Search results for "diamond."
showing 10 items of 232 documents
Optical polarization of nuclear ensembles in diamond
2012
We report polarization of a dense nuclear-spin ensemble in diamond and its dependence on magnetic field and temperature. The polarization method is based on the transfer of electron spin polarization of negatively charged nitrogen vacancy color centers to the nuclear spins via the excited-state level anti-crossing of the center. We polarize 90% of the 14N nuclear spins within the NV centers, and 70% of the proximal 13C nuclear spins with hyperfine interaction strength of 13-14 MHz. Magnetic-field dependence of the polarization reveals sharp decrease in polarization at specific field values corresponding to cross-relaxation with substitutional nitrogen centers, while temperature dependence o…
Fabrication of $^{15}\textrm{NV}^{-}$ centers in diamond using a deterministic single ion implanter
2021
Nitrogen Vacancy (NV) centers in diamond are a platform for several important quantum technologies, including sensing, communication and elementary quantum processors. In this letter we demonstrate the creation of NV centers by implantation using a deterministic single ion source. For this we sympathetically laser-cool single $^{15}\textrm{N}_2^+$ molecular ions in a Paul trap and extract them at an energy of 5.9\,keV. Subsequently the ions are focused with a lateral resolution of 121(35)\,nm and are implanted into a diamond substrate without any spatial filtering by apertures or masks. After high-temperature annealing, we detect the NV centers in a confocal microscope and determine a conve…
Hyperfine level structure in nitrogen-vacancy centers near the ground-state level anticrossing
2019
Energy levels of nitrogen-vacancy centers in diamond were investigated using optically detected magnetic-resonance spectroscopy near the electronic ground-state level anticrossing (GSLAC) at an axial magnetic field around 102.4~mT in diamond samples with a nitrogen concentration of 1~ppm and 200~ppm. By applying radiowaves in the frequency ranges from 0 to 40 MHz and from 5.6 to 5.9 GHz, we observed transitions that involve energy levels mixed by the hyperfine interaction. We developed a theoretical model that describes the level mixing, transition energies, and transition strengths between the ground-state sublevels, including the coupling to the nuclear spin of the NV center\textquotesing…
Prospects of SPIN Gyroscopes Based on Nitrogen-Vacancy Centers in Diamond
2019
This project aims to develop solid-state gyroscopes based on ensembles of negatively charged nitrogen-vacancy (NV) centers in diamond [1], [2]. The NV center is a defect formed in diamond by one substitutional nitrogen atom and an adjacent vacancy. The NV- center features a ground state with electronic spin $\mathrm{S}=1$ , which can be initialized, manipulated, and detected via convenient optical, microwave and radiofrequency transitions (Fig. 1). Nuclear spins are appealing in the context of gyroscopes because they have much smaller gyromagnetic ratios than that of the electron (by a factor of about 1000), reducing the requirements on static magnetic-field stability and homogeneity. The l…
Dynamic N14 nuclear spin polarization in nitrogen-vacancy centers in diamond
2020
We studied the dynamic nuclear spin polarization of nitrogen in negatively charged nitrogen-vacancy (NV) centers in diamond both experimentally and theoretically over a wide range of magnetic fields from 0--1100 G covering both the excited-state level anticrossing and the ground-state level anticrossing magnetic field regions. Special attention was paid to the less studied ground-state level anticrossing region. The nuclear spin polarization was inferred from measurements of the optically detected magnetic resonance signal. These measurements show that a very large (up to $96\ifmmode\pm\else\textpm\fi{}2%$) nuclear spin polarization of nitrogen can be achieved over a very broad range of mag…
Fundaments of photoelectric readout of spin states in diamond
2021
Abstract The chapter “Fundaments of photoelectric readout of spin states in diamond” deals with the detection of NV centre spins in diamond using the photoelectric detection of magnetic resonances (PDMR) method, introduced in a series of recent publications. It provides in particular insights into the physics of electronic transitions of the NV center, leading to the free carrier generation, and discusses methodologies how to implement the photocurrent detection principles in the dynamically evolving field of quantum technologies. Recent results on the single electron and the single nuclear spin qubits photoelectric readout are presented, along with a microwave-free NV magnetometry techniqu…
Estimating the magnetic moment of microscopic magnetic sources from their magnetic field distribution in a layer of nitrogen-vacancy (NV) centres in …
2016
We have used a synthetic diamond with a layer of nitrogen-vacancy (NV) centres to image the magnetic field distributions of magnetic particles on the surface of the diamond. Magnetic field distributions of 4 µ m and 2 µ m ferromagnetic and 500 nm diameter superparamagnetic particles were obtained by measuring the position of the optically detected magnetic resonance peak in the fluorescence emitted by the NV centres for each pixel. We fitted the results to a model in order to determine the magnetic moment of the particles from the magnetic field image and compared the results to the measured magnetic moment of the particles. The best-fit magnetic moment differed from the value expected base…
Counter-propagating difference frequency mixing in diamond with terahertz waves
2013
We investigate four-wave mixing between terahertz and optical pulses in diamond. We observe the occurrence of sum and difference frequency generation, with the latter being phase-matched for terahertz pulses counter-propagating to the optical field.
Electrochemical Abatement of Organic Pollutants in Continuous-Reaction Systems through the Assembly of Microfluidic Cells in Series
2015
The electrochemical treatment of wastewater contaminated by organic pollutants was performed under a continuous mode by using, for the first time, various micro-electrochemical cells in series. A synthetic solution of acid orange 7 (AO7), a largely used azoic dye, was chosen as model wastewater. Both the electro-Fenton (EF) method with a cheap compact graphite cathode and electrochemical oxidation (EO) at a boron-doped diamond (BDD) anode were used. EO gave higher abatement of total organic carbon (TOC), but drastically higher energetic consumptions than EF. It is worth mentioning that very different operating conditions were set for EF and EO to optimize their performances. The utilization…
Genetic and Biochemical Characterization of Field-Evolved Resistance to Bacillus thuringiensis Toxin Cry1Ac in the Diamondback Moth, Plutella xyloste…
2004
ABSTRACT The long-term usefulness of Bacillus thuringiensis Cry toxins, either in sprays or in transgenic crops, may be compromised by the evolution of resistance in target insects. Managing the evolution of resistance to B. thuringiensis toxins requires extensive knowledge about the mechanisms, genetics, and ecology of resistance genes. To date, laboratory-selected populations have provided information on the diverse genetics and mechanisms of resistance to B. thuringiensis , highly resistant field populations being rare. However, the selection pressures on field and laboratory populations are very different and may produce resistance genes with distinct characteristics. In order to better…