6533b855fe1ef96bd12aff13

RESEARCH PRODUCT

Possible light-induced superconductivity in K3C60 at high temperature.

Andrea CavalleriMatteo MitranoA. CantaluppiDieter JakschP. Di PietroStefan KaiserM. RiccòAndrea PerucchiDaniele PontiroliStephen R. ClarkDaniele NicolettiStefano Lupi

subject

SuperconductivityElectron mobilityMultidisciplinaryMaterials scienceCondensed matter physicsPhononTerahertz radiationBilayerPhotoconductivity02 engineering and technology021001 nanoscience & nanotechnology01 natural sciencesOptical conductivityArticleCondensed Matter::Superconductivity0103 physical sciencesCuprate010306 general physics0210 nano-technology

description

The non-equilibrium control of emergent phenomena in solids is an important research frontier, encompassing effects such as the optical enhancement of superconductivity. Nonlinear excitation of certain phonons in bilayer copper oxides was recently shown to induce superconducting-like optical properties at temperatures far greater than the superconducting transition temperature, Tc. This effect was accompanied by the disruption of competing charge-density-wave correlations, which explained some but not all of the experimental results. Here we report a similar phenomenon in a very different compound, K3C60. By exciting metallic K3C60 with mid-infrared optical pulses, we induce a large increase in carrier mobility, accompanied by the opening of a gap in the optical conductivity. These same signatures are observed at equilibrium when cooling metallic K3C60 below Tc (20 kelvin). Although optical techniques alone cannot unequivocally identify non-equilibrium high-temperature superconductivity, we propose this as a possible explanation of our results.

10.1038/nature16522https://pubmed.ncbi.nlm.nih.gov/26855424