Search results for "Spectroscopy"

showing 10 items of 10293 documents

Nitric Oxide-Releasing Drug Glyceryl Trinitrate Targets JAK2/STAT3 Signaling, Migration and Invasion of Triple-Negative Breast Cancer Cells

2021

Triple-negative breast cancer (TNBC) is a highly aggressive disease with invasive and metastasizing properties associated with a poor prognosis. The STAT3 signaling pathway has shown a pivotal role in cancer cell migration, invasion, metastasis and drug resistance of TNBC cells. IL-6 is a main upstream activator of the JAK2/STAT3 pathway. In the present study we examined the impact of the NO-donor glyceryl trinitrate (GTN) on the activation of the JAK2/STAT3 signaling pathway and subsequent migration, invasion and metastasis ability of TNBC cells through in vitro and in vivo experiments. We used a subtoxic dose of carboplatin and/or recombinant IL-6 to activate the JAK2/STAT3 signaling path…

STAT3 Transcription FactorQH301-705.5Triple Negative Breast NeoplasmsmigrationArticleCatalysisStat3 Signaling PathwayMetastasisInorganic ChemistryMiceNitroglycerinchemistry.chemical_compoundCell Movementnitric oxideIn vivoCell Line TumormedicineAnimalsHumanscancermetastasisNeoplasm InvasivenessNitric Oxide DonorsBiology (General)Physical and Theoretical ChemistrySTAT3QD1-999Molecular BiologySpectroscopyTriple-negative breast cancerMice Inbred BALB CbiologyActivator (genetics)Organic ChemistryCancerGeneral MedicineJanus Kinase 2invasionmedicine.diseaseCarboplatinComputer Science ApplicationsChemistrychemistrybiology.proteinCancer researchFemalesignalingSignal TransductionInternational Journal of Molecular Sciences
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Computational determination of the dominant triplet population mechanism in photoexcited benzophenone

2014

In benzophenone, intersystem crossing occurs efficiently between the S-1(n pi(star)) state and the T-1 state of dominant n pi(star) character, leading to excited triplet states after photoexcitation. The transition mechanism between S-1(n pi(star)) and T-1 is still a matter of debate, despite several experimental studies. Quantum mechanical calculations have been performed in order to assess the relative efficiencies of previously proposed mechanisms, in particular, the direct S-1 -> T-1 and indirect S-1 -> T-2(pi pi(star)) -> T-1 ones. Multiconfigurational wave function based methods are used to discuss the nature of the relevant states and also to determine minimum energy paths a…

STATE DIPOLE-MOMENTSPopulationMechanistic organic photochemistryEXCITED BENZOPHENONEGeneral Physics and AstronomyGAS-PHASEABSORPTION-SPECTROSCOPYchemistry.chemical_compoundORGANIC-PHOTOCHEMISTRYMOLECULAR WAVE-FUNCTIONSBenzophenonePhysical and Theoretical ChemistryeducationWave functioneducation.field_of_studyROW ATOMSChemistryCONICAL INTERSECTIONSPhotoexcitation[CHIM.THEO]Chemical Sciences/Theoretical and/or physical chemistryIntersystem crossingExcited state2ND-ORDER PERTURBATION-THEORYANO BASIS-SETSAtomic physicsPhosphorescence
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Gamma-ray spectroscopy of191,193Bi

2001

Very neutron-deficient Bi-191,Bi-193 nuclei have been studied at the Department of Physics, University of Jyvaskyla, Finland (JYFL) employing the Jurosphere II Ge-detector array coupled to the gas-filled recoil separator RITU and different tagging techniques. For the first time in heavy odd-mass nuclei, a collective band (oblate) is identified above the 2p-1h (1/2(+)) proton intruder state in Bi-191. In both Bi-191,Bi-193, a band based on isomeric 13/2(+) state has been observed and oblate deformation for this state has been deduced. ispartof: Acta Physica Polonica B vol:32 issue:3 pages:1019-1023 ispartof: location:POLAND, ZAKOPANE status: published

STATESNUCLEITLBIspektroskopiaALPHA-DECAYISOTOPESSpectroscopy
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Optical absorption of torus-shaped metal nanoparticles in the visible range

2007

Received 22 November 2007; published 19 December 2007We theoretically and experimentally investigated the optical response of a thin metal nanotorus in the visiblerange. The close formulas describing the extinction cross sections of a torus are obtained in the nonretardedapproximation. We demonstrate a good agreement between numerical simulations and experimental data. Ourfindings show that the main resonance is highly sensitive to the external medium and the geometrical param-eters of the particle.DOI: 10.1103/PhysRevB.76.245422 PACS number s : 78.67.Bf, 73.20.Mf, 78.20.Ci

SURFACE PLASMONMaterials science02 engineering and technology01 natural sciencesMolecular physicsResonance (particle physics)Optics[ PHYS.COND.CM-MSQHE ] Physics [physics]/Condensed Matter [cond-mat]/Mesoscopic Systems and Quantum Hall Effect [cond-mat.mes-hall]0103 physical sciences[SPI.NANO]Engineering Sciences [physics]/Micro and nanotechnologies/Microelectronics010306 general physicsAbsorption (electromagnetic radiation)Spectroscopy[PHYS.COND.CM-MSQHE]Physics [physics]/Condensed Matter [cond-mat]/Mesoscopic Systems and Quantum Hall Effect [cond-mat.mes-hall]TORUS[PHYS.PHYS.PHYS-OPTICS]Physics [physics]/Physics [physics]/Optics [physics.optics]SPECTROSCOPY[ PHYS.PHYS.PHYS-OPTICS ] Physics [physics]/Physics [physics]/Optics [physics.optics]Extinction crossbusiness.industrySurface plasmonTorus021001 nanoscience & nanotechnologyCondensed Matter PhysicsElectronic Optical and Magnetic MaterialsQuasiparticleVisible range[ SPI.NANO ] Engineering Sciences [physics]/Micro and nanotechnologies/Microelectronics0210 nano-technologybusiness
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Scanning tunneling microscopy and spectroscopy of Mo clusters grown on TiO2(110).

2007

Molybdenum was deposited in two steps (3 eq. ML and 1 eq. ML) on the light blue rutile TiO2 10) (1 x 1) surface at room temperature, each Mo deposition cycle being followed by an annealing up to 950-1000 K. This procedure was found to lead to formation of separated clusters having a size in very wide range (1-20 nm). Scanning tunneling microscopy showed a dependence of the cluster morphology as a function of the size. The scanning tunneling spectra of Mo clusters was studied as a function of cluster dimensions and discussed in comparison with photoelectron spectroscopy results previously obtained for homogeneous Mo films. The dI/d V curves do not display the valence band structure of deposi…

SURFACEAnnealing (metallurgy)Schottky barrierScanning tunneling spectroscopyAnalytical chemistrychemistry.chemical_element02 engineering and technologyGrowth01 natural scienceslaw.inventionX-ray photoelectron spectroscopylaw0103 physical sciencesmorphologyMaterials ChemistryCluster (physics)GOLD010306 general physicsSpectroscopyroughnessMolybdenumNANOPOROUS TIO2 FILMSTitanium oxideScanning tunnelling spectroscopiesSurface structureSurfaces and Interfaces021001 nanoscience & nanotechnologyCondensed Matter PhysicsSurfaces Coatings and FilmsCrystallographyScanning tunnelling microscopyand topographychemistryMolybdenumScanning tunneling microscope0210 nano-technology
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Evidence for the Existence of an Effective Interfacial Tension between Miscible Fluids: Isobutyric Acid-Water and 1-Butanol-Water in a Spinning-Drop …

2006

We report definitive evidence for an effective interfacial tension between two types of miscible fluids using spinning-drop tensiometry (SDT). Isobutyric acid (IBA) and water have an upper critical solution temperature (UCST) of 26.3 degrees C. We created a drop of the IBA-rich phase in the water-rich phase below the UCST and then increased the temperature above it. Long after the fluids have reached thermal equilibrium, the drop persists. By plotting the inverse of the drop radius cubed (r(-)(3)) vs the rotation rate squared (omega(2)), we confirmed that an interfacial tension exists and estimated its value. The transition between the miscible fluids remained sharp instead of becoming more…

SURFACE-TENSIONThermodynamicsGRADIENTSInstabilityIsobutyric acidSurface tensionchemistry.chemical_compoundNONEQUILIBRIUM FLUCTUATIONS1-ButanolIsobutyratesGRAVITYUpper critical solution temperatureElectrochemistrySurface TensionGeneral Materials ScienceSpectroscopyThermal equilibriumAqueous solutionDrop (liquid)ButanolDIFFUSION-COEFFICIENTWaterSurfaces and InterfacesCondensed Matter PhysicsKORTEWEG STRESSESLIGHT-SCATTERINGCAPILLARY TUBESButyrateschemistrySolubilityLIQUID-MIXTURESSYSTEM
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Analysis of metallic impurity content by means of VUV and SXR diagnostics in hybrid discharges with hot-spots on the JET-ITER-like wall poloidal limi…

2019

In preparation for the upcoming JET D-T campaign, great effort has been devoted during the 2015-2016 JET campaigns with the ITER-like wall (ILW) to the extension of the high performance H-mode phase in baseline and hybrid scenarios. Hybrid discharges were the only ones that have been stopped by the real-time vessel protection system due hot-spot formation on the outboard poloidal limiter. Generation of hot-spots was linked to the application of high neutral beams injection and ion cyclotron resonance heating (ICRH) power. In tokamaks with high-Z plasma components, the use of ICRH heating is also accompanied by an increased metallic impurity content. Simultaneous control of hot-spot temperat…

SXRhot-spot; plasma impurity; plasma physics; SXR; tokamaks; tungsten; VUV spectroscopyplasma impurityMaterials scienceTokamaktungsten01 natural sciences010305 fluids & plasmasIonlaw.inventionImpuritylaw0103 physical sciencesplasma physicLimiter010306 general physicstokamakJet (fluid)plasma physicsMagnetic confinement fusionPlasmahot-spotCondensed Matter PhysicsNuclear Energy and EngineeringElectric currentAtomic physicstokamaksVUV spectroscopy
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On-line in-tube solid phase microextraction coupled to capillary liquid chromatography-diode array detection for the analysis of caffeine and its met…

2019

Abstract In-tube solid phase microextraction (IT-SPME) coupled on-line to capillary liquid chromatography with diode array detection provides a simple and fast analytical methodology for the simultaneous quantitation of caffeine and its three primary metabolites (theobromine, paraxanthine and theophylline) in micro samples of serum, saliva and urine matrices. The sample amount required for one analysis was only 2.5 μL of saliva, 6.25 μL of serum or 40 μL of urine, a requirement for its implementation in a hospital laboratory for preterm newborns, where sample availability is a major problem. In standard conditions, 25 μL of diluted saliva or serum (or 100 μL of urine) were processed by IT-S…

SalivaAnalyteClinical BiochemistryPharmaceutical ScienceUrineUrineSolid-phase microextraction01 natural sciencesAnalytical Chemistrychemistry.chemical_compoundTheophyllineCaffeineDrug DiscoverymedicineHumansSalivaTheobromineSolid Phase MicroextractionSpectroscopyParaxanthineDetection limitChromatography010405 organic chemistryElution010401 analytical chemistry0104 chemical scienceschemistryCalibrationTheobromineBiological samples Capillary liquid chromatography In-tube solid-phase microextraction TrimethylxanthinesChromatography Liquidmedicine.drug
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Infrared based saliva screening test for COVID‐19

2021

Severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) has resulted in an unprecedented need for diagnostic testing that is critical in controlling the spread of COVID-19. We propose a portable infrared spectrometer with purpose-built transflection accessory for rapid point-of-care detection of COVID-19 markers in saliva. Initially, purified virion particles were characterized with Raman spectroscopy, synchrotron infrared (IR) and AFM-IR. A data set comprising 171 transflection infrared spectra from 29 subjects testing positive for SARS-CoV-2 by RT-qPCR and 28 testing negative, was modeled using Monte Carlo Double Cross Validation with 50 randomized test and model sets. The testing se…

SalivaMaterials scienceCoronavirus disease 2019 (COVID-19)Spectrophotometry InfraredInfraredPoint-of-care testingInfrared spectroscopy010402 general chemistry01 natural sciencesProof of Concept StudySensitivity and SpecificityCatalysisSpecimen HandlingCohort Studies03 medical and health sciences0302 clinical medicineCOVID-19 TestingSpectrophotometryChlorocebus aethiopsmedicineCOVID-19 diagnostic infrared spectroscopy Raman spectroscopy saliva SARS-CoV-2 virionsAnimalsHumansQDLeast-Squares AnalysisSalivaVero CellsMass screening030304 developmental biologyDetection limit0303 health sciencessalivaChromatographymedicine.diagnostic_test010405 organic chemistrySARS-CoV-2COVID-19Discriminant AnalysisGeneral Chemistry030206 dentistryGeneral Medicine0104 chemical sciences3. Good healthPoint-of-Care TestingMonte Carlo MethodATR-FTIRResearch ArticleAngewandte Chemie (International Ed. in English)
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Mechanism of genotoxicity and electron density distribution by NMR of 5-nitro-3-thiophenecarboxamides, a novel group of direct-acting mutagens in Sal…

1993

Abstract The mutagenic activity of 23 5-nitro-3-thiophenecarboxanilides and of 5-nitro-3-thiophenecarboxamide, the prototype, (NTCAs) have been evaluated in the Ames test on Salmonella typhimurium strains TA100 ad TA98 with and without metabolic activation. Effects of different substituents (electron-donating and electron-withdrawing) were studied to evaluate structural features that affect the metabolism and the bacterial mutagenic potency. All the derivatives were direct-acting mutagens, the mutagenic potency ranging from 0.7 to 142 revertants (rev.)/nmol in TA100 and from 0.09 to 68 rev./nmol in TA98 strain. Results obtained with strains TA98NR and TA98/1,8-DNP 6 indicated that the mutag…

Salmonella typhimuriumendocrine systemMagnetic Resonance SpectroscopyFree RadicalsStereochemistryMutagenThiophenesToxicologymedicine.disease_causeAmes testNitroreductasechemistry.chemical_compoundStructure-Activity RelationshipAcetyltransferasesNitrationmedicinechemistry.chemical_classificationChemistrySuperoxideMutagenicity Testsfungifood and beveragesGeneral MedicineNitroreductasesEnzymeNitroGenotoxicityMutagensChemico-biological interactions
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