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showing 10 items of 8115 documents

Metabolic shift of polyphosphate-accumulating organisms with different levels of polyphosphate storage

2012

Previous studies have shown that polyphosphate-accumulating organisms (PAOs) are able to behave as glycogen-accumulating organisms (GAOs) under different conditions. In this study we investigated the behavior of a culture enriched with Accumulibacter at different levels of polyphosphate (poly-P) storage. The results of stoichiometric ratios Gly degraded/HAc uptake, PHB synthesized/HAc uptake, PHV synthesized/HAc uptake and P release/HAc uptake confirmed a metabolic shift from PAO metabolism to GAO metabolism: PAOs with high poly-P content used the poly-P to obtain adenosine tri-phosphate (ATP), and glycogen (Gly) to obtain nicotinamide adenine dinucleotide (NADH) and some ATP. In a test whe…

Accumulibacter Type IIWaste component removalUnclassified drugPhysiologyChemical compositionMicrobial metabolismStorageWastewaterNicotinamide adenine dinucleotidePolyhydroxyalkanoic acidchemistry.chemical_compoundBacteriumBioreactorsPolyphosphatesGlycolysisAnaerobiosisBiomassPolyphosphate-accumulating organismsWaste Management and DisposalAccumulibacter Type IGlycogen accumulating organismPriority journalWater Science and TechnologyFluorescence microscopyPolyhydroxyvalerateSewageGlycogenHydrolysisFluorescence in situ hybridizationEcological ModelingPhosphorusHydrogen-Ion ConcentrationBioaccumulationPollutionStoichiometryWaste treatmentPolyphosphate-accumulating organismsBiodegradation EnvironmentalEnhanced biological phosphorus removalBiochemistryGlycogen-accumulating metabolism (GAM)Nicotinamide adenine dinucleotideAccumulibacter type 1Accumulibacter type 2GlycolysisGlycogenMetabolic Networks and PathwaysAccumulibacterAdenosine triphosphateEnvironmental EngineeringBiologyAcetic acidArticleAssociative storagePolyphosphate-accumulating metabolism (PAM)PolyphosphateGlycogen-accumulating organismsGlycogen-accumulating metabolismsTECNOLOGIA DEL MEDIO AMBIENTEPolyphosphate accumulating organismCivil and Structural EngineeringPolyphosphate-accumulating organisms (PAO)BacteriaPolyphosphateMetabolismIn situ measurementGlycogen-accumulating organisms (GAO)Polyphosphate-accumulating metabolismsNonhumanAmidesCarbonMetabolismchemistryPolyphosphate (poly-P)Bacterial metabolismCell cultureVolatilizationWater Research
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A molecular dynamics study on the role of the protonation state in the biosynthesis of R-PAC by AHAS

2019

Abstract The effect of the protonation state of the hydroxyl-ethylthiamin diphosphate intermediate, HEThDP, on the enzyme-substrate interactions and their consequences on the biosynthesis of R-phenylacetylcarbinol, R-PAC, by the acetohydroxy acid synthase, AHAS, is addressed by molecular dynamics simulations. It is found that the form of HEThDP, which favors the formation of R-PAC, is that having the 4-aminopyrimidine ring with the N1′ atom protonated and the N4′ atom as aminopyrimidinium ion. Under this form both active sites of AHAS have the ability to perform the catalysis, unlike that observed for the other possible protonation states of N1′ and N4′ atoms.

Acetohydroxy Acid SynthaseStereochemistryGeneral Physics and AstronomyProtonation02 engineering and technology010402 general chemistry021001 nanoscience & nanotechnologyRing (chemistry)01 natural sciences0104 chemical sciencesCatalysisIonchemistry.chemical_compoundMolecular dynamicsBiosynthesischemistryAtomPhysical and Theoretical Chemistry0210 nano-technologyChemical Physics Letters
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Purification and characterization of the catabolic ?-acetolactate synthase from Leuconostoc mesenteroides subsp. cremoris

1995

The α-acetolactate synthase from Leuconostoc mesenteroides subsp. cremoris was purified to homogeneity in SDS-PAGE. The enzyme is a trimer of 3×55,000 Da. It was unstable but could be preserved by addition of pyruvate and thiamine pyrophosphate in the buffer. The enzyme exhibits Michaelis-Menten kinetics, and Km for pyruvate is 10 mM. Three intermediates in glucose metabolism (ATP, 3-phosphoglycerate, and phosphoenolpyruvate) exhibit a noncompetitive inhibition towards the enzyme. This enzyme does not require any divalent metal ion for activity. The α-acetolactate synthase from Leuconostoc mesenteroides subsp. cremoris is not inhibited by the branched-chain amino acids (valine, leucine, and…

Acetolactate synthasebiologyATP synthaseGeneral Medicinebiology.organism_classificationApplied Microbiology and BiotechnologyMicrobiologychemistry.chemical_compoundNon-competitive inhibitionchemistryBiochemistryBiosynthesisValineLeuconostoc mesenteroidesbiology.proteinIsoleucineThiamine pyrophosphateCurrent Microbiology
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Reversed phase liquid chromatography for the enantioseparation of local anaesthetics in polysaccharide-based stationary phases. Application to biodeg…

2020

[EN] A comprehensive study on the chiral separation of bupivacaine, mepivacaine, prilocaine and propanocaine with eight commercial polysaccharide-based chiral stationary phases (CSPs) in reversed phase conditions compatible with MS detection is performed. Methanol and acetonitrile are used as organic modifiers. Retention and resolution values obtained for each compound in the different CSPs and mobile phases are compared. The polysaccharide-based CSPs tested present different enantioselectivity towards the analytes. From the results, the experimental conditions for determining the enantiomers of bupivacaine, mepivacaine, prilocaine and propanocaine in saline aqueous samples using MS detecti…

AcetonitrilesResolution (mass spectrometry)Mepivacaine010402 general chemistry01 natural sciencesBiochemistryAnalytical Chemistrychemistry.chemical_compoundReversed phase conditionsPolysaccharidesPhase (matter)medicineEnantioselective biodegradation studyAnesthetics LocalAcetonitrileLocal anaestheticsChromatography High Pressure LiquidChromatography Reverse-PhaseAqueous solutionChromatographyCellulose and amylose-based chiral stationary phasesMethanol010401 analytical chemistryOrganic ChemistryEnantioselective synthesisWaterStereoisomerismGeneral MedicineReversed-phase chromatography0104 chemical sciencesMolecular WeightBiodegradation EnvironmentalchemistryEnantiomermedicine.drugJournal of chromatography. A
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Detection of an O-methyltransferase synthesising acetosyringone in methyl jasmonate-treated tobacco cell-suspensions cultures.

2013

Acetosyringone (3',5'-dimethoxy-4'-hydroxyacetophenone) is a well-known and very effective inducer of the virulence genes of Agrobacterium tumefaciens but the precise pathway of its biosynthesis in plants is still unknown. We have used two tobacco cell lines, cultured in suspension and exhibiting different patterns of accumulation of acetosyringone in their culture medium upon treatment with methyl jasmonate, to study different steps of acetosyringone biosynthesis. In the two cell lines studied, treatment with 100 mu M methyl jasmonate triggered a rapid and transient increase in acetovanillone synthase activity followed by a progressive increase in S-adenosyl-L-methionine: 5-hydroxyacetovan…

AcetosyringoneAcetosyringone5-Hydroxyacetovanillone[SDV]Life Sciences [q-bio]Nicotiana tabacumPlant ScienceCyclopentanesHorticultureAcetatesBiochemistryHydroxylationchemistry.chemical_compoundStructure-Activity RelationshipBiosynthesisSuspensionsTobacco[SDV.BV]Life Sciences [q-bio]/Vegetal BiologyOxylipinsMolecular BiologyCells CulturedJasmonic acidMethyl jasmonatebiologyDose-Response Relationship DrugMolecular StructureJasmonic acidAcetophenonesGeneral MedicineAgrobacterium tumefaciensMethyltransferasesbiology.organism_classificationO-methyltransferasechemistryBiochemistry[SDE]Environmental Sciencesbiology.proteinPhytochemistry
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Aminosäureester als chirale Hilfsgruppen in Lewis-Säure-katalysierten Diels-Alder-Reaktionen

1990

Amino Acid Esters as Chiral Auxiliaries in Lewis Acid Catalyzed Diels-Alder Reactions Cyclopentadiene, cyclohexadiene and alkyl-substituted butadienes react with N-acryloyl-, N-crotonoyl- and N-(4-nitro-cinnamoyl)-(S)-proline benzyl and allyl ester in the presence of Lewis acids to give the cycloadducts in high yields and with stereoselectivities of up to 97:3 for the endo isomers. The sense of the asymmetric induction in these reactions can be directed by the use of differently coordinating catalysts (e.g. TiCl4: (2R):(2S) = 96:4; EtAlCl2: (2R):(2S) = 10:90 at 0°C). In the TiCl4-catalyzed reactions with the fumaric acid derivatives the ratio of the diastereomers reaches values of up to 112…

Acid catalysisChemistryOrganic ChemistryIodolactonizationDiastereomerEnantioselective synthesisOrganic chemistryIminiumLewis acids and basesPhysical and Theoretical ChemistryAsymmetric inductionMedicinal chemistryLewis acid catalysisLiebigs Annalen der Chemie
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Acid-mediated reaction of bis(pyridine)iodonium(I) tetrafluoroborate with aromatic compounds. A selective and general iodination method

1993

Reaction of aromatic compounds with bis(pyridine)iodonium(I) tetrafluoroborate (IPy2BF4) in the presence of HBF4 or CF3SO3H in CH2Cl2 at room temperature furnishes monoiodo derivatives with excellent regioselectivity and yields. Use of either acid gives comparable results with activated aromatics, whereas CF3SO3H is much more effective in the iodination of deactivated aromatics. © 1993 American Chemical Society.

Acid catalysischemistry.chemical_compoundElectrophilic substitutionTetrafluoroboratechemistryOrganic ChemistryPyridineRegioselectivityHalogenationOrganic chemistryBis(pyridine)iodonium(I) tetrafluoroborateChemical societyThe Journal of Organic Chemistry
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Modeling the anaerobic treatment of sulfate rich urban wastewater. Application to AnMBR technology

2020

[EN] Although anaerobic membrane bioreactors (AnMBR) are a core technology in the transition of urban wastewater (UWW) treatment towards a circular economy, the transition is being held back by a number of bottlenecks. The dissolved methane released from the effluent, the need to remove nutrients (ideally by recovery), or the energy lost by the competition between methanogenic and sulfate-reducing bacteria (SRB) for the biodegradable COD have been identified as the main issues to be addressed before AnMBR becomes widespread. Mathematical modeling of this technology can be used to obtain further insights into these bottlenecks plus other valuable information for design, simulation and contro…

AcidogenesisAnaerobic membrane bioreactorEnvironmental EngineeringMethanogenesis0208 environmental biotechnology02 engineering and technology010501 environmental sciencesWastewater01 natural sciencesWaste Disposal FluidBioreactorsBNRM2BioreactorAnaerobiosisWaste Management and DisposalEffluentTECNOLOGIA DEL MEDIO AMBIENTE0105 earth and related environmental sciencesWater Science and TechnologyCivil and Structural EngineeringSulfate-rich urban wastewaterSulfatesEcological ModelingModelingPulp and paper industryPollution020801 environmental engineeringAnaerobic digestionPilot plantWastewaterAcetogenesisEnvironmental scienceMethane
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Application of the General Model "Biological Nutrient Removal Model No.1" to upgrade two full-scale WWTPs

2012

In this paper, two practical case studies for upgrading two wastewater treatment plants (WWTPs) using the general model BNRM1 (Biological Nutrient Removal Model No. 1) are presented. In the first case study, the Tarragona WWTP was upgraded by reducing the phosphorus load to the anaerobic digester in order to minimize the precipitation problems. Phosphorus load reduction was accomplished by mixing the primary sludge and the secondary sludge and by elutriating the mixed sludge. In the second case study, the Alcantarilla WWTP, the nutrient removal was enhanced by maintaining a relatively low dissolved oxygen concentration in Stage A to maintain the acidogenic bacteria activity. The VFA produce…

AcidogenesisBiological nutrient removalWATER TREATMENT PLANTSAerobic bacteriachemistry.chemical_elementActivated sludge modelPhosphatesWater PurificationWASTE-WATERBNRM1Environmental ChemistryAnaerobiosisOrganic ChemicalsWaste Management and DisposalTECNOLOGIA DEL MEDIO AMBIENTEWater Science and TechnologyCALIBRATIONSewagePhosphorusEnvironmental engineeringGeneral MedicineModels TheoreticalASM2DAerobiosisACTIVATED-SLUDGE MODELActivated sludge modelsEnhanced biological phosphorus removalWastewaterchemistrySIMULATIONPlant-wide mathematical modellingEnvironmental scienceSewage treatmentWater treatmentSanitary EngineeringWWTP upgrading
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Complete genome sequence of the strain Defluviitoga tunisiensis L3, isolated from a thermophilic, production-scale biogas plant.

2015

An anaerobic, thermophilic bacterium belonging to the phylum Thermotogae was isolated from a rural, thermophilic biogas plant (54 degrees C) producing methane-rich biogas from maize silage, barley, cattle and pig manure. Here we report the first complete genome sequence of the Defluviitoga tunisiensis strain L3, an isolate from the family Thermotogaceae. The strain L3 encodes several genes predicted to be involved in utilization of a large diversity of complex carbohydrates including cellobiose and xylan for the production of acetate, hydrogen (H-2) and carbon dioxide (CO2). The genome sequence of D. tunisiensis L3 provides the basis for biotechnological exploitation of genetic determinants…

AcidogenesisSilageMolecular Sequence DataBioengineeringCellobioseRenewable primary productsApplied Microbiology and Biotechnologychemistry.chemical_compoundBiogasBotanyAlphaproteobacteriaWhole genome sequencingThermotogaebiologyBase SequenceThermophileGeneral MedicineSequence Analysis DNAAcidogenesisbiology.organism_classificationBiogas productionchemistryGenes BacterialThermotogaeCarbohydrate utilizationFermentationGenome BacterialBiotechnologyJournal of biotechnology
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