Search results for "fission"
showing 10 items of 421 documents
Odd-Even Effects in the Reaction 241Am(2n,f)
1992
Fission yields of the light fission products in the reaction 241Am(2n,f) have been measured. The results indicate an odd-even proton effect in the yield distribution of this odd nucleus with Z=95.
Rapid chemical separation procedures
1976
Fast, discontinuous separation procedures are described for zirconium, niobium, technetium and antimony from fission products. Other rapid separation methods from aqueous solutions are summarized. The combination of a gas jet recoil transport system with a continuous solvent extraction technique and with a thermochromatographic separation method is presented. The application of such procedures to the investigation of new and already known short-lived nuclides is illustrated by some examples.
Status of independent yield measurements
1996
Recent progress in the measurement of independent yields in low energy nuclear fission is presented. Different experimental approaches are discussed and a survey of the most important experimental results obtained is given. Physical consequences for the understanding of the fission process are briefly referred.
High Yield Ultrafast Intramolecular Singlet Exciton Fission in a Quinoidal Bithiophene
2015
We report the process of singlet exciton fission with high-yield upon photoexcitation of a quinoidal thiophene molecule. Efficient ultrafast triplet photogeneration and its yield are determined by photoinduced triplet-triplet absorption, flash photolysis triplet lifetime measurements, as well as by femtosecond time-resolved transient absorption and fluorescence methods. These experiments show that optically excited quinoidal bithiophene molecule undergoes ultrafast formation of the triplet-like state with the lifetime ∼57 μs. CASPT2 and RAS-SF calculations have been performed to support the experimental findings. To date, high singlet fission rates have been reported for crystalline and pol…
New antineutrino energy spectra predictions from the summation of beta decay branches of the fission products
2012
In this paper, we study the impact of the inclusion of the recently measured beta decay properties of the $^{102;104;105;106;107}$Tc, $^{105}$Mo, and $^{101}$Nb nuclei in an updated calculation of the antineutrino energy spectra of the four fissible isotopes $^{235, 238}$U, and $^{239,241}$Pu. These actinides are the main contributors to the fission processes in Pressurized Water Reactors. The beta feeding probabilities of the above-mentioned Tc, Mo and Nb isotopes have been found to play a major role in the $\gamma$ component of the decay heat of $^{239}$Pu, solving a large part of the $\gamma$ discrepancy in the 4 to 3000\,s range. They have been measured using the Total Absorption Techni…
Measurement of the heaviest Beta-delayed 2-neutron emitter: 136Sb
2017
The Beta-delayed neutron emission probability, Pn , of very exotic nuclei is crucial for the understanding of nuclear structure properties of many isotopes and astrophysical processes such as the rapid neutron capture process (r-process). In addition Beta-delayed neutrons are important in a nuclear power reactor operated in a prompt sub-critical, delayed critical condition, as they contribute to the decay heat inducing fission reactions after a shut down. The study of neutron-rich isotopes and the measurement of Beta-delayed one-neutron emitters (Beta1n) is possible thanks to the Rare Isotope Beam (RIB) facilities, where radioactive beams allow the production of exotic nuclei of interest, w…
Stability and synthesis of superheavy elements: Fighting the battle against fission – example of $^{254}$No
2016
International audience; Superheavy nuclei exist solely due to quantum shell effects,which create a pocket in the potential-energy surface of the nucleus, thusproviding a barrier against spontaneous fission. Determining the height ofthe fission barrier and its angular-momentum dependence is important toquantify the role that microscopic shell corrections play in enhancing andextending the limits of nuclear stability. In this talk, the first measurement ofa fission barrier in the very heavy nucleus 254No will be presented.
Rapid Synthesis of Radioactive Transition-Metal Carbonyl Complexes at Ambient Conditions
2012
Carbonyl complexes of radioactive transition metals can be easily synthesized with high yields by stopping nuclear fission or fusion products in a gas volume containing CO. Here, we focus on Mo, W, and Os complexes. The reaction takes place at pressures of around 1 bar at room temperature, i.e., at conditions that are easy to accommodate. The formed complexes are highly volatile. They can thus be transported within a gas stream without major losses to setups for their further investigation or direct use. The rapid synthesis holds promise for radiochemical purposes and will be useful for studying, e.g., chemical properties of superheavy elements.
Study of fusion reactions forming Cf nuclei
2013
The formation of a compound nucleus in different projectile and target combinations is a powerful method for investigating the fusion process. Recently, the dominance of quasi-fission over fusion-fission has been inferred for 34 S+208 Pb in comparison to 36 S+206 Pb; both reactions lead to the compound nucleus 242 Cf* .The mass and angle distributions of the fission fragments from these reactions were studied in order to further investigate the presence of quasi-fission.
Ultrafast internal conversion of excited cytosine via the lowest pipi electronic singlet state.
2003
Computational evidence at the CASPT2 level supports that the lowest excited state pipi* contributes to the S1/S0 crossing responsible for the ultrafast decay of singlet excited cytosine. The computed radiative lifetime, 33 ns, is consistent with the experimentally derived value, 40 ns. The nOpi* state does not play a direct role in the rapid repopulation of the ground state; it is involved in a S2/S1 crossing. Alternative mechanisms through excited states pisigma* or nNpi* are not competitive in cytosine.