Search results for "ta114"
showing 10 items of 1144 documents
Characterization of a cryogenic ion guide at IGISOL
2012
A small volume cryogenic ion guide has been characterized at the IGISOL facility, Jyvaskyla, as a prototype to verify whether there are any major obstacles to the use of high-density cryogenic helium gas for the stopping and extraction of high-energy ions from a large volume cryogenic ion catcher. The expected temperature scaling of the mass flow through the ion guide has been confirmed, showing that for the same helium density, the differential pumping requirements are less stringent for cryogenic operation. At 90 K a clear reduction in the mass-analyzed impurities is achieved, although lower temperatures are required to freeze out oxygen and nitrogen. This is supported by the reduction in…
Site-specific targeting of enterovirus capsid by functionalized monodisperse gold nanoclusters
2014
Development of precise protocols for accurate site-specific conjugation of monodisperse inorganic nanoparticles to biological material is one of the challenges in contemporary bionanoscience and nanomedicine. We report here a successful site-specific covalent conjugation of functionalized atomically monodisperse gold clusters with 1.5-nm metal cores to viral surfaces. Water-soluble Au102(para-mercaptobenzoic acid)44 clusters, functionalized by maleimide linkers to target cysteines of viral capsid proteins, were synthesized and conjugated to enteroviruses echovirus 1 and coxsackievirus B3. Quantitative analysis of transmission electron microscopy images and the known virus structures showed …
Communication modes in vector diffraction
2010
The communication modes, which mathematically correspond to singular value decomposition, have proven a useful concept in optical scalar-field diffraction, with applications in resolution studies, image synthesis, and wave propagation. For optical near-field geometries the communication modes have to be extended to electromagnetic field accounting for the polarization properties. In this paper we present the vector-valued communication modes method based on the rigorous electric-field diffraction integral. As a special case the transverse-electric scalar field modes are obtained. The intensity and polarization properties of the leading electromagnetic communication modes in near-field arran…
Stimulated quasiparticles in spin-split superconductors
2015
Under the terms of the Creative Commons Attribution License 3.0 (CC-BY).
Synthetic electromagnetic knot in a three-dimensional skyrmion
2018
We experimentally simulate a quantum-mechanical particle interacting with knotted electromagnetic fields.
Time-dependent Kohn-Sham approach to quantum electrodynamics
2010
We prove a generalization of the van Leeuwen theorem towards quantum electrodynamics, providing the formal foundations of a time-dependent Kohn-Sham construction for coupled quantized matter and electromagnetic fields. Thereby we circumvent the symmetry-causality problems associated with the action-functional approach to Kohn-Sham systems. We show that the effective external four-potential and four-current of the Kohn-Sham system are uniquely defined and that the effective four-current takes a very simple form. Further we rederive the Runge-Gross theorem for quantum electrodynamics.
Ultra-nonlocality in density functional theory for photo-emission spectroscopy.
2014
We derive an exact expression for the photo-current of photo-emission spectroscopy using time-dependent current density functional theory (TDCDFT). This expression is given as an integral over the Kohn-Sham spectral function renormalized by effective potentials that depend on the exchange-correlation kernel of current density functional theory. We analyze in detail the physical content of this expression by making a connection between the density-functional expression and the diagrammatic expansion of the photo-current within many-body perturbation theory. We further demonstrate that the density functional expression does not provide us with information on the kinetic energy distribution of…
Hidden Structural Features of Multicompartment Micelles Revealed by Cryogenic Transmission Electron Tomography
2014
The demand for ever more complex nanostructures in materials and soft matter nanoscience also requires sophisticated characterization tools for reliable visualization and interpretation of internal morphological features. Here, we address both aspects and present synthetic concepts for the compartmentalization of nanoparticle peripheries as well as their in situ tomographic characterization. We first form negatively charged spherical multicompartment micelles from ampholytic triblock terpolymers in aqueous media, followed by interpolyelectrolyte complex (IPEC) formation of the anionic corona with bis-hydrophilic cationic/neutral diblock copolymers. At a 1:1 stoichiometric ratio of anionic a…
Gigahertz Single-Electron Pumping Mediated by Parasitic States
2018
In quantum metrology, semiconductor single-electron pumps are used to generate accurate electric currents with the ultimate goal of implementing the emerging quantum standard of the ampere. Pumps based on electrostatically defined tunable quantum dots (QDs) have thus far shown the most promising performance in combining fast and accurate charge transfer. However, at frequencies exceeding approximately 1 GHz, the accuracy typically decreases. Recently, hybrid pumps based on QDs coupled to trap states have led to increased transfer rates due to tighter electrostatic confinement. Here, we operate a hybrid electron pump in silicon obtained by coupling a QD to multiple parasitic states, and achi…
Towards saturation of the electron-capture delayed fission probability: The new isotopes $^{240}Es$ and $^{236}Bk$
2016
Abstract The new neutron-deficient nuclei 240 Es and 236 Bk were synthesised at the gas-filled recoil separator RITU. They were identified by their radioactive decay chains starting from 240 Es produced in the fusion–evaporation reaction 209 Bi( 34 S,3n) 240 Es. Half-lives of 6 ( 2 ) s and 22 − 6 + 13 s were obtained for 240 Es and 236 Bk, respectively. Two groups of α particles with energies E α = 8.19 ( 3 ) MeV and 8.09 ( 3 ) MeV were unambiguously assigned to 240 Es. Electron-capture delayed fission branches with probabilities of 0.16 ( 6 ) and 0.04 ( 2 ) were measured for 240 Es and 236 Bk, respectively. These new data show a continuation of the exponential increase of ECDF probabilitie…