Search results for "terahertz"

Implementation of signal-processing functionalities in the Terahertz frequency domain

2020

Gas-phase detection of HSOD and empirical equilibrium structure of oxadisulfane

2006

We present the first gas phase spectra of singly deuterated oxadisulfane, HSOD, in its vibrational ground state. More than 100 transitions have been recorded with highest frequency accuracy using the Cologne Terahertz Spectrometer. The molecular parameters derived from a least squares fit analysis proof HSOD to be an almost accidental symmetric prolate top molecule with an asymmetry parameter kZK0.9985. Spectra of c-type and weaker b-type transitions have been recorded in the range from 716 to 772 GHz. The ratio of the dipole moments mc/mbZ2.4(3) has been derived from measured line intensities. The c-type transitions are split by the tunneling motion of a hindered internal rotation, whereas…

Room temperature antiferromagnetic resonance and inverse spin-Hall voltage in canted antiferromagnets

2021

We study theoretically and experimentally the spin pumping signals induced by the resonance of canted antiferromagnets with Dzyaloshinskii-Moriya interaction and demonstrate that they can generate easily observable inverse spin-Hall voltages. Using a bilayer of hematite/heavy metal as a model system, we measure at room temperature the antiferromagnetic resonance and an associated inverse spin-Hall voltage, as large as in collinear antiferromagnets. As expected for coherent spin pumping, we observe that the sign of the inverse spin-Hall voltage provides direct information about the mode handedness as deduced by comparing hematite, chromium oxide and the ferrimagnet yttrium-iron garnet. Our r…

Resolving the Fundamentals of Magnetotransport in Metals with Ultrafast Terahertz Spectroscopy

2016

Using terahertz spectroscopy we directly resolved the fundamentals of spin-dependent conductivity in ferromagnetic metals. We quantified the differences in conduction by Fermi-level electrons with opposite spins on the sub-100 fs timescale of electron momentum scattering.

High gain/bandwidth off-chip antenna loaded with metamaterial unit-cell impedance matching circuit for sub-terahertz near-field electronic systems

2022

An innovative of-chip antenna (OCA) is presented that exhibits high gain and efciency performance at the terahertz (THz) band and has a wide operational bandwidth. The proposed OCA is implemented on stacked silicon layers and consists of an open circuit meandering line. It is shown that by loading the antenna with an array of subwavelength circular dielectric slots and terminating it with a metamaterial unit cell, its impedance bandwidth is enhanced by a factor of two and its gain on average by about 4 dB. Unlike conventional antennas, where the energy is dissipated in a resistive load, the technique proposed here signifcantly reduces losses. The antenna is excited from underneath the anten…

Bottom-Up, On-Surface-Synthesized Armchair Graphene Nanoribbons for Ultra-High-Power Micro-Supercapacitors

2020

Bottom-up-synthesized graphene nanoribbons (GNRs) with excellent electronic properties are promising materials for energy storage systems. Herein, we report bottom-up-synthesized GNR films employed as electrode materials for micro-supercapacitors (MSCs). The micro-device delivers an excellent volumetric capacitance and an ultra-high power density. The electrochemical performance of MSCs could be correlated with the charge carrier mobility within the differently employed GNRs, as determined by pump–probe terahertz spectroscopy studies.

Possible light-induced superconductivity in K3C60 at high temperature.

2015

The non-equilibrium control of emergent phenomena in solids is an important research frontier, encompassing effects such as the optical enhancement of superconductivity. Nonlinear excitation of certain phonons in bilayer copper oxides was recently shown to induce superconducting-like optical properties at temperatures far greater than the superconducting transition temperature, Tc. This effect was accompanied by the disruption of competing charge-density-wave correlations, which explained some but not all of the experimental results. Here we report a similar phenomenon in a very different compound, K3C60. By exciting metallic K3C60 with mid-infrared optical pulses, we induce a large increas…

Light-induced superconductivity

2016

Intense light pulses irradiating a sample of K3C60 result in dramatic changes of its high-frequency (terahertz) conductivity. Could these be signatures of fleeting superconductivity at 100 K and beyond?

Counter-propagating frequency mixing with Terahertz waves in diamond

2013

Frequency conversion by means of Kerr nonlinearity is one of the most common and exploited nonlinear optical processes in the UV, visible, IR, and mid-IR spectral regions. Here we show that wave mixing of an optical field and a terahertz wave can be achieved in diamond, resulting in the frequency conversion of the terahertz radiation either by sum- or difference-frequency generation. In the latter case, we show that this process is phase matched and most efficient in a counterpropagating geometry.

Terahertz Time-Domain Spectroscopy setup based on photoconductive antennas

2016

Despite the technical difficulties in developing efficient and compact sources and detectors for Terahertz (THz) radiation, this region of the electromagnetic spectrum is attracting an ever-increasing interest, due to its peculiar and high-potential applications in several fields, such as wideband communications, medicine, biology, non-destructive testing, security and defense. Within such contexts, the most widespread approach aiming to deal with THz pulses is based on the THz Time-Domain Spectroscopy (THz-TDS) system. In this work, we present our experimental results obtained by means of a THz-TDS set-up based on photoconductive antennas for both the generation and detection stage. It is …