Search results for "engineering.material"
showing 10 items of 2352 documents
Prospects of SPIN Gyroscopes Based on Nitrogen-Vacancy Centers in Diamond
2019
This project aims to develop solid-state gyroscopes based on ensembles of negatively charged nitrogen-vacancy (NV) centers in diamond [1], [2]. The NV center is a defect formed in diamond by one substitutional nitrogen atom and an adjacent vacancy. The NV- center features a ground state with electronic spin $\mathrm{S}=1$ , which can be initialized, manipulated, and detected via convenient optical, microwave and radiofrequency transitions (Fig. 1). Nuclear spins are appealing in the context of gyroscopes because they have much smaller gyromagnetic ratios than that of the electron (by a factor of about 1000), reducing the requirements on static magnetic-field stability and homogeneity. The l…
Electronic, magnetic, and structural properties of the ferrimagnet Mn2CoSn
2011
The magnetic ground state of the Heusler compound Mn${}_{2}$CoSn was predicted to be nearly half-metallic ferrimagnetic with a high spin polarization by ab initio electronic structure calculations. Mn${}_{2}$CoSn was synthesized, and the magnetic behavior of the compound was studied using a superconducting quantum interference device and x-ray magnetic circular dichroism. The experimental values were found to be in fair accordance with the theoretical predictions. The electronic structure and the crystal structure of Mn${}_{2}$CoSn were characterized comprehensively using x-ray powder diffraction, $^{119}\mathrm{Sn}$ M\"ossbauer spectroscopy, nuclear magnetic resonance, and hard x-ray photo…
Test of band structure calculations for Heusler compounds by spin-resolved photoemission spectroscopy
2012
The electronic density of states of epitaxial thin films of the Heusler compound Co${}_{2}$MnGa is probed in situ by spin-resolved ultraviolet photoemission spectroscopy. The experiments reveal several characteristic features in the intensity spectrum and a clear Fermi edge signature. A high spin polarization of $\ensuremath{\simeq}\phantom{\rule{-0.16em}{0ex}}55%$ at the Fermi edge is followed by a sign change at the binding energy of $\ensuremath{\simeq}$0.8 eV. Corresponding calculations of the band structure and the photoemission spectrum were performed employing a spin-polarized relativistic Korringa-Kohn-Rostoker code. Good agreement between the experimental data and calculations was …
Dynamic N14 nuclear spin polarization in nitrogen-vacancy centers in diamond
2020
We studied the dynamic nuclear spin polarization of nitrogen in negatively charged nitrogen-vacancy (NV) centers in diamond both experimentally and theoretically over a wide range of magnetic fields from 0--1100 G covering both the excited-state level anticrossing and the ground-state level anticrossing magnetic field regions. Special attention was paid to the less studied ground-state level anticrossing region. The nuclear spin polarization was inferred from measurements of the optically detected magnetic resonance signal. These measurements show that a very large (up to $96\ifmmode\pm\else\textpm\fi{}2%$) nuclear spin polarization of nitrogen can be achieved over a very broad range of mag…
Fundaments of photoelectric readout of spin states in diamond
2021
Abstract The chapter “Fundaments of photoelectric readout of spin states in diamond” deals with the detection of NV centre spins in diamond using the photoelectric detection of magnetic resonances (PDMR) method, introduced in a series of recent publications. It provides in particular insights into the physics of electronic transitions of the NV center, leading to the free carrier generation, and discusses methodologies how to implement the photocurrent detection principles in the dynamically evolving field of quantum technologies. Recent results on the single electron and the single nuclear spin qubits photoelectric readout are presented, along with a microwave-free NV magnetometry techniqu…
Heavy fermion spin liquid in herbertsmithite
2015
We analyze recent heat capacity measurements in herbertsmithite $\rm ZnCu_3(OH)_6Cl_2$ single crystal samples subjected to strong magnetic fields. We show that the temperature dependence of specific heat $C_{mag}$ formed by quantum spin liquid at different magnetic fields $B$ resembles the electronic heat capacity $C_{el}$ of the HF metal $\rm YbRh_2Si_2$. We demonstrate that the spinon effective mass $M^*_{mag}\propto C_{mag}/T$ exhibits a scaling behavior like that of $C_{el}/T$. We also show that the recent measurements of $C_{mag}$ are compatible with those obtained on powder samples. These observations allow us to conclude that $\rm ZnCu_3(OH)_6Cl_2$ holds a stable strongly correlated …
First-principles electronic structure of spinelLiCr2O4:A possible half-metal
2004
We have employed first-principles electronic structure calculations to examine the hypothetical (but plausible) oxide spinel, ${\mathrm{LiCr}}_{2}{\mathrm{O}}_{4}$ with the ${d}^{2.5}$ electronic configuration. The cell (cubic) and internal (oxygen position) structural parameters have been obtained for this compound through structural relaxation in the first-principles framework. Within the one-electron band picture, we find that ${\mathrm{LiCr}}_{2}{\mathrm{O}}_{4}$ is magnetic, and a candidate half-metal. The electronic structure is substantially different from the closely related and well-known rutile half-metal ${\mathrm{CrO}}_{2}.$ In particular, we find a smaller conduction-band width…
Negative magnetoresistance of ultra-narrow superconducting nanowires in the resistive state
2008
We present a phenomenological model qualitatively explaining negative magnetoresistance in quasi-one-dimensional superconducting channels in the resistive state. The model is based on the assumption that fluctuations of the order parameter (phase slips) are responsible for the finite effective resistance of a narrow superconducting wire sufficiently close to the critical temperature. Each fluctuation is accompanied by an instant formation of a quasi-normal region of the order of the non-equilibrium quasiparticle relaxation length 'pinned' to the core of the phase slip. The effective time-averaged voltage measured in experiment is a sum of two terms. First one is the conventional contributio…
Estimating the magnetic moment of microscopic magnetic sources from their magnetic field distribution in a layer of nitrogen-vacancy (NV) centres in …
2016
We have used a synthetic diamond with a layer of nitrogen-vacancy (NV) centres to image the magnetic field distributions of magnetic particles on the surface of the diamond. Magnetic field distributions of 4 µ m and 2 µ m ferromagnetic and 500 nm diameter superparamagnetic particles were obtained by measuring the position of the optically detected magnetic resonance peak in the fluorescence emitted by the NV centres for each pixel. We fitted the results to a model in order to determine the magnetic moment of the particles from the magnetic field image and compared the results to the measured magnetic moment of the particles. The best-fit magnetic moment differed from the value expected base…
Photoelectron spectra from first principles: from the many-body to the single-particle picture
2008
We derive a many-body method to evaluate photoelectron spectra of atoms, molecules and clusters from first principles. The excitation energies and the spectroscopic factors are calculated from the linear-response time-dependent density functional theory. The method is applied to noble metal anions, anionic clusters and to neutral small molecules. Our approach shows significant improvement over a simple single-particle treatment and gives an insight into the necessary conditions under which the single-particle picture holds. The consideration of the spectroscopic factor is shown to be crucial for the correct description of inner valence photoelectron peaks.