total ener…

Quantum emitter states dressed by the plasmon modes of a metal nanoparticle in the strong coupling regim

2017

The quantum control of emitters is a key issue for quantum information processing at the nanoscale. This generally necessitates the strong coupling of emitters to a high Q-cavity for efficient manipulation of the atoms and field dynamics (cavity quantum electrodynamics or cQED). Since almost a decade, strong efforts are put to transpose cQED concepts to plasmonics in order to profit of the strong mode confinement of surface plasmons polaritons. Despite the intrinsic presence of lossy channels leading to strong decoherence in plasmonics systems, it has been experimentally proven that it is possible to reach the strong coupling regim [1].