Gamma-ray spectroscopy of191,193Bi

Very neutron-deficient Bi-191,Bi-193 nuclei have been studied at the Department of Physics, University of Jyvaskyla, Finland (JYFL) employing the Jurosphere II Ge-detector array coupled to the gas-filled recoil separator RITU and different tagging techniques. For the first time in heavy odd-mass nuclei, a collective band (oblate) is identified above the 2p-1h (1/2(+)) proton intruder state in Bi-191. In both Bi-191,Bi-193, a band based on isomeric 13/2(+) state has been observed and oblate deformation for this state has been deduced. ispartof: Acta Physica Polonica B vol:32 issue:3 pages:1019-1023 ispartof: location:POLAND, ZAKOPANE status: published

Backbending in the pear-shaped 223(90)Th nucleus: Evidence of a high-spin octupole to quadrupole shape transition in the actinides

International audience; Relatively neutron-rich thorium isotopes lie at the heart of a nuclear region of nuclei exhibiting octupole correlation effects. The detailed level structure of Th223 has been investigated in measurements of γ radiation following the fusion-evaporation channel of the Pb208(O18,3n)Th223 reaction at 85 MeV beam energy. The level structure has been extended up to spin 49/2, and 33 new γ rays have been added using triple-γ coincidence data. The spins and parities of the newly observed states have been confirmed by angular distribution ratios. In addition to the two known yrast bands based on a K=5/2 configuration, a non-yrast band has been established up to spin 35/2. We…

Spectroscopy of low-spin states in $^{157}\mathrm{Dy}$: Search for evidence of enhanced octupole correlations

Low-spin states of 157Dy have been studied using the JUROGAM II array, following the 155Gd ({\alpha}, 2n) reaction at a beam energy of 25 MeV. The level scheme of 157Dy has been expanded with four new bands. Rotational structures built on the [523]5/2- and [402]3/2+ neutron orbitals constitute new additions to the level scheme as do many of the inter- and intra-band transitions. This manuscript also reports the observation of cross I- to (I-1)- and I- to (I-1)+ E1 dipole transitions inter-linking structures built on the [523]5/2- (band 5) and [402]3/2+ (band 7) neutron orbitals. These interlacing band structures are interpreted as the bands of parity doublets with simplex quantum number s =…

First observation of high-K isomeric states in $$^{249}$$Md and $$^{251}$$Md

Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-K isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of 2.8(5) ms and an excitation energy $\ge 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of 1.4(3) s and an excitation energy $\ge 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-K states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nucle…

First candidates for γ vibrational bands built on the [505]11/2⁻ neutron orbital in odd-A Dy isotopes

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd(α,2n)157Dy and 148Nd(12C,5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ=2+γ vibrational band, built on the [505]11/2− neutron orbital, in both odd-A155,157Dy isotopes. The coupling of the first excited K=0+ states or the so-called β vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2− orbital, to produce a Kπ=11/2− band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the cor…

In-beam gamma-ray and electron spectroscopy of $^{249,251}$Md

The odd-Z Md251 nucleus was studied using combined γ-ray and conversion-electron in-beam spectroscopy. Besides the previously observed rotational band based on the [521]1/2− configuration, another rotational structure has been identified using γ-γ coincidences. The use of electron spectroscopy allowed the rotational bands to be observed over a larger rotational frequency range. Using the transition intensities that depend on the gyromagnetic factor, a [514]7/2− single-particle configuration has been inferred for this band, i.e., the ground-state band. A physical background that dominates the electron spectrum with an intensity of ≃60% was well reproduced by simulating a set of unresolved ex…

A Recoil-Beta Tagging Study of N = Z nucleus [sup 66]As

A Recoil‐Beta Tagging (RBT) experiment was recently performed at the accelerator laboratory at the University of Jyvaskyla in order to identify T = 1 excited states in the medium‐heavy N = Z = 33 nucleus 66As. The fusion‐evaporation reaction 28Si(40Ca,pn)66As was employed at a beam energy of 75 MeV. The experiment was carried out utilising the JUROGAM II γ‐ray spectrometer in conjunction with the gas‐filled recoil separator RITU and the GREAT focal plane spectrometer system. The half‐lives and ordering of the two known isomeric states in 66As have been determined. In addition, several new prompt γ‐ray transitions from excited states both bypassing and decaying to the isomeric states in 66As…

Characterizing the atomic mass surface beyond the proton drip line via a-decay measurements of the s1/2 ground state of 165Re and the h11/2 isomer in 161Ta

The a-decay chains originating from the s1/2 and h11/2 states in 173Au have been investigated following fusion-evaporation reactions. Four generations of a radioactivities have been correlated with 173Aum leading to a measurement of the a decay of 161Tam. It has been found that the known a decay of 161Ta, which was previously associated with the decay of the ground state, is in fact the decay of an isomeric state. This work also reports on the first observation of prompt g rays feeding the ground state of 173Au. This prompt radiation was used to aid the study of the a-decay chain originating from the s1/2 state in 173Au. Three generations of a decays have been correlated with this state lea…

Shell-Structure and Pairing Interaction in Superheavy Nuclei: Rotational Properties of the Z=104 Nucleus (256)Rf

The rotational band structure of the Z ¼ 104 nucleus 256Rf has been observed up to a tentative spin of 20@ using state-of-the-art -ray spectroscopic techniques. This represents the first such measurement in a superheavy nucleus whose stability is entirely derived from the shell-correction energy. The observed rotational properties are compared to those of neighboring nuclei and it is shown that the kinematic and dynamic moments of inertia are sensitive to the underlying single-particle shell structure and the specific location of high-j orbitals. The moments of inertia therefore provide a sensitive test of shell structure and pairing in superheavy nuclei which is essential to ensure the val…

Coulomb excitation of $^{78}$Kr

Expérience à JYFL cyclotron (Jyväskylä, Finlande); The Kr isotopes are considered to be among the best cases for shape coexistence studies in the mass A$\sim$70 region. Our campaign to investigate in detail the development of the shape coexistence in the neutron deficient Kr isotopes was started with the stable nucleus $^{78}$Kr. To obtain the information about the intrinsic shape, Coulomb excitation experiments were performed. A total of 26 matrix elements were determined for $^{78)$Kr. Simple geometrical and algebraic models do not reproduce all details of the electromagnetic structure. A good interpretation of the complex structure of the nucleus with competing oblate and prolate shapes …

First candidates for $\gamma$ vibrational bands built on the $[505]11/{2}^{-}$ neutron orbital in odd-$A$ Dy isotopes

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the 155Gd({\alpha},2n)157Dy and 148Nd(12C, 5n)155Dy reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a K{\pi}= 2+ {\gamma} vibrational band, built on the [505]11/2- neutron orbital, in both odd-A 155, 157Dy isotopes. The coupling of the first excited K=0+ states or the so-called \b{eta} vibrational bands at 661 and 676 keV in 154Dy and 156Dy to the [505]11/2- orbital, to produce a K{\pi}=11/2- band, was not observed in both 155Dy and 157Dy, respectively. The implication of these findings on the interpretation of the f…

Shape coexistence in neutron-deficient Hg isotopes studied via lifetime measurements in 184,186Hg and two-state mixing calculations

The neutron-deficient mercury isotopes, $^{184,186}$Hg, were studied with the Recoil Distance Doppler Shift (RDDS) method using the Gammasphere array and the K\"oln Plunger device. The Differential Decay Curve Method (DDCM) was employed to determine the lifetimes of the yrast states in $^{184,186}$Hg. An improvement on previously measured values of yrast states up to $8^{+}$ is presented as well as first values for the $9_{3}$ state in $^{184}$Hg and $10^{+}$ state in $^{186}$Hg. $B(E2)$ values are calculated and compared to a two-state mixing model which utilizes the variable moment of inertia (VMI) model, allowing for extraction of spin-dependent mixing strengths and amplitudes.

Production cross section and decay study of $^{243}$Es and $^{249}$Md

In the study of the odd-$Z$, even-$N$ nuclei $^{243}$Es and $^{249}$Md, performed at the University of Jyv\"askyl\"a, the fusion-evaporation reactions $^{197}$Au($^{48}$Ca,2$n$)$^{243}$Es and $^{203}$Tl($^{48}$Ca,2$n$)$^{249}$Md have been used for the first time. Fusion-evaporation residues were selected and detected using the RITU gas-filled separator coupled with the focal-plane spectrometer GREAT. For $^{243}$Es, the recoil decay correlation analysis yielded a half-life of $24 \pm 3$s, and a maximum production cross section of $37 \pm 10$ nb. In the same way, a half-life of $26 \pm 1$ s, an $\alpha$ branching ratio of 75 $\pm$ 5%, and a maximum production cross section of 300 $\pm$ 80 nb…

Recoil-isomer tagging techniques at RITU

Techniques have been developed to study isomeric states in nuclei with the use of RITU (gas filled separator) at the University of Jyvaskyla. The first was the recoil-isomer tagging technique initially, utilised by D.M. Cullen to study the K π = 8− isomeric state in 138Gd [1]. The juro-sphere array was employed in conjunction with ritu and a focal plane array which consisted of several Compton-suppressed Germanium detectors, placed in close geometry around a multi wire proportional counter (mwpc) and a silicon strip detector used for the implantation of recoiling nuclei. This technique correlates prompt and delayed γ-ray transitions across isomeric states and identifies the lifetime of the …

Shape coexistence at the proton drip-line: First identification of excited states in 180Pb

Excited states in the extremely neutron-deficient nucleus, 180Pb, have been identified for the first time using the JUROGAM II array in conjunction with the RITU recoil separator at the Accelerator Laboratory of the University of Jyvaskyla. This study lies at the limit of what is presently achievable with in-beam spectroscopy, with an estimated cross-section of only 10 nb for the 92Mo(90Zr,2n)180Pb reaction. A continuation of the trend observed in 182Pb and 184Pb is seen, where the prolate minimum continues to rise beyond the N=104 mid-shell with respect to the spherical ground state. Beyond mean-field calculations are in reasonable correspondence with the trends deduced from experiment.

Multi-point galactic cosmic ray measurements between 1 and 4.5 AU over a full solar cycle

The radiation data collected by the Standard Radiation Environment Monitor (SREM) aboard ESA missions INTEGRAL (INTErnational Gamma-Ray Astrophysics Laboratory), Rosetta, Herschel, Planck and Proba-1, and by the high-energy neutron detector (HEND) instrument aboard Mars Odyssey, are analysed with an emphasis on characterising galactic cosmic rays (GCRs) in the inner heliosphere. A cross calibration between all sensors was performed for this study, which can also be used in subsequent works. We investigate the stability of the SREM detectors over long-term periods. The radiation data are compared qualitatively and quantitatively with the corresponding solar activity. Based on INTEGRAL and Ro…

Observation ofK=1/2octupole deformed bands in227Th

High-spin states in 227Th have been populated using the reaction 226Ra(α,3n)227Th at a bombarding energy of 33 MeV. The high-spin rotational structures of this nucleus have been refined and extended. In addition, the linking of these structures with the low-spin states known from 231U α decay has allowed a comprehensive decay scheme of this nucleus to be assembled for the first time. Four previously known rotational bands are interpreted as Coriolis coupled Kπ=1/2+ and Kπ=1/2− bands, in agreement with predictions using a reflection-asymmetric mean field approach. The determination of decoupling parameters for these bands is consistent with the a(Kπ=1/2+)=−a(Kπ=1/2−) rigid octupole rotor exp…

Alpha decay studies of translead nuclei at the proton drip line

Extensive α-decay studies of the very neutron deficient isotopes 191Po, 195Rn, and 196Rn have been performed at the RITU gas-filled recoil separator. The recoil-α–(α) correlation technique and the α–γ coincidence technique have been utilized to unambiguously connect the observed α-decays to proper nuclei. Illustrative examples on how the α-decay can yield spectroscopic information on the nuclei studied will be presented. peerReviewed

Shape coexistence in183Tl

Recoil Isomer Tagging on Proton-Rich Odd–Odd N=77 Isotones 142Tb and 144Ho

The isomeric structure of the N=77 isotones 14265Tb and 14467Ho have been studied with the 92Mo(54Fe, xpn) fusion evaporation reaction at the University of Jyväskylä. The Jurospehere II germanium array was employed in conjunction with the RITU gas filled recoil separator. The feeding and decay of a 500(20) ns isomeric state in 144Ho has been established for the first time together with states built upon the known 15 μs isomer in 142Tb. The behavior of these new structures above the isomers suggest that they are low deformation configurations which display signs of triaxiality. peerReviewed

Probing structures of exotic heavy nuclei

The JYFL gas-filled recoil separator RITU, combined with Ge detector arrays, has successfully been employed in Recoil-Decay-Tagging (RDT) experiments in order to probe, for the first time, structures of several very neutron deficient heavy nuclei. In this contribution new data for light even-mass Hg, Pb and Po nuclei are shown and discussed. peerReviewed

High K bands in mid-supershell nuclei

The spectrum of prompt conversion electrons emitted by excited 254No nuclei has been measured, revealing discrete lines arising from transitions within the ground state band. A striking feature is a broad distribution that peaks near 100 keV and comprises high multiplicity electron cascades, probably originating from M1 transitions within rotational bands built on high K states. Evidence for the existence of isomeric states in 254No is presented. peerReviewed

In-beam γ-ray and electron spectroscopy of Md249,251

The odd-Z 251Md nucleus was studied using combined γ-ray and conversion-electron in-beam spectroscopy. Besides the previously observed rotational band based on the [521]1/2− configuration, another rotational structure has been identified using γ−γ coincidences. The use of electron spectroscopy allowed the rotational bands to be observed over a larger rotational frequency range. Using the transition intensities that depend on the gyromagnetic factor, a [514]7/2− single-particle configuration has been inferred for this band, i.e., the ground-state band. A physical background that dominates the electron spectrum with an intensity of ≃60% was well reproduced by simulating a set of unresolved ex…

Studies of 225,226U alpha decay chains

Studies of 225,226U α -decay chains produced via heavy ion induced fusion reactions of 22Ne + 208Pb → 230U and of 18O + 208Pb → 226Th were carried out using the JYFL gas-filled magnetic recoil separator RITU. The data obtained for α -decays of 225,226U, 221,222Th, 218Ra and 213Rn concerning their α -particle energies, half-lives and α -decay fine structures are compared to previous investigations. peerReviewed

Sex differences in renal damage induced in the mouse by Amanita virosa.

Summary The sensitivity of male and female mice to Amanita virosa was compared. Dried, homogenizedmushroom was given orally by stomach tubing at doses of 100, 200, 400 and 800 mg dried mushroom/kg body weight. Both in males and in females, the kidneys were the only organs showing macroscopical changes. The dose of 100 mg/kg caused renal damage in females, whereas in males the first signs of kidney damage were seen at the dose of 400 mg/kg. The renal lesions observed in the males were located in the cortex, while in the females they were limited to the outer stripe of the outer medullary zone. Testectomy diminished the nephrotoxicity of A. virosa in male mice and caused changes in the locali…

Investigation of 246Fm : in-beam spectroscopy at the limits\u2028

Identification of isomeric states in the N=73 neutron-deficient nuclei 132Pr and 130La

Decays from isomeric states in the neutron-deficient N=73 nuclei 132Pr and 130La have been observed for the first time. Half-lives of 486(70) ns and 2.46(4) μs were measured for two isomeric states in 132Pr. The decay from the 486ns (8 -) isomer has been interpreted as a hindered E1 transition from the bandhead state of the excited πh 11/2νg 7/2 configuration. The decay from the 2.5 μs (8 +) isomer is consistent with the Weisskopf estimate for a low-energy E2 transition. An analogous 0.74(3) μs decay from an (8 +) isomer in the neighboring isotone 130La has also been observed which similarly can be explained if the transition has E2 character. The Weisskopf interpretation for the isomer hin…

High-spin intruder band in $^{107}$In

High-spin states in the neutron deficient nucleus $^{107}$In were studied via the $^{58}$Ni($^{52}$Cr, 3p) reaction. In-beam $\gamma$ rays were measured using the JUROGAM detector array. A rotational cascade consisting of ten $\gamma$-ray transitions which decays to the 19/2$^{+}$ level at 2.002 MeV was observed. The band exhibits the features typical for smooth terminating bands which also appear in rotational bands of heavier nuclei in the A$\sim$100 region. The results are compared with Total Routhian Surface and Cranked Nilsson-Strutinsky calculations.

Delayed or absent π(h11/2)2 alignment in 111Xe

Excited states have been identified in the very neutron-deficient N = Z + 3 nucleus 111Xe for the first time, using the 58Ni(58Ni, αn) heavy-ion fusion-evaporation reaction. γ -ray transitions have been unambiguously assigned to 111Xe by correlation with the characteristic 111Xe → 107Te → 103Sn α-decay chain using the method of recoil-decay tagging. Inspection of γ γ -coincidence data has shown that five of the transitions form a rotational-like sequence. Excitation-energy systematics suggest that the sequence could be the favored signature partner of a band built on an h11/2 neutron. Aligned angular momenta of states in the band have been compared to analogous bands in neighboring xenon is…

The influence of quasineutron configurations on 161Ta and nearby odd-A Nuclei

Several strongly coupled bands in the neutron‐deficient nucleus 161Ta have been identified and quasiparticle configuration assignments have been made on the basis of rotational alignments and cranked shell model calculations. The level scheme elucidated for 161Ta highlights the competition between the ν(h9/2) and ν(i13/2) orbitals to form the yrast spectrum. The band structures in 161Ta also provide new insights into the structural features of other heavy odd‐A nuclei populated with much lower reaction cross sections in this region at the proton drip line.