Search results for "Solid-state"
showing 10 items of 530 documents
First-principles simulations for attosecond photoelectron spectroscopy based on time-dependent density functional theory
2018
We develop a first-principles simulation method for attosecond time-resolved photoelectron spectroscopy. This method enables us to directly simulate the whole experimental processes, including excitation, emission and detection on equal footing. To examine the performance of the method, we use it to compute the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) experiments of gas-phase Argon. The computed RABBITT photoionization delay is in very good agreement with recent experimental results from [Klünder et al., Phys. Rev. Lett. 106, 143002 (2011)] and [Guénot et al., Phys. Rev. A 85, 053424 (2012)]. This indicates the significance of a fully-consiste…
Infrared radiation harmonic generation in degenerate semiconductors
2004
The basic properties of infrared laser radiation odd harmonic generation due to electron-charged impurity collisions in degenerate semiconductors are investigated. It is found that in the case of relatively weak fields, the electron Fermi distribution is the cause of an anomalous suppression of harmonic radiation. In the case of strong fields, the effect of the selective suppression of single harmonics is established.
One-dimensional Ising-like systems: an analytical investigation of the static and dynamic properties, applied to spin-crossover relaxation
2000
We investigate the dynamical properties of the 1-D Ising-like Hamiltonian taking into account short and long range interactions, in order to predict the static and dynamic behavior of spin crossover systems. The stochastic treatment is carried out within the frame of the local equilibrium method [1]. The calculations yield, at thermodynamic equilibrium, the exact analytic expression previously obtained by the transfer matrix technique [2]. We mainly discuss the shape of the relaxation curves: (i) for large (positive) values of the short range interaction parameter, a saturation of the relaxation curves is observed, reminiscent of the behavior of the width of the static hysteresis loop [3]; …
A polymer chain trapped between two parallel repulsive walls: A Monte-Carlo test of scaling behavior
1998
An off-lattice bead-spring model of a polymer chain trapped between two parallel walls a distance D apart is studied by Monte-Carlo methods, using chain lengths N in the range $$32 \le N \le 512$$ and distances D from 4 to 32 (in units of the maximum spring extension). The scaling behavior of the coil linear dimensions parallel to the plates and of the force on the walls is studied and discussed with the help of current theoretical predictions. Also the density profiles of the monomers across the slit are obtained and it is shown that the predicted variation with the distance z from a wall, $$\rho (z) \propto {z^{1/\nu }}$$ , is obtained only when one introduces an extrapolation length λ in…
The influence of the dynamics of ionic multiplets onto electronic transport properties of heavy-fermion systems: a semi-phenomenological approach
2001
We present calculations of the electronic transport properties of heavy-fermion systems within a semi-phenomenological approach to the dynamical mean field theory. In this approach the dynamics of the Hund's rules 4f (5f )-ionic multiplet split in a crystalline environment is taken into account. Within the scope of this calculation we use the linear response theory to reproduce qualitative features of the temperature-dependent resistivity and hall conductivity, the magneto-resistivity and the thermoelectric power typical for heavy-fermion systems. The model calculations are directly compared with experimental results on CeCu2Si2.
Many-electron transport in Aharonov-Bohm interferometers: Time-dependent density-functional study
2012
We apply time-dependent density-functional theory to study many-electron transport in Aharonov-Bohm interferometers in a non-equilibrium situation. The conductance properties in the system are complex and depend on the enclosed magnetic flux in the interferometer, the number of interacting particles, and the mutual distance of the transport channels at the points of encounter. Generally, the electron-electron interactions do not suppress the visibility of Aharonov-Bohm oscillations if the interchannel distance -- determined by the positioning of the incompressible strips through the external magnetic field -- is optimized. However, the interactions also impose an interesting Aharonov-Bohm p…
Density Functional Theory of Multicomponent Quantum Dots
2004
Quantum dots with conduction electrons or holes originating from several bands are considered. We assume the particles are confined in a harmonic potential and assume the electrons (or holes) belonging to different bands to be different types of fermions with isotropic effective masses. The density functional method with the local density approximation is used. The increased number of internal (Kohn-Sham) states leads to a generalisation of Hund's first rule at high densities. At low densitites the formation of Wigner molecules is favored by the increased internal freedom.
Heavy fermion spin liquid in herbertsmithite
2015
We analyze recent heat capacity measurements in herbertsmithite $\rm ZnCu_3(OH)_6Cl_2$ single crystal samples subjected to strong magnetic fields. We show that the temperature dependence of specific heat $C_{mag}$ formed by quantum spin liquid at different magnetic fields $B$ resembles the electronic heat capacity $C_{el}$ of the HF metal $\rm YbRh_2Si_2$. We demonstrate that the spinon effective mass $M^*_{mag}\propto C_{mag}/T$ exhibits a scaling behavior like that of $C_{el}/T$. We also show that the recent measurements of $C_{mag}$ are compatible with those obtained on powder samples. These observations allow us to conclude that $\rm ZnCu_3(OH)_6Cl_2$ holds a stable strongly correlated …
Correlation gap in the heavy-fermion antiferromagnetUPd2Al3
2002
The optical properties of the heavy-fermion compound ${\mathrm{UPd}}_{2}{\mathrm{Al}}_{3}$ have been measured in a frequency range from 0.04 to 5 meV $(0.3--40{\mathrm{cm}}^{\ensuremath{-}1})$ at temperatures $2\mathrm{K}lTl300\mathrm{K}.$ Below the coherence temperature ${T}^{*}\ensuremath{\approx}50\mathrm{K},$ a hybridization gap opens around 10 meV. As the temperature decreases further $(Tl~20\mathrm{K}),$ a well-pronounced pseudogap of approximately 0.2 meV develops in the optical response; we relate this to the antiferromagnetic ordering which occurs below ${T}_{N}\ensuremath{\approx}14\mathrm{K}.$ The frequency-dependent mass and scattering rate give evidence that the enhancement of …
Nature of Heavy Quasiparticles in Magnetically Ordered Heavy FermionsUPd2Al3andUPt3
2002
The optical conductivity of the heavy fermions $\mathrm{UPd}{}_{2}{\mathrm{Al}}_{3}$ and $\mathrm{UPt}{}_{3}$ has been measured in the energy range from 0.04 to 5 meV. In both compounds a well pronounced pseudogap of less than 1 meV develops in the optical response at low temperatures; we relate this to the antiferromagnetic ordering. From the energy dependence of the effective mass and scattering rate we conclude that the enhancement of the mass mainly occurs below the energy which is related to magnetic correlations between the local magnetic moments and the itinerant electrons. This implies that the magnetic order in these compounds is the prerequisite to the formation of the heavy quasi…