Search results for "mesoscopic"
showing 10 items of 709 documents
Probing magnetism in 2D van der Waals crystalline insulators via electron tunneling
2018
Magnetic insulators are a key resource for next-generation spintronic and topological devices. The family of layered metal halides promises varied magnetic states, including ultrathin insulating multiferroics, spin liquids, and ferromagnets, but device-oriented characterization methods are needed to unlock their potential. Here, we report tunneling through the layered magnetic insulator CrI₃ as a function of temperature and applied magnetic field.We electrically detect the magnetic ground state and interlayer coupling and observe a fieldinducedmetamagnetic transition.The metamagnetic transition results in magnetoresistances of 95, 300, and 550% for bilayer, trilayer, and tetralayer CrI₃ bar…
Mesoscopic structural organization in fluorinated room temperature ionic liquids
2018
The presence of fluorous tails in room-temperature ionic liquids imparts new properties to their already rich spectrum of appealing features. The interest towards this class of compounds that are of ionic nature with melting point less than 25 degrees C is accordingly growing; in particular, compounds bearing relatively long fluorous tails have begun to be considered. In this invited presentation, we show recent results arising from the systematic study of structural properties of a series of fluorinated room temperature ionic liquids, with growing fluorous chain length. At odd with the current understanding of this class of compounds, we show experimentally that they are characterized by t…
Nanoscale organization in the fluorinated room temperature ionic liquid: Tetraethyl ammonium (trifluoromethanesulfonyl)(nonafluorobutylsulfonyl)imide
2018
Fluorinated Room Temperature Ionic Liquids (FRTILs) are a branch of ionic liquids that is the object of growing interest for a wide range of potential applications, due to the synergic combination of specifically ionic features and those properties that stem from fluorous tails. So far limited experimental work exists on the micro-and mesoscopic structural organization in this class of compounds. Such a work is however necessary to fully understand morphological details at atomistic level that would have strong implications in terms of bulk properties. Here we use the synergy between X-ray and neutron scattering together with molecular dynamics simulations to access structural details of a …
Simultaneous photonic and excitonic coupling in spherical quantum dot supercrystals
2020
Semiconductor nanocrystals, or quantum dots (QDs), simultaneously benefit from inexpensive low-temperature solution processing and exciting photophysics, making them the ideal candidates for next-generation solar cells and photodetectors. While the working principles of these devices rely on light absorption, QDs intrinsically belong to the Rayleigh regime and display optical behavior limited to electric dipole resonances, resulting in low absorption efficiencies. Increasing the absorption efficiency of QDs, together with their electronic and excitonic coupling to enhance charge carrier mobility, is therefore of critical importance to enable practical applications. Here, we demonstrate a ge…
Temperature Effects on the Phonon Spectrum in YBa2Cu3O7 Single Crystals and Thin Films
1989
We have performed a detailed investigation of the temperature dependence of the 385cm-1 phonon in single crystals and thin films of the YBa2Cu3O7 superconductor by means of Raman spectroscopy. In the single crystal the frequency of this phonon shows a downshift of about 5 cm-1 on passing the superconducting transition from above, which is referred to a strong electron-phonon interaction in the superconductor. The shift of the phonon in thin epitaxial films on MgO or SrTiO3 substrates is only about 2.5 cm-1. This difference may be a result of a structural transition in the single crystal which is possibly suppressed in the films because of the epitaxy. The electron-phonon interaction is also…
Magnetic Anisotropies and Coupling Mechanisms inFe/Mo(110)Nanostripes
2005
Using low-temperature (5 K) spin-polarized scanning tunneling microscopy, we have studied the morphology and magnetic properties of monolayer (ML) and double layer (DL) thick Fe nanowires grown by step flow on a Mo(110) single crystal. Magnetic contrast has been obtained using tungsten tips covered by Au/Co thin films. We find that the DL Fe nanowires, similarly to ML Fe nanowires, are perpendicularly magnetized. Because of the dipolar coupling, separated DL Fe nanowires are antiferromagnetically coupled. DL wires that are touching at step edges are ferromagnetically ordered due to direct exchange coupling. We measured the widths of the magnetic domain walls in the ML and DL Fe nanowires. T…
Current-Induced Skyrmion Generation through Morphological Thermal Transitions in Chiral Ferromagnetic Heterostructures.
2018
© 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim Magnetic skyrmions promise breakthroughs in future memory and computing devices due to their inherent stability and small size. Their creation and current driven motion have been recently observed at room temperature, but the key mechanisms of their formation are not yet well-understood. Here it is shown that in heavy metal/ferromagnet heterostructures, pulsed currents can drive morphological transitions between labyrinth-like, stripe-like, and skyrmionic states. Using high-resolution X-ray microscopy, the spin texture evolution with temperature and magnetic field is imaged and it is demonstrated that with transient Joule heating, topologica…
Spin Hall magnetoresistance in the non-collinear ferrimagnet GdIG close to the compensation temperature
2017
We investigate the spin Hall magnetoresistance (SMR) in a gadolinium iron garnet (GdIG)/platinum (Pt) heterostructure by angular dependent magnetoresistance measurements. The magnetic structure of the ferromagnetic insulator GdIG is non-collinear near the compensation temperature, while it is collinear far from the compensation temperature. In the collinear regime, the SMR signal in GdIG is consistent with the usual [Formula: see text] relation well established in the collinear magnet yttrium iron garnet, with [Formula: see text] the angle between magnetization and spin Hall spin polarization direction. In the non-collinear regime, both an SMR signal with inverted sign and a more complex an…
Meshless meso-modeling of masonry in the computational homogenization framework
2017
In the present study a multi-scale computational strategy for the analysis of structures made-up of masonry material is presented. The structural macroscopic behavior is obtained making use of the Computational Homogenization (CH) technique based on the solution of the Boundary Value Problem (BVP) of a detailed Unit Cell (UC) chosen at the mesoscale and representative of the heterogeneous material. The attention is focused on those materials that can be regarded as an assembly of units interfaced by adhesive/cohesive joints. Therefore, the smallest UC is composed by the aggregate and the surrounding joints, the former assumed to behave elastically while the latter show an elastoplastic soft…
Wave-vector analysis of plasmon-assisted distributed nonlinear photoluminescence along Au nanowires
2020
We report a quantitative analysis of the wavevector diagram emitted by nonlinear photoluminescence generated by a tightly focused pulsed laser beam and distributed along Au nanowire via the mediation of surface plasmon polaritions. The nonlinear photoluminescence is locally excited at key locations along the nanowire in order to understand the different contributions constituting the emission pattern measured in a conjugate Fourier plane of the microscope. Polarization-resolved measurements reveal that the nanowire preferentially emits nonlinear photoluminescence polarized transverse to the long axis at close to the detection limit wavevectors with a small azimuthal spread in comparison to …