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showing 10 items of 4920 documents
Probing the Conformational States of a pH-Sensitive DNA Origami Zipper via Label-Free Electrochemical Methods
2021
Funding Information: Financial support from EPSRC DTP (grant EP/R513349/1), the Emil Aaltonen Foundation, the Sigrid Jusélius Foundation, the Jane and Aatos Erkko Foundation, and the Vilho, Yrjö and Kalle Väisälä Foundation of the Finnish Academy of Science and Letters is gratefully acknowledged. This work was carried out under the Academy of Finland Centers of Excellence Programme (2014–2019). We acknowledge the provision of facilities and technical support by Aalto University Bioeconomy Facilities and OtaNano—Nanomicroscopy Center (Aalto-NMC) and Micronova Nanofabrication Center. Publisher Copyright: © 2021 The Authors. Published by American Chemical Society DNA origami structures represe…
Internally Contracted Multireference Coupled Cluster Calculations with a Spin-Free Dirac-Coulomb Hamiltonian: Application to the Monoxides of Titaniu…
2017
We combine internally contracted multireference coupled cluster theory with a four-component treatment of scalar-relativistic effects based on the spin-free Dirac–Coulomb Hamiltonian. This strategy allows for a rigorous treatment of static and dynamic correlation as well as scalar-relativistic effects, which makes it viable to describe molecules containing heavy transition elements. The use of a spin-free formalism limits the impact of the four-component treatment on the computational cost to the non-rate-determining steps of the calculations. We apply the newly developed method to the lowest singlet and triplet states of the monoxides of titanium, zirconium, and hafnium and show how the in…
Region-based segmentation on depth images from a 3D reference surface for tree species recognition.
2013
International audience; The aim of the work presented in this paper is to develop a method for the automatic identification of tree species using Terrestrial Light Detection and Ranging (T-LiDAR) data. The approach that we propose analyses depth images built from 3D point clouds corresponding to a 30 cm segment of the tree trunk in order to extract characteristic shape features used for classifying the different tree species using the Random Forest classifier. We will present the method used to transform the 3D point cloud to a depth image and the region based segmentation method used to segment the depth images before shape features are computed on the segmented images. Our approach has be…
Manufacturing and characterization of single cell intermediate-temperature solid oxide fuel cells for APU in transportation application
2014
The fabrications of large area IT-SOFC planar cell by new simple and cost effective process were explained. The optimization of the new process with respect to pore formers, thickness of layers, sintering temperature were performed. The electrochemical results of 10cm2 performed in Fiaxell open flange set up were detailed with respect to different configuration. Long term ageing performance tests of single cells were conducted in Fiaxell device and results are discussed. Preparation of new test bench and stacking process performed till now were briefed.
Titan's 3-micron spectral region from ISO high-resolution spectroscopy
2006
Abstract The near-infrared spectrum of Titan, Saturn's largest moon and one of the Cassini/Huygens' space mission primary targets, covers the 0.8 to 5 micron region in which it shows several weak CH 4 absorption regions, and in particular one centered near 2.75 micron. Due to the interference of telluric absorption, only part of this window region (2.9–3.1 μm) has previously been observed from the ground [Noll, K.S., Geballe, T.R., Knacke, R., Pendleton, F., Yvonne, J., 1996. Icarus 124, 625–631; Griffith, C.A., Owen, T., Miller, G.A., Geballe, T., 1998. Nature 395, 575–578; Griffith, C.A., Owen, T., Geballe, T.R., Rayner, J., Rannou, P., 2003. Science 300, 628–630; Geballe, T.R., Kim, S.J.…
Titan's surface and atmosphere from Cassini/VIMS data with updated methane opacity
2013
International audience; We present an analysis of Titan data acquired by the Cassini Visual and Infrared Mapping Spectrometer (VIMS), making use of recent improvements in methane spectroscopic parameters in the region 1.3-5.2 μm. We first analyzed VIMS spectra covering a 8 × 10-km2 area near the Huygens landing site in order to constrain the single scattering albedo (ω0) of the aerosols over all of the VIMS spectral range. Our aerosol model agrees with that derived from Huygens Probe Descent Imager/Spectral Radiometer (DISR) in situ measurements below 1.6 μm. At longer wavelengths, ω0 steadily decreases from 0.92 at 1.6 μm to about 0.70 at 2.5 μm and abruptly drops to about 0.50 near 2.6 μm…
Theoretical principles of near-field optical microscopies and spectroscopies
2000
International audience; This paper deals with the principles of detection of optical signals near a surface in a manner permitting the mapping of the distribution of the fields close to various kinds of illuminated samples. We begin with a discussion of the main physical properties of the optical fields near a surface in the absence of any probe tip. This mainly concerns phenomena involving evanescent waves for which the local decay lengths are governed not only by the sizes but also by the intrinsic properties of the surface structures. The interpretation of the detection process is reviewed on the basis of a discussion about the possibility of establishing direct comparisons between exper…
Shallow water rogue waves in nonlinear optical fibers
2013
The dynamics of extreme waves, often known as freak or rogue waves (RW), is presently a subject of intensive research. In oceanography, RW are mostly known as a sudden deep-water event which is responsible for ship wreakages and can be modeled by the 1D Nonlinear Schrodinger Equation (NLSE). In this framework, an ideal testbed is provided by optical pulse propagation in nonlinear optical fibers: extreme solitary wave emissions during supercontinuum generation or the first experimental observation of the Peregrine solitons have indeed been carried out exploiting the modulation instability occuring in fibers with anomalous dispersion.
Spatio-temporal beam dynamics in multimode nonlinear optical fibers
2017
We overview recent advances in the spatio-temporal nonlinear dynamics of optical pulses propagating in multimode optical fibers. The Kerr effect leads to spatial beam self-cleaning in a graded-index multimode optical fiber, followed by sideband series generation spanning multiple octaves. Effectively single mode supercontinuum spanning from the visible to the mid-infrared was also demonstrated. Enhancement of Kerr beam self-cleaning was observed in active fiber with quasi-step index profile. Moreover, mutual self-cleaning was recently reported for both the fundamental and the second harmonic beams in optically poled multimode fibers with cubic and quadratic nonlinearity.
Nonlinear spatial self-cleaning in multimode amplifying fiber and fiber laser cavity
2017
During the last years, multimode fibers (MMFs) were used as an experimental platform for the observation of complex nonlinear propagation phenomena, thanks to their additional spatiotemporal degrees of freedom with respect to single mode fibers. Multimode solitons [1], geometric parametric instability [2], self-induced beam cleaning (SBC) [3] and supercontinuum generation have been reported [4]. In all of these situations considered so far the MMFs were standard graded-index fibers: the intermodal interactions took place in a conservative system (propagation losses were negligible). In this work we have experimentally investigated the Kerr SBC in three dissipative systems: a MMF with signif…