Search results for "nanoscale"
showing 10 items of 752 documents
Effective Seiberg-Witten gauge theory of noncollinear magnetism
2020
Smoothly varying magnetization textures such as domain walls, skyrmions or hopfions serve as promising candidates for the information bits of the future. Understanding their physical properties is both a major field of interest and a theoretical challenge, involving the physics on different length scales. Here, we apply the phase space formulation of quantum mechanics to magnetic insulators and metals in the limit of zero temperature to obtain a gradient expansion in terms of real-space derivatives of the magnetization. Our primary focus is the anomalous Hall effect in noncollinear magnets which serves as an important proxy in the detection of localized magnetic structures. We formulate the…
Atlas for the properties of elemental 2D metals
2018
Common two-dimensional (2D) materials have a layered 3D structure with covalently bonded, atomically thin layers held together by weak van der Waals forces. However, in a recent transmission electron microscopy experiment, atomically thin 2D patches of iron were discovered inside a graphene nanopore. Motivated by this discovery, we perform a systematic density-functional study on atomically thin elemental 2D metal films, using 45 metals in three lattice structures. Cohesive energies, equilibrium distances, and bulk moduli in 2D are found to be linearly correlated to the corresponding 3D bulk properties, enabling the quick estimation of these values for a given 2D metal and lattice structure…
Lanthanide molecular nanomagnets as probabilistic bits
2023
Abstract Over the decades, the spin dynamics of a large set of lanthanide complexes have been explored. Lanthanide-based molecular nanomagnets are bistable spin systems, generally conceptualized as classical bits, but many lanthanide complexes have also been presented as candidate quantum bits (qubits). Here we offer a third alternative and model them as probabilistic bits (p-bits), where their stochastic behavior constitutes a computational resource instead of a limitation. We present a modelling tool for molecular spin p-bits, we demonstrate its capability to simulate bulk magnetic relaxation data and ac experiments and to simulate a minimal p-bit network under realistic conditions. Final…
Low-frequency excitation of double quantum dots
2008
We address theoretically adiabatic regime of charge transport for a model of two tunnel-coupled quantum dots connected in series. The energy levels of the two dots are harmonically modulated by an external potential with a constant phase shift between the two. Motivated by recent experiments with surface-acoustic-wave excitation, we consider two situations: (a) pure pumping in the absence of external voltage (also at finite temperature), and (b) adiabatic modulation of the current driven by large external bias. In both cases we derive results consistent with published experimental data. For the case (b) we explicitly derive the adiabatic limit of Tien-Gordon formula for photon-assisted tunn…
Heat transfer across a vacuum gap induced by piezoelectrically mediated acoustic phonon tunneling
2023
In contradictin to the common concept that acoustic phonons can only travel inside a material medium, they can in fact "tunnel" across a vacuum gap with the help of piezoelectricity, transmitting a significantly stronger heat flux than that of blackbody radiation. Here, we present a theoretical formulation for the heat flux of such piezoelectrically mediated heat transfer, applicable to any anisotropic piezoelectric crystals with an arbitrary orientation. A few numerical results are demonstrated and compared to heat transfer driven by other close-range mechanisms, including near-field radiative heat transfer and other acoustic phonon tunneling mechanisms. We find that piezoelectrically medi…
Mechanical effects in quantum dots in magnetic and electric fields
2001
The mechanical effects in finite two-dimensional electron systems (quantum dots or droplets) in a strong perpendicular magnetic field are studied. It is shown that, due to asymmetry of the cyclotron dynamics, an additional in-plane electric field causes a ground state transition accompanied by a change in the average total angular momentum of the system, unless the lateral confining potential is exactly parabolic. A precise mechanical experiment is proposed in which a macroscopic angular momentum of a dense matrix of quantum dots could be measured and used to detect and estimate anharmonicity of the confinement.
Coexistence of weak and strong coupling with a quantum dot in a photonic molecule
2018
We study the emission from a molecular photonic cavity formed by two proximal photonic crystal defect cavities containing a small number (<3) of In(Ga)As quantum dots. Under strong excitation we observe photoluminescence from the bonding and antibonding modes in excellent agreement with expectations from numerical simulations. Power dependent measurements reveal an unexpected peak, emerging at an energy between the bonding and antibonding modes of the molecule. Temperature dependent measurements show that this unexpected feature is photonic in origin. Time-resolved measurements show the emergent peak exhibits a lifetime $��_M=0.75 \, \pm 0.1 \, ns $, similar to both bonding and antibondi…
Noise in refrigerating tunnel junctions and in microbolometers
2000
Microrefrigerators based on normal metal-insulator-superconductor (NIS) junctions represent a very attractive alternative to cool the microbolometers and calorimeters for astrophysical observations in space-borne experiments. The performance in such measurements requires a good knowledge of the noise sources in the detectors. In this paper we present detailed calculations of the thermal fluctuations and of the noise equivalent power due to the heat transfer through the NIS junctions or due to the thermal contact between different subsystems of the detector. The influence of the background radiation will also be evaluated. Analytical approximations, valid at low temperatures, are given.
First-principles many-body calculations of electronic conduction in thiol- and amine-linked molecules
2011
The electronic conductance of a benzene molecule connected to gold electrodes via thiol, thiolate, and amino anchoring groups is calculated using nonequilibrium Green functions in combination with the fully selfconsistent GW approximation. The calculated conductance of benzenedithiol and benzenediamine is five times lower than predicted by standard density functional theory (DFT) in very good agreement with experiments. In contrast, the widely studied benzenedithiolate structure is found to have a significantly higher conductance due to the unsaturated sulfur bonds. These findings suggest that more complex gold/thiolate structures where the thiolate anchors are chemically passivated by Au a…
Electronic and optical trends in carbon nanotubes under pure bending
2010
The high aspect ratio of carbon nanotubes makes them prone to bending. To know how bending affects the tubes is therefore crucial for tube identification and for electrical component design. Very few studies, however, have investigated tubes under small bending well below the buckling limit, because of technical problems due to broken translational symmetry. In this Letter a cost-effective and exact modeling of singe-walled nanotubes under such small bending is enabled by revised periodic boundary conditions, combined with density-functional tight-binding. The resulting, bending-induced changes in electronic and optical properties fall in clear chirality-dependent trend families. While the …