Search results for "Solutions"

showing 10 items of 757 documents

Highlights on contemporary recognition and sensing of fluoride anion in solution and in the solid state

2012

The fluoride anion has recently gained well deserved attention among the scientific community for its importance in many fields of human activities, but also for concerns on its effect on health and the environment. Although surprisingly overlooked in systematic studies in the past, fluoride has nowadays become a topical target in the field of anion recognition. A multitude of scientific reports are published every year where the establishment of efficient and specific interaction with fluoride is sought in polar and aqueous media. Here, the emphasis is directed to a detailed description of the most interesting contemporary studies in the field, with a particular focus given to those publis…

AnionsAqueous mediumChemistryMultitudeSolid-stateMolecular ConformationWaterNanotechnologyHydrogen BondingGeneral ChemistryCrystallography X-RaySolutionschemistry.chemical_compoundFluoridesHumansEngineering ethicsFluorideta116Chemical Society Reviews
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Characterization of poly(4-vinylpyridine 1-oxide) by free-solution capillary electrophoresis and micellar electrokinetic chromatography

2008

The migration characteristics of poly(4-vinylpyridine 1-oxide) (PVP-NO) in phosphate buffers of acidic pH (20 mM H 3 PO 4 or NaH 2 PO 4 ) have been studied using both free-solution capillary electrophoresis (FSCE) and MEKC. To inhibit adsorption, 250 mM o-phosphoethanolamine (2-aminoethyl dihydrogen phosphate) was used. In FSCE, PVP-NO showed a narrow peak and a broader band, both having anionic behavior. These peak and band were attributed to the free and aggregated or micellized PVP-NO forms, respectively. According to surface tension measurements, the CMC of SDS in the BGE was 1.8 and 0.48 mM in the absence and in the presence of 1000 μpg/mL PVP-NO, respectively, and the association of t…

AnionsDetergentsClinical BiochemistryOxidemacromolecular substancesBuffersBiochemistryMicelleMicellar electrokinetic chromatographyAnalytical ChemistrySurface tensionchemistry.chemical_compoundCapillary electrophoresisAdsorptionSurface TensionMicellesLaunderingchemistry.chemical_classificationChromatographyChromatographytechnology industry and agricultureElectrophoresis CapillaryWaterPolymerPhosphateOrganophosphatesSolutionschemistryPolyvinylpyridine N-OxideELECTROPHORESIS
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A highly enantioselective abiotic receptor for malate dianion in aqueous solution

2006

The highly enantioselective molecular recognition of the malate dianion by a synthetic receptor in aqueous solution has been studied by potentiometric titrations, mass spectrometry (ESI-MS), diffusion measurements (PGSE NMR) and molecular modeling. Garcia-España Monsonis, Enrique, Enrique.Garcia-Es@uv.es

AnionsModels MolecularMalate dianionSpectrometry Mass Electrospray IonizationMagnetic Resonance SpectroscopyMolecular modelUNESCO::QUÍMICADiffusionPotentiometric titrationMalatesMolecular modelingAbiotic receptorMass spectrometry:QUÍMICA [UNESCO]CatalysisSubstrate SpecificityMolecular recognitionComputational chemistryMaterials ChemistryOrganic chemistryAqueous solutionReceptorAbiotic componentEnantioselectiveAqueous solutionMolecular StructureChemistrySpectrometryMeasurementsMetals and AlloysEnantioselective synthesisWaterHydrogen BondingStereoisomerismGeneral ChemistryGeneral MedicineUNESCO::QUÍMICA::Química macromolecularCombinatorial chemistrySurfaces Coatings and FilmsElectronic Optical and Magnetic MaterialsSolutionsCeramics and CompositesPotentiometryEnantioselective ; Abiotic receptor ; Malate dianion ; Aqueous solution ; Spectrometry ; Measurements ; Molecular modeling:QUÍMICA::Química macromolecular [UNESCO]
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Antioxidant Activity of All-trans-retinol in Homogeneous Solution and in Phosphatidylcholine Liposomes

1993

A kinetic quantification of the lipoperoxyl radical-scavenging activity of all-trans-retinol has been carried out in homogeneous solution, when radicals were produced from the oxidation of methyl linoleate in methanol, initiated by the lipid-soluble 2,2′-azobis (2,4-dimethyl-valeronitrile) (AMVN) as well as in a soybean phosphatidylcholine membrane model, in which peroxidation was induced either by AMVN or the hydrophylic 2,2′-azobis(2-amidinopropane)hydrochloride (AAPH). The physical microenvironment contributes to the determination of antioxidant efficiency of all-trans-retinol. In homogeneous solution the kinetic constant kinh is 3.5 × 105 M-1 s-1 and appears of the same order of magnitu…

AntioxidantFree Radicalsmedicine.medical_treatmentRadicalLipid BilayersAmidinesBiophysicsSynthetic membranealpha tocopherolTritiumBiochemistryphosphatidylcholine: retinolchemistry.chemical_compoundPhosphatidylcholineNitrilesmedicineOrganic chemistryAll trans retinolVitamin ALipid bilayerMolecular BiologyChromatography High Pressure LiquidLiposomeBilayerFree Radical ScavengersOxidantsSolutionsKineticschemistryliposomeLiposomesPhosphatidylcholinesBiophysicsLipid PeroxidationAzo CompoundsArchives of Biochemistry and Biophysics
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Betacyanins as phenol antioxidants. Chemistry and mechanistic aspects of the lipoperoxyl radical-scavenging activity in solution and liposomes.

2009

Reaction kinetics of betanin and its aglycone betanidin towards peroxyl radicals generated from the azo-initiated oxidation of methyl linoleate in methanol, and of a heterogeneous aqueous/soybean phosphatidylcholine liposomal system, were studied by monitoring formation of linoleic acid hydroperoxides and consumption of the pigments. Betanin was a weak retarder in methanol, and an effective chain breaking antioxidant in the liposomal model, indicating that kinetic solvent effects and partition in lipid bilayers may affect its activity. Betanidin behaved as a chain terminating antioxidant in both models. Kinetic parameters characterizing peroxyl radical-scavenging activity showed that betani…

Antioxidantmedicine.medical_treatmentLipid Bilayersalpha-TocopherolBiochemistryChemical kineticsLinoleic Acidchemistry.chemical_compoundStructure-Activity RelationshipReaction rate constantSettore BIO/10 - BiochimicamedicineBetacyaninsOrganic chemistryChromatography High Pressure LiquidBetaninAqueous solutionMolecular StructureMethanolWaterDrug SynergismGeneral MedicineFree Radical ScavengersSolutionsAglyconechemistryLinoleic Acidsbetacyanins betanin betanidin lipid peroxides liposomes antioxidant phytochemicalsSpectrophotometryLiposomesPhosphatidylcholinesSolventsMethanolBetacyaninsLipid PeroxidationOxidation-ReductionFree radical research
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On the existence and multiplicity of solutions for Dirichlet's problem for fractional differential equations

2016

In this paper, by using variational methods and critical point theorems, we prove the existence and multiplicity of solutions for boundary value problem for fractional order differential equations where Riemann-Liouville fractional derivatives and Caputo fractional derivatives are used. Our results extend the second order boundary value problem to the non integer case. Moreover, some conditions to determinate nonnegative solutions are presented and examples are given to illustrate our results.

Applied Mathematics010102 general mathematicsMathematical analysisMultiplicity (mathematics)01 natural sciencesDirichlet distribution010101 applied mathematicssymbols.namesakeSettore MAT/05 - Analisi MatematicasymbolsApplied mathematics0101 mathematicsFractional differentialAnalysisfractional differential equations critical points theorem variational methods multiple solutionsMathematics
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Singular solutions to a quasilinear ODE

2005

In this paper, we prove the existence of infinitely many radial solutions having a singular behaviour at the origin for a superlinear problem of the form $-\Delta_pu=|u|^{\delta-1}u$ in $B(0,1)\setminus\{0\}\subset\mathbb R^N$,\, $u=0$ for $|x|=1$, where $N>p>1$ and $\delta>p-1$. Solutions are characterized by their nodal properties. The case $\delta+1 <\frac{Np}{N-p}$ is treated. The study of the singularity is based on some energy considerations and takes into account the classification of the behaviour of the possible solutions available in the literature. By following a shooting approach, we are able to deduce the main multiplicity result from some estimates on the rotation numbers asso…

Applied Mathematics34B1634B15Singular solutions superlinear problem multiplicity result p-Laplacian equation rotation number radial solutionsAnalysis35J60
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Thin obstacle problem : Estimates of the distance to the exact solution

2018

We consider elliptic variational inequalities generated by obstacle type problems with thin obstacles. For this class of problems, we deduce estimates of the distance (measured in terms of the natural energy norm) between the exact solution and any function that satisfies the boundary condition and is admissible with respect to the obstacle condition (i.e., they are valid for any approximation regardless of the method by which it was found). Computation of the estimates does not require knowledge of the exact solution and uses only the problem data and an approximation. The estimates provide guaranteed upper bounds of the error (error majorants) and vanish if and only if the approximation c…

Applied MathematicsComputation010102 general mathematicsMathematical analysista111estimates of the distance to the exact solutionthin obstaclevariaatiolaskentaFunction (mathematics)variationals problems01 natural sciences010101 applied mathematicsExact solutions in general relativityObstacleNorm (mathematics)free boundary problemsVariational inequalityObstacle problemBoundary value problem0101 mathematicsMathematicsInterfaces and Free Boundaries
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Nonlinear nonhomogeneous Neumann eigenvalue problems

2015

We consider a nonlinear parametric Neumann problem driven by a nonhomogeneous differential operator with a reaction which is $(p-1)$-superlinear near $\pm\infty$ and exhibits concave terms near zero. We show that for all small values of the parameter, the problem has at least five solutions, four of constant sign and the fifth nodal. We also show the existence of extremal constant sign solutions.

Applied MathematicsConcave termnodal solutionMathematical analysisZero (complex analysis)superlinear reactionDifferential operatorExtremal constant sign solutionNonlinear systemMaximum principlemaximum principleNeumann boundary conditionextremal constant sign solutionsQA1-939superlinear reaction concave terms maximum principle extremal constant sign solutions nodal solution critical groupsconcave termsConstant (mathematics)critical groupsEigenvalues and eigenvectorsCritical groupMathematicsMathematicsSign (mathematics)Electronic Journal of Qualitative Theory of Differential Equations
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A geometrical criterion for nonexistence of constant-sign solutions for some third-order two-point boundary value problems

2020

We give a simple geometrical criterion for the nonexistence of constant-sign solutions for a certain type of third-order two-point boundary value problem in terms of the behavior of nonlinearity in the equation. We also provide examples to illustrate the applicability of our results.

Applied MathematicsMathematical analysislcsh:QA299.6-433lcsh:AnalysisType (model theory)nonexistence of solutionsthird-order two-point boundary value problemsNonlinear systemThird orderSimple (abstract algebra)comparison methods for the first zero functionsBoundary value problemConstant (mathematics)Value (mathematics)AnalysisMathematicsSign (mathematics)Nonlinear Analysis
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