Search results for "surface plasmon"
showing 10 items of 393 documents
Coupling of a dipolar emitter into one-dimensional surface plasmon.
2013
Quantum plasmonics relies on a new paradigm for light-matter interaction. It benefits from strong confinement of surface plasmon polaritons (SPP) that ensures efficient coupling at a deep subwavelength scale, instead of working with a long lifetime cavity polariton that increases the duration of interaction. The large bandwidth and the strong confinement of one dimensional SPP enable controlled manipulation of a nearby quantum emitter. This paves the way to ultrafast nanooptical devices. However, the large SPP bandwidth originates from strong losses so that a clear understanding of the coupling process is needed. In this report, we investigate in details the coupling between a single emitte…
Nonlinear plasmonic amplification via dissipative soliton-plasmon resonances
2017
In this contribution we introduce a new strategy for the compensation of plasmonic losses based on a recently proposed nonlinear mechanism: the resonant interaction between surface plasmon polaritons and spatial solitons propagating in parallel along a metal/dielectric/Kerr structure. This mechanism naturally leads to the generation of a quasi-particle excitation, the so-called soliplasmon resonance. We analyze the role played by the effective nonlinear coupling inherent to this system and how this can be used to provide a new mechanism of quasi-resonant nonlinear excitation of surface plasmon polaritons. We will pay particular attention to the introduction of asymmetric linear gain in the …
Variational theory of soliplasmon resonances
2013
We present a first-principles derivation of the variational equations describing the dynamics of the interaction of a spatial soliton and a surface plasmon polariton (SPP) propagating along a metal/dielectric interface. The variational ansatz is based on the existence of solutions exhibiting differentiated and spatially resolvable localized soliton and SPP components. These states, referred to as soliplasmons, can be physically understood as bound states of a soliton and a SPP. Their respective dispersion relations permit the existence of a resonant interaction between them, as pointed out in Ref.[1]. The existence of soliplasmon states and their interesting nonlinear resonant behavior has …
Soliton-plasmon resonances as Maxwell nonlinear bound states
2012
We demonstrate that soliplasmons (soliton–plasmon bound states) appear naturally as eigenmodes of nonlinear Maxwell’s equations for a metal/Kerr interface. Conservative stability analysis is performed by means of finite element numerical modeling of the time-independent nonlinear Maxwell equations. Dynamical features are in agreement with the presented nonlinear oscillator model.
Plasmonic Focusing Reduces Ensemble Linewidth
2012
In this chapter I present an effect the coating of gold nanorods with a silver shell is evocating: a reduction of the ensemble plasmon linewidth by changing the plasmon-shape relation, which connects the particle shape with its plasmon resonance wavelength. This change, we term “plasmonic focusing” (Sect. 10.2), leads to less variation of resonance wavelengths for the same particle size distribution. Section 10.3 explains the effect of increasing single particle linewidth during the coating process, which is therefore not the reason for the observed ensemble linewidth decrease. This is rather a result from a change in the plasmon-shape relation explained in Sect. 10.4. Using a simple model,…
Photon bunching of the nonlinear photoluminescence emitted by plasmonics metals
2021
International audience; In this report, we investigate the statistical temporal distribution of nonlinear upconverted photoluminescence emitted by gold and silver nanostructures excited by focused near-infrared laser pulses. We systematically observe a clear signature of photon bunching regardless of the nano-object's geometry, material's crystalline arrangement, and electronic band structure. The similarity of the data obtained across very different plasmonic objects confirms that these types of nonlinear radiation share a common chaotic origin and result from a collection of emitters. The correlation of photons at a picosecond time scale released by nanoscale nonlinear sources of broadban…
Surface Plasmons for Chiral Sensing
2021
Chiral sensitive techniques have been used to probe the fundamental symmetries of the universe, study biomolecular structures, and even develop safe drugs. The traditional method for the measurement of chirality is through optical activity, however, chiroptical signals are inherently weak and often suppressed by large backgrounds. Different techniques have been proposed to overcome the limitations of traditionally used optical polarimetry, such as cavity- and/or nanophotonic-based schemes. In this chapter we demonstrate how surface plasmon resonance can be employed as a new research tool for chiral sensing, which we term here as CHIral Surface Plasmon Resonance (CHISPR). We present how surf…
Momentum-space spectroscopy for advanced analysis of dielectric-loaded surface plasmon polariton coupled and bent waveguides
2013
We perform advanced radiation leakage microscopy of routing dielectric-loaded plasmonic waveguiding structures. By direct plane imaging and momentum-space spectroscopy, we analyze the energy transfer between coupled waveguides as a function of gap distance and reveal the momentum distribution of curved geometries. Specifically, we observed a clear degeneracy lift of the effective indices for strongly interacting waveguides in agreement with coupled-mode theory. We use momentum-space representations to discuss the effect of curvature on dielectric-loaded waveguides. The experimental images are successfully reproduced by a numerical and an analytical model of the mode propagating in a curved …
Delocalization of Nonlinear Optical Responses in Plasmonic Nanoantennas
2015
Remote excitation and emission of two-photon luminescence and second-harmonic generation are observed in micrometer long gold rod optical antennas upon local illumination with a tightly focused near-infrared femtosecond laser beam. We show that the nonlinear radiations can be emitted from the entire antenna and the measured far-field angular patterns bear the information regarding the nature and origins of the respective nonlinear processes. We demonstrate that the nonlinear responses are transported by the propagating surface plasmon at excitation frequency, enabling thereby polariton-mediated tailoring and design of nonlinear responses.
Designed surface modes propagating along hyperbolic metamaterials
2013
We report on surface-wave propagation (SWP) that occurs in semi-infinite hyperbolic metamaterials whose optical axis is set in the interface plane. In practice it is implemented by a multi-layered metal-dielectric nanostructure that is cut normally to the layers. Our theoretical analysis shows that various conditions can be designed enabling distinct regimes of SWP. We concluded that hybridization of SWP polarization leads to tighter confinement near the interface as compared with conventional surface plasmon polaritons. By using the finite-element method (FEM), we demonstrate that the fields are enhanced on the walls of metallic films, and thus minimizing significantly its presence inside …