Search results for "spontaneous emission"
showing 10 items of 145 documents
Comparison of asymmetric and symmetric cavity configurations of erbium-doped fiber laser in active Q-switched regime
2012
We present a comparative analysis of the dynamics of an actively Q-switched erbium-doped fiber laser assembled in two configurations of Fabry–Perot cavity, asymmetric and symmetric, specified by the location of an acousto-optic Q-switch modulator relative to the output couplers. In both configurations, the length of an active (Er3+-doped) fiber is chosen such that the laser does not spuriously emit at the moments when the modulator is blocked, which is important for the pulse-on-demand operation. We show experimentally that the symmetric cavity configuration permits enlarging of the active fiber length twice as compared to the asymmetric one, thereby increasing the energy and decreasing the…
Halide perovskite amplifiers integrated in polymer waveguides
2016
Semiconductor organometallic halide perovskites (CH 3 NH 3 PbX 3 , X=Cl, Br, I) (HPVK) have emerged as a new promising material able to improve the optoelectronic technology performance. Although this material has mostly been applied to improve the efficiency of photovoltaic devices, it also shows amazing properties for photonic applications. In particular, HPVK exhibits high photoluminescence (PL) quantum yield (up to 70%) at room temperature together with a tunable band-gap controlled by its chemical composition. In addition, since HPVKs is deposited in solution at room conditions, it can be easily incorporated in different photonic structures to efficiently exploit its emission propertie…
Tunable all-optical negative multitap microwave filters based on uniform fiber Bragg gratings.
2003
We present a novel and simple technique for obtaining transversal filters with negative coefficients by using uniform fiber Bragg gratings. We demonstrate a wide tuning range, good performance, low cost, and easy implementation of multitap filters in an all-optical passive configuration in which negative taps are obtained by use of the transmission of a broadband source through uniform Bragg gratings.
Inhibition of light emission from the metastable tetragonal phase at low temperatures in island-like films of lead iodide perovskites
2019
Photonic applications based on halide perovskites, namely CH3NH3PbI3 (MAPbI3), have recently attracted remarkable attention due to the high efficiencies reported for photovoltaic and light emitting devices. Despite these outstanding results, there are many temperature-, laser excitation power-, and morphology-dependent phenomena that require further research to be completely understood. In this work, we have investigated in detail the nature of exciton optical transitions and recombination dynamics below and above the orthorhombic/tetragonal ('O'-/'T'-) temperature phase transition (∼150 K) depending on the material continuity (continuous-like) or discontinuity (island-like) in MAPbI3 films…
Integration of a perovskite-based amplifier and photodetector system in rigid and solid substrates
2021
During the last years, organometallic lead halide perovskites (LHP) have been widely studied as outstanding materials for photovoltaics and photonics applications [1] . These emerging semiconductors are fabricated by cheap and straightforward solution process techniques on polycrystalline film of the compound CH 3 NH 3 PbX 3 (X=Cl, Br, I). Their outstanding properties of these films include large absorption coefficients above the bandgap, high electronic mobilities, high quantum yield of emission at room temperature or tunable band-gap with the composition [1] . In this work, we exploit the excellent light emitting and photodetection properties of CH 3 NH 3 PbI 3 thin films to integrate a w…
Polymer Halide Perovskites-Waveguides Integrated in Nanocellulose as a Wearable Amplifier-Photodetector System
2018
Semiconductor organometallic halide (CH 3 NH 3 PbX 3 , X=Cl, Br, I) perovskites (MHP) have emerged as a very high promising material for optoelectronics. Their large absorption coefficients, high electronic mobilities, excellent quantum yield of emission at room temperature and tunable band-gap with the composition resulted in a new generation of photovoltaics and electronic devices. In this work, HPVK materials are successfully incorporated on a nanocellulose (NC) substrate with the intention to exploit the interesting properties of HPVK materials to construct wearable devices. In particular, a bilayer Poly(methyl methacrylate) /HPVK deposited on NC resulted in a suitable waveguide to demo…
Experimental and theoretical studies of polaron optical properties in KNbO3 perovskite
2004
Time-resolved absorption and luminescence spectra have been measured in KNbO3 perovskite crystals after pulsed band-gap excitation by 200 fs laser pulses and 10 ns electron pulses. Quantum chemical calculations using the large unit cell periodic model support the interpretation of the observed transient absorption bands at 0.8 and 1.1 eV as the self-trapped electron polarons and bound hole polarons, respectively. The activation energy for the 2.2 eV green luminescence quenching is 0.05 eV. We suggest that the short lifetime (,15 ns) of the luminescence at RT is caused by the radiative recombination of nearest electron and hole polarons. q 2003 Elsevier Ltd. All rights reserved.
Radiative phonon-assisted and Auger recombination in Si nanocrystals
2010
Abstract Recent analysis of the literature shows that the photoluminescence (PL) of Si nanocrystals and porous silicon is caused by phonon-assisted exciton radiative recombination, as well as by direct radiative electron transfer from the second to the first conduction sub-band, which is related to the Auger recombination. The PL decay curve for porous silicon after excitation with ultraviolet laser pulse has been established experimentally. We have constructed continuity equations for the first and the second conduction sub-bands, including radiative phonon-assisted exciton recombination, Auger recombination and direct radiative transition from the second to the first conduction sub-band. …
Delayed Luminescence in Lead Halide Perovskite Nanocrystals
2017
The mechanism responsible for the extremely long photoluminescence (PL) lifetimes observed in many lead halide perovskites is still under debate. While the presence of trap states is widely accepted, the process of electron detrapping back to the emissive state has been mostly ignored, especially from deep traps as these are typically associated with nonradiative recombination. Here, we study the photophysics of methylammonium lead bromide perovskite nanocrystals (PNCs) with a photoluminescence quantum yield close to unity. We show that the lifetime of the spontaneous radiative recombination in PNCs is as short as 2 ns, which is expected considering the direct bandgap character of perovskit…
Different temperature renormalizations for heavy and light-hole states of monolayer-thick heterostructures
2000
Abstract We have found that the energy splitting between peaks in the linearly polarized emission from the cleaved surface of an InAs/GaAs monolayer structure triples with increasing temperature in the range from 5 to 150 K. For each polarization the main emission line corresponds to the radiative recombination of either heavy or light-hole excitons bound to the monolayer. The striking temperature behavior of the peak energies originates from the different hole–phonon coupling due to the much larger penetration of the light-hole envelope function into the GaAs. We prove this assertion by confining the light holes to the InAs plane with a strong magnetic field, which leads to a reduction of …