0000000000004274
AUTHOR
Stefan Trotzky
Time-resolved Observation and Control of Superexchange Interactions with Ultracold Atoms in Optical Lattices
Quantum mechanical superexchange interactions form the basis of quantum magnetism in strongly correlated electronic media. We report on the direct measurement of superexchange interactions with ultracold atoms in optical lattices. After preparing a spin-mixture of ultracold atoms in an antiferromagnetically ordered state, we measure a coherent superexchange-mediated spin dynamics with coupling energies from 5 Hz up to 1 kHz. By dynamically modifying the potential bias between neighboring lattice sites, the magnitude and sign of the superexchange interaction can be controlled, thus allowing the system to be switched between antiferromagnetic or ferromagnetic spin interactions. We compare our…
Counting atoms using interaction blockade in an optical superlattice.
We report on the observation of an interaction blockade effect for ultracold atoms in optical lattices, analogous to Coulomb blockade observed in mesoscopic solid state systems. When the lattice sites are converted into biased double wells, we detect a discrete set of steps in the well population for increasing bias potentials. These correspond to tunneling resonances where the atom number on each side of the barrier changes one by one. This allows us to count and control the number of atoms within a given well. By evaluating the amplitude of the different plateaus, we can fully determine the number distribution of the atoms in the lattice, which we demonstrate for the case of a superfluid …
Electromagnetically Induced Transparency and Light Storage in an Atomic Mott Insulator
We experimentally demonstrate electromagnetically induced transparency and light storage with ultracold 87Rb atoms in a Mott insulating state in a three dimensional optical lattice. We have observed light storage times of about 240 ms, to our knowledge the longest ever achieved in ultracold atomic samples. Using the differential light shift caused by a spatially inhomogeneous far detuned light field we imprint a "phase gradient" across the atomic sample, resulting in controlled angular redirection of the retrieved light pulse.
Direct observation of second-order atom tunnelling
Tunnelling of material particles through a classically impenetrable barrier constitutes one of the hallmark effects of quantum physics. When interactions between the particles compete with their mobility through a tunnel junction, intriguing novel dynamical behaviour can arise where particles do not tunnel independently. In single-electron or Bloch transistors, for example, the tunnelling of an electron or Cooper pair can be enabled or suppressed by the presence of a second charge carrier due to Coulomb blockade. Here we report on the first direct and time-resolved observation of correlated tunnelling of two interacting atoms through a barrier in a double well potential. We show that for we…
Expansion of a quantum gas released from an optical lattice
We analyze the interference pattern produced by ultracold atoms released from an optical lattice. Such interference patterns are commonly interpreted as the momentum distributions of the trapped quantum gas. We show that for finite time-of-flights the resulting density distribution can, however, be significantly altered, similar to a near-field diffraction regime in optics. We illustrate our findings with a simple model and realistic quantum Monte Carlo simulations for bosonic atoms, and compare the latter to experiments.
Ligand removal from soluble CdTe nanocrystals evidenced by time-resolved photoluminescence spectroscopy
We present experimental studies on the effect of pyridine treatment on the optical properties of ligand-stabilized colloidal CdTe nanocrystals. We demonstrate, by quasi-stationary and time-resolved photoluminescence (PL) spectroscopy, a drastic reduction in the PL lifetime and a concomitant decrease in the PL yield by more than 90% when dissolving the nanocrystals in pyridine. The pyridine solvent efficiently removes the ligand shell and thus enables a rapid energy transfer from the quantum dot to optically dark surface states or into the solvent. The demonstrated removal of the ligand shell is a key step towards integrating such CdTe nanocrystals in hybrid organic/inorganic nanocomposites,…
Quantum Spin Dynamics of Mode-Squeezed Luttinger Liquids in Two-Component Atomic Gases
We report on the observation of the phase dynamics of interacting one-dimensional ultracold bosonic gases with two internal degrees of freedom. By controlling the non-linear atomic interactions close to a Feshbach resonance we are able to induce a phase diffusive many-body spin dynamics. We monitor this dynamical evolution by Ramsey interferometry, supplemented by a novel, many-body echo technique. We find that the time evolution of the system is well described by a Luttinger liquid initially prepared in a multimode squeezed state. Our approach allows us to probe the non-equilibrium evolution of one-dimensional many-body quantum systems.
Femtosecond up-conversion technique for probing the charge transfer in a P3HT : PCBM blend via photoluminescence quenching
We report on an experimental study of the charge transfer dynamics in a P3HT : PCBM blend by means of a femtosecond fluorescence up-conversion technique. Using two-photon excitation we probe the exciton dynamics in P3HT and a P3HT : PCBM blend with a weight ratio of 1 : 1 at excitation densities of up to 6 × 1018 cm−3. In both samples we find strongly nonexponential decay traces compatible with (i) diffusion-limited exciton–exciton annihilation and (ii) diffusion-limited donor–acceptor charge transfer in the polymer blend. Additionally, our results indicate that in the P3HT : PCBM blend about 50% of the photogenerated excitons undergo a prompt charge transfer process on a time scale of abou…