Search results for "Ultrashort pulse"
showing 10 items of 153 documents
Parallel laser micromachining based on diffractive optical elements with dispersion compensated femtosecond pulses
2013
We experimentally demonstrate multi-beam high spatial resolution laser micromachining with femtosecond pulses. The effects of chromatic aberrations as well as pulse stretching on the material processed due to diffraction were significantly mitigated by using a suited dispersion compensated module (DCM). This permits to increase the area of processing in a factor 3 in comparison with a conventional setup. Specifically, 52 blind holes have been drilled simultaneously onto a stainless steel sample with a 30 fs laser pulse in a parallel processing configuration.
New photonic devices for ultrafast pulse processing operating on the basis of the diffraction-dispersion analogy
2008
The space-time analogy is a well-known topic within wave optics that brings together some results from beam diffraction and pulse dispersion. On the above basis, and taking as starting point some classical concepts in Optics, several photonic devices have been proposed during the last few years with application in rapidly evolving fields such as ultrafast (femtosecond) optics or RF and microwave signal processing. In this contribution, we briefly review the above ideas with particular emphasis in the generation of trains of ultrafast pulses from periodic modulation of the phase of a CW laser source. This is the temporal analogue of Fresnel diffraction by a pure phase grating. Finally, we ex…
A wideband THz Time Domain Spectroscopy table-top system based on ultrafast pulsed laser: Model and experiments
2014
We present an analytical model carefully describing the time-frequency behavior of all the stages composing our whole Terahertz Time Domain Spectroscopy laser based system, from the THz pulses generation via Optical Rectification, to their detection through Electro-Optic Sampling technique, by way of diffraction, collecting and focusing effects. In order to prove the effectiveness of our work, we report on the comparison among the experimental waveforms and the simulation results.
Spatiotemporal reaction kinetics of an ultrafast photoreaction pathway visualized by time-resolved liquid x-ray diffraction.
2006
We have studied the reaction dynamics for HgI 2 in methanol by using time-resolved x-ray diffraction (TRXD). Although numerous time-resolved spectroscopic studies have provided ample information about the early dynamics of HgI 2 , a comprehensive reaction mechanism in the solution phase spanning from picoseconds up to microseconds has been lacking. Here we show that TRXD can provide this information directly and quantitatively. Picosecond optical pulses triggered the dissociation of HgI 2 , and 100-ps-long x-ray pulses from a synchrotron probed the evolving structures over a wide temporal range. To theoretically explain the diffracted intensities, the structural signal from the solute, the…
Intramolecular charge transfer and dual fluorescence of 4-(dimethylamino)benzonitrile: ultrafast branching followed by a two-fold decay mechanism.
2011
International audience; In this contribution we present new experimental and theoretical results for the intramolecular charge transfer (ICT) reaction underlying the dual fluorescence of 4-(dimethylamino) benzonitrile ( DMABN), which indicate that the fully twisted ICT (TICT) state is responsible for the time-resolved transient absorption spectrum while a distinct partially twisted ICT (pTICT) structure is suggested for the fluorescent ICT state.
Visualizing coherent molecular rotation in a gaseous medium
2021
Inducing and controlling the ultrafast molecular rotational dynamics using shaped laser fields is essential in numerous applications. Several approaches exist that allow following the coherent molecular motion in real-time, including Coulomb explosion-based techniques and recovering molecular orientation from the angular distribution of high harmonics. We theoretically consider a non-intrusive optical scheme for visualizing the rotational dynamics in an anisotropic molecular gas. The proposed method allows determining the instantaneous orientation of the principal optical axes of the gas. The method is based on probing the sample using ultra-short circularly polarized laser pulses and recor…
Optical Imaging of Coherent Molecular Rotors
2020
International audience; Short laser pulses are widely used for controlling molecular rotational degrees of freedom and inducing molecular alignment, orientation, unidirectional rotation and other types of coherent rotational motion. To follow the ultra-fast rotational dynamics in real time, several techniques for producing molecular movies have been proposed based on the Coulomb explosion of rotating molecules, or recovering molecular orientation from the angular distribution of high-harmonics. The present work offers and demonstrates a novel non-destructive optical method for direct visualization and recording of movies of coherent rotational dynamics in a molecular gas. The technique is b…
All-fibered high-quality 1.5–2 THz femtosecond pulse sources
2009
Generation of high-quality ultra-high repetition rate optical pulse trains around 1.55µm has become increasingly interesting for many scientific applications such as optical sampling, ultra-high capacity transmission systems, component testing or nonlinear phenomena studies. Unfortunately, the current bandwidth limitations of optoelectronic devices do not enable the direct generation of pulses with repetition rate higher than 80GHz and a temporal width below a few ps.
Fiber-based device for the detection of low-intensity fluctuations of ultrashort pulses
2012
International audience; We describe a fiber-based device that can significantly enhance the low intensity fluctuations of an ultrashort pulse train to detect them more easily than with usual direct detection systems. Taking advantage of the Raman intrapulse effect that progressively shifts the central frequency of a femtosecond pulse propagating in an anomalous dispersion fiber, a subsequent spectral filtering can efficiently increase the level of fluctuations by more than one order of magnitude. We show that attention has to be paid to maintain the shape of the statistical distribution unaffected by the nonlinear process.
Pulse trains produced by phase-modulation of ultrashort optical pulses: tailoring and characterization
2009
1094-4087; In this paper, creation of pulse doublets and pulse trains by spectral phase modulation of ultrashort optical pulses is investigated. Pulse doublets with specific features are generated through step-like and triangular spectral phase modulation, whereas sequences of pulses with controllable delay and amplitude are produced via sinusoidal phase modulations. A temporal analysis of this type of tailored pulses is exposed and a complete characterization with the SPIDER technique (Spectral Phase Interferometry for Direct Electric-field Reconstruction) is presented. (C) 2004 Optical Society of America.