Search results for "Thorium"
showing 10 items of 37 documents
Preparation of targets for the gas-filled recoil separator TASCA by electrochemical deposition and design of the TASCA target wheel assembly
2008
Abstract The Transactinide Separator and Chemistry Apparatus (TASCA) is a recoil separator with maximized transmission designed for performing advanced chemical studies as well as nuclear reaction and structure investigations of the transactinide elements ( Z >103) on a one-atom-at-a-time basis. TASCA will provide a very clean transactinide fraction with negligible contamination of lighter elements from nuclear side reactions in the target. For TASCA a new target chamber was designed and built at GSI including the rotating target wheel assembly ARTESIA for beam intensities up to 2 μA (particle). For the production of longer-lived isotopes of neutron-rich heavier actinide and transactinide e…
Distillation and stripping pilot plants for the JUNO neutrino detector: Design, operations and reliability
2019
Abstract This paper describes the design, construction principles and operations of the distillation and stripping pilot plants tested at the Daya Bay Neutrino Laboratory, with the perspective to adapt these processes, system cleanliness and leak-tightness standards to the final full scale plants to be used for the purification of the liquid scintillator of the JUNO neutrino detector. The main goal of these plants is to remove radio impurities from the liquid scintillator while increasing its optical attenuation length. Purification of liquid scintillator will be performed with a system combining alumina oxide, distillation, water extraction and steam (or N 2 gas) stripping. Such a combined…
The Design and Sensitivity of JUNO's scintillator radiopurity pre-detector OSIRIS
2021
The European physical journal / C 81(11), 973 (2021). doi:10.1140/epjc/s10052-021-09544-4
Gamma activity and geochemical features of building materials: estimation of gamma dose rate and indoor radon levels in Sicily.
2001
A high-purity germanium detector has been used to measure the abundance of radium (Ra), thorium (Th) and potassium (K) in building materials used in Sicilian dwellings. The measurements were performed to evaluate which material was suitable for the construction of an enclosure, which would have a low background emission. The materials examined in this work showed concentrations of 226Ra, 232Th and 40K dramatically variable depending on the lithologies, particularly in the case of blocks, sands and aggregates commonly used in building materials in Sicily. The results are discussed and a criterion is indicated to reduce the radiation dose to humans. Since radon inlet is a major health problem…
Development of two-color resonance ionization scheme for Th using an automated wide-range tunable Ti:sapphire laser system
2018
Two-color resonance ionization schemes of Th were investigated by an automated wide-range tunable, grating-assisted Ti:Sa laser system with intracavity SHG option. A two-color ionization scheme via autoionizing state (1st step: 372.049 nm and 2nd step: 401.031 nm) was developed and its relative efficiency was lower by factor of three compared to a known three color scheme. peerReviewed
Identification of Thorium-236
1973
Abstract The new nuclide 236Th has been produced via the (γ, 2 p) reaction by irradiation of 238U with 140 MeV bremsstrahlung. After chemical separation of thorium, the half-life was determined to be 36 ± 3 min -from the growth-decay curve of the strongest γ-ray transition of the daughter nuclide, 9 min 236Pa.
Assignment of complex species by affinity capillary electrophoresis: The case of Th(IV)‐desferrioxamine B
2020
International audience; The electrophoretic mobility change of desferrioxamine B (DFO) was monitored by UV absorption spectrophotometry upon increasing the thorium(IV) concentration in the background electrolyte at two acidities ([HClO4]Tot = 0.0316 and 0.0100 M). These data enabled to assess the speciation model and to determine the equilibrium constant of [Th(DFO)H2]3+ at fixed ionic strength (I = 0.1 M (H,Na)ClO4). Affinity capillary electrophoresis (ACE) turned out to be most helpful in identifying the complexed species by ascertaining its charge and protonation state. The assignment of the correct stoichiometry relied on the reliable estimation of the electrophoretic mobility by assumi…
The role of nano-perovskite in the negligible thorium release in seawater from Greek bauxite residue (red mud)
2016
AbstractWe present new data about the chemical and structural characteristics of bauxite residue (BR) from Greek Al industry, using a combination of microscopic, analytical, and spectroscopic techniques. SEM-EDS indicated a homogeneous dominant “Al-Fe-Ca-Ti-Si-Na-Cr matrix”, appearing at the microscale. The bulk chemical analyses showed considerable levels of Th (111 μg g−1), along with minor U (15 μg g−1), which are responsible for radioactivity (355 and 133 Bq kg−1 for 232Th and 238U, respectively) with a total dose rate of 295 nGy h−1. Leaching experiments, in conjunction with SF-ICP-MS, using Mediterranean seawater from Greece, indicated significant release of V, depending on S/L ratio,…
Thorium partitioning in Greek industrial bauxite investigated by synchrotron radiation and laser-ablation techniques
2011
Abstract Typical red–brown (Fe-rich) and high-quality white–grey (Fe-depleted) bauxite samples from active mines of the Parnassos-Ghiona area, central Greece, were investigated. According to XRF and ICP-MS analyses their actinide content, and particularly of Th, is relatively increased. Fe-depleted samples contain up to 62.75 ppm Th corresponding to 220 Bq/kg due to 228Ac (232Th-series), whereas Fe-rich samples are less Th-radioactive (up to 58.25 ppm Th, 180 Bq/kg due to 228Ac). Powder-XRD patterns showed that Th-enriched (Fe-depleted) bauxite consists mostly of diaspore (AlOOH polymorph), anatase and rutile (TiO2 polymorphs). SEM-EDS indicated the presence of Ti–Fe–containing phases (e.g.…
Characterization of 233U alpha recoil sources for 229()Th beam production
2019
Radioactive $^{233}$U alpha recoil sources are being considered for the production of a thorium ion source to study the low-energy isomer in $^{229}$Th with high-resolution collinear laser spectroscopy at the IGISOL facility of the University of Jyv\"askyl\"a. In this work two different $^{233}$U sources have been characterized via alpha and gamma spectroscopy of the decay radiation obtained directly from the sources and from alpha-recoils embedded in implantation foils. These measurements revealed rather low $^{229}$Th recoil efficiencies of only a few percent. Although the low efficiency of one of the two sources can be attributed to its inherent thickness, the low recoil efficiency of th…