Search results for "plasmon"
showing 10 items of 614 documents
The SVZ plasmon
1985
The sum rule technique of Shifman, Vainshtein and Zakharov is applied to a non-relativistic many-body system, the homogeneous, degenerate electron gas. The operator product expansion for the nonrelativistic correlation function is derived and shown to be equivalent in lowest order to a moment expansion. The nonperturbative terms in this expansion characterize the interacting ground state (“vacuum”) of the system. For the electron gas they can be related to the correlation energy which is very well known. Following as close as possible the SVZ procedure the mass of the plasmon (i.e. the dispersion coefficient of the collective plasma excitation) is calculated and compared with results from c…
Bulk-plasmon dispersion relations in metals
1991
En utilisant une technique de la regle de somme dans l'approximation de la phase aleatoire etendue, on examine la relation de dispersion des plasmons en volume, en introduisant les effets de la correlation et de l'echange dans le modele du jellium. Les resultats obtenus sont compares aux resultats experimentaux. On souligne le role cle que jouent les effets de la correlation et de l'echange dans l'amelioration de l'accord entre la theorie et l'experience. On calcule egalement la polarisabilite statique en fonction de 9. Les formules peuvent etre facilement modifiees pour incorporer les effets de la structure de bandes (a travers une masse effective electronique intrabande) et les effets de …
Electron-gas clusters: the ultimate jellium model
1995
The local spin-density approximation is used to calculate ground- and isomeric-state geometries of jellium clusters with 2 to 22 electrons. The positive background charge of the model is completely deformable, both in shape and in density. The model has no input parameters. The resulting shapes of the clusters exhibit breaking of axial and inversion symmetries; in general the shapes are far from ellipsoidal. Those clusters which lack inversion symmetry are extremely soft against odd-multipole deformations. Some clusters can be interpreted as molecules built from magic clusters. The deformation produces a gap at the Fermi level. This results in a regular odd-even staggering of the total ener…
Dressed states of a quantum emitter strongly coupled to a metal nanoparticle
2016
Hybrid molecule-plasmonic nanostructures have demonstrated their potential for surface enhanced spectroscopies, sensing, or quantum control at the nanoscale. In this Letter, we investigate the strong coupling regime and explicitly describe the hybridization between the localized plasmons of a metal nanoparticle and the excited state of a quantum emitter, offering a simple and precise understanding of the energy exchange in full analogy with cavity quantum electrodynamics treatment and a dressed atom picture. Both near-field emission and far-field radiation are discussed, revealing the richness of such optical nanosources.
Quantum emitter states dressed by the plasmon modes of a metal nanoparticle in the strong coupling regim
2017
The quantum control of emitters is a key issue for quantum information processing at the nanoscale. This generally necessitates the strong coupling of emitters to a high Q-cavity for efficient manipulation of the atoms and field dynamics (cavity quantum electrodynamics or cQED). Since almost a decade, strong efforts are put to transpose cQED concepts to plasmonics in order to profit of the strong mode confinement of surface plasmons polaritons. Despite the intrinsic presence of lossy channels leading to strong decoherence in plasmonics systems, it has been experimentally proven that it is possible to reach the strong coupling regim [1].
Coupling of a dipolar emitter into one-dimensional surface plasmon.
2013
Quantum plasmonics relies on a new paradigm for light-matter interaction. It benefits from strong confinement of surface plasmon polaritons (SPP) that ensures efficient coupling at a deep subwavelength scale, instead of working with a long lifetime cavity polariton that increases the duration of interaction. The large bandwidth and the strong confinement of one dimensional SPP enable controlled manipulation of a nearby quantum emitter. This paves the way to ultrafast nanooptical devices. However, the large SPP bandwidth originates from strong losses so that a clear understanding of the coupling process is needed. In this report, we investigate in details the coupling between a single emitte…
Nonlinear plasmonic amplification via dissipative soliton-plasmon resonances
2017
In this contribution we introduce a new strategy for the compensation of plasmonic losses based on a recently proposed nonlinear mechanism: the resonant interaction between surface plasmon polaritons and spatial solitons propagating in parallel along a metal/dielectric/Kerr structure. This mechanism naturally leads to the generation of a quasi-particle excitation, the so-called soliplasmon resonance. We analyze the role played by the effective nonlinear coupling inherent to this system and how this can be used to provide a new mechanism of quasi-resonant nonlinear excitation of surface plasmon polaritons. We will pay particular attention to the introduction of asymmetric linear gain in the …
Near Field of Strongly Coupled Plasmons: Uncovering Dark Modes
2012
Strongly coupled plasmons in a system of individual gold nanoparticles placed at subnanometer distance to a gold film (nanoparticle-on-plane, NPOP) are investigated using two complementary single particle spectroscopy techniques. Optical scattering spectroscopy exclusively detects plasmon modes that couple to the far field via their dipole moment (bright modes). By using photoemission electron microscopy (PEEM), we detect in the identical NPOPs near-field modes that do not couple to the scattered far field (dark modes) and are characterized by a strongly enhanced nonlinear electron emission process. To our knowledge, this is the first time that both far- and near-field spectroscopy are carr…
Numerical study on the limit of quasi-static approximation for plasmonic nanosphere
2019
Plasmonic nanospheres are often employed as resonant substrates in many nanophotonic applications, like in enhanced spectroscopy, near-field microscopy, photovoltaics, and sensing. Accurate calculation and tuning of optical responses of such nanospheres are essential to achieve optimal performance. Mie theory is widely used to calculate optical properties of spherical particles. Although, an approximated version of Mie approach, the quasi-static approximation (QSA) can also be used to determine the very same properties of those spheres with a lot simpler formulations. In this work, we report our numerical study on the limit and accuracy of QSA with respect to the rigorous Mie approach. We c…
Intensity-Based Single Particle Plasmon Sensing.
2021
Plasmon sensors respond to local changes of their surrounding environment with a shift in their resonance wavelength. This response is usually detected by measuring light scattering spectra to determine the resonance wavelength. However, single wavelength detection has become increasingly important because it simplifies the setup, increases speed, and improves statistics. Therefore, we investigated theoretically how the sensitivity toward such single wavelength scattering intensity changes depend on the material and shape of the plasmonic sensor. Surprisingly, simple equations describe this intensity sensitivity very accurately and allow us to distinguish the various contributions: Rayleigh…