0000000000006409
AUTHOR
G. Ulm
Nuclear moments of strongly deformed strontium isotopes
Nuclear spins, moments and mean square charge radii of78–100Sr have been obtained by fast ion-beam collinear laserspectroscopy. The experiments performed at ISOLDE have been extended to include99Sr, measured by a non-optical detection scheme with a two-step optical pumping sequence. The results for the strongly deformed isotopes are discussed in the frame of the particle-plus-deformed core model.
Quadrupole moments of radium isotopes from the 7p 2 P 3/2 hyperfine structure in Ra II
The hyperfine structure and isotope shift of221–226Ra and212,214Ra have been measured in the ionic (Ra II) transition 7s 2 S 1/2–7p 2 P 3/2 (λ=381.4 nm). The method of on-line collinear fast-beam laser spectroscopy has been applied using frequency-doubling of cw dye laser radiation in an external ring cavity. The magnetic hyperfine fields are compared with semi-empirical and ab initio calculations. The analysis of the quadrupole splitting by the same method yields the following, improved values of spectroscopic quadrupole moments:Q s (221Ra)=1.978(7)b,Q s (223Ra)=1.254(3)b and the reanalyzed valuesQ s (209Ra)=0.40(2)b,Q s (211Ra)=0.48(2)b,Q s (227Ra)=1.58(3)b,Q s (229Ra)=3.09(4)b with an ad…
Collinear two-photon excitation of indium rydberg states in a fast atomic beam
The 29p-Rydberg state of neutral indium was produced by double resonant two-photon excitation in a fast atomic beam and detected via field ionization in a longitudinal electric field.
Nuclear orientation of radon isotopes by spin exchange optical pumping
This paper reports the first demonstration of nuclear orientation of radon atoms. The method employed was spin exchange with potassium atoms polarized by optical pumping. The radon isotopes were produced at the ISOLDE isotope separator of CERN. The nuclear alignment of /sup 209/Rn and /sup 223/Rn has been measured by observation of ..gamma..-ray anisotropies and the magnetic dipole moment for /sup 209/Rn has been measured by the nuclear-magnetic-resonance method to be chemically bond..mu..chemically bond = 0.838 81(39)..mu../sub N/.
Collinear laser spectroscopy on108g, 108m In using an ion source with bunched beam release
The hyperfine structure and isotope shift of108gIn and108mIn have been investigated by means of collinear fast-beam laser spectroscopy in the resonance line atλ=451 nm. The indium isotopes were prepared at the GSI on-line mass separator following a fusion evaporation reaction. For the first time, a FEBIAD ion source with bunched release of indium was used. Magnetic dipole moments, electric quadrupole moments and isotope shifts were determined. The present results lead us to assign the spinI=2 to the108In (T 1/2=40 min) state. Spins and moments are discussed in the framework of thejj-coupling model.
Isotope shift of182Hg and an update of nuclear moments and charge radii in the isotope range181Hg-206Hg
The technique of collinear fast-beam laser spectroscopy has been used to measure the isotope shifts of the even-even isotopes of Hg (Z=80) in the mass range 182≤A≤198 at the on-line mass separator ISOLDE at CERN. The atomic transition studied (6s 6p 3 P 2- 6s7s 3 S 1,λ=546.1 nm) starts from a metastable state, which is populated in a quasi resonant charge transfer process. The resulting changes in nuclear mean square charge radii show clearly that182Hg follows the trend of the heavier, even, weakly oblate isotopes. Correspondingly the huge odd-even shape staggering in the light Hg isotopes continues and the nuclear shape staggering and shape coexistence persists down to the last isotope inv…
Nuclear spins, moments and charge radii of108?111Sn
The hyperfine structure splittings (hfs) and isotope shifts (IS) in the atomic transitions 5s2 5p21S0 → 5s2 5p6s1,3P1 have been measured for the radioactive isotopes108−111Sn and all stable ones. The tin isotopes were prepared as fast atomic beams for collinear laser spectroscopy at the GSI online mass separator following a fusion reaction. Nuclear spins, magnetic dipole, electric quadrupole moments and changes in mean square charge radii have been determined. In109Sn the spinI=5/2 was measured for the nuclear ground state (T1/2=18 min) in contradiction to the literature value. The mean square charge radii show a parabolic behaviour with a maximum at N=66. This is interpreted by collective …
Systematics of nuclear ground state properties inSr78–100by laser spectroscopy
Hyperfine structures and isotope shifts of strontium isotopes with A=78 to A=98 and A=100 were measured by collinear fast beam laser spectroscopy. Nuclear spins, moments and changes in mean square charge radii are extracted from the data. The spins and moments of most of the odd isotopes are explained in the framework of the single particle model. The changes in mean square charge radii are compared with predictions of the droplet model and of Hartree-Fock-plus-BCS calculations. For the isotopes in the transitional regions below and above the N=50 shell closure, the inclusion of quadrupole zero point motion in the Droplet model describes part of the observed shell effect. An additional chan…
First absolute mass measurements of short-lived isotopes
Absolute mass measurements of short-lived isotopes have been performed at the on-line mass separator ISOLDE at CERN by determining the cyclotron frequencies of ions confined in a Penning trap. The cyclotron frequencies for77,78,85,86,88Rb and88Sr ions could be determined with a resolving power of 3×105 and an accuracy of better than 10−6, which corresponds to 100 keV for massA=100. The shortest-lived isotope under investigation was77Rb with a half-life of 3.7 min. The resonances obtained for the isobars88Rb and88Sr were clearly resolved.
Nuclear ground state spins of short-lived strontium isotopes
Nuclear ground state spins of the odd-mass strontium isotopes between A=79 and 97 were determined by measurements of the hyperfine structure in the ionic transition 5s2S1/2−5p2P3/2. The spins of93Sr and97Sr are revised to I=5/2 and I=1/2, respectively, while assignments for the remaining isotopes are confirmed.
Nuclear moments and charge radii of107?111in determined by laser spectroscopy
Collinear fast beam laser spectroscopy has been used to measure the hyperfine structure and isotope shift in the atomic 5s 2 5p 2 P 3/2-5s 2 6s 2 S 1/2 transition (λ=451 nm) of107–111In. Secondary beams of neutron deficient indium isotopes were prepared at the GSI on-line mass separator following fusion evaporation reactions. Magnetic dipole moments and electric quadrupole moments have been determined. The isotope shifts are discussed in terms of the change of the mean square nuclear charge radii and compared with the droplet model predictions and the deformation values calculated from the quadrupole moments.
A New Sensitive Technique for Laser Spectroscopic Studies of Radioactive Rare-Gas Isotopes
The concept of laser ionization has been widely used in spectroscopy studies and for the detection of minute samples of atoms. Being based on ion counting, it avoids the sensitivity problems of conventional fluorescence spectroscopy, which are due to low detection efficiency and large background from scattered laser light. We report the first application of an alternative ionization scheme which we have developed for collinear laser spectroscopy on fast atomic beams /1/. Here the increase in sensitivity has considerably enlarged the range of isotopes very far from stability, for which nuclear moments and radii can be investigated in hyperfine structure and isotope shift measurements.
Moments and Radii of 78–100Sr
The chain of Sr isotopes ranges from the neutron-shell closure at N = 50 into both the N = 38 and N = 60 deformation regions which represent the main topic of this workshop. For a detailed understanding of the nature of these nuclei, laser spectroscopy can provide the ground state spins and moments, as well as the the changes in the mean square charge radii as a function of the neutron number N. Recent experiments at Karlsruhe [1] and at Daresbury [2] essentially cover the neutron-deficient and stable Sr isotopes between N = 40 and N = 50. In order to complement these results, and to extend the measurements into the region of neutron-rich isotopes, we have performed an experiment at the ISO…
High resolution spectroscopy of rydberg states in indium I
Two-photon laser spectroscopy in a dense indium vapour allowed to investigatenp2P1/2, 3/2 states (n=27–35) for113, 115In with a thermionic diode. Precise data on the fine structure splitting of these states and the isotope shift of the two photon transitions have been obtained. The fine structure splitting shows a hydrogenic behaviour. By using the result of our isotope shift measurement in combination with literature values, level isotope shifts with reference to the ionization limit are deduced and analysed with respect to the different contributions.
Nuclear spin and magnetic moment of 11Li
Abstract Nuclear spin and magnetic moment of 11Li have been measured by optical pumping of a fast atomic beam. The angular asymmetry of the β-radiation from the polarized nuclei was used to detect the hfs of the 2s 2 S 1 2 −2 p 2 P 1 2 resonance line and the NMR signal cubic LiF crystal lattice. The results I= 3 2 and μI=3.6673(25) n.m. indicate a pure 1p 3 2 state of the valence proton.
Optical spectroscopy using mass-separated beams: Nuclear properties of unstable indium and tin isotopes
Abstract Collinear fast-beam laser-spectroscopy has been used to measure the hyperfine structure and isotope shift of several indium and tin isotopes. The related experimental techniques are described, including the preparation of mass-separated beams of neutron-deficient indium and tin isotopes at the GSI on-line mass separator following fusion-evaporation reactions. The deviation of the observed dependence of the charge radii upon the neutron number from the expected behaviour is briefly discussed.
Intense beams of mass-separated, neutron-deficient indium, tin, thallium and lead isotopes
A discharge ion source of the FEBIAD-type that delivers intense beams of neutron-deficient isotopes of indium, tin, thallium and lead produced in heavy-ion-induced fusion reactions is described. After mass separation the isotopically pure beams with intensities of up to 3 × 107 ions/s were available for gamma and laser spectroscopy. This corresponds to an overall separation efficiency of about 30%.
Nuclear moments and charge radii of105, 106In
With high resolution collinear fast beam laser spectroscopy in the 451 nm-line of Indium nuclear moments and the change in the mean square radii of the nuclear charge distribution of105,106 In have been determined.
Hyperfine structure and isotope shift investigations in $^{202-222}$Rn for the study of nuclear structure beyond Z = 82
The hyperfine structure (hfs) and isotope shift (IS) in the isotopic chain of the radioactive element radon have been studied for the first time. The measurements were carried out by collinear fast-beam laser spectroscopy at the mass separator facility ISOLDE at CERN. The IS between 16 isotopes in the mass range 202≦A≦222 and the hfs of 7 odd-A isotopes were determined in the transitions 7s [3/2]2-7p [5/2]3 (745 nm) of Rn I. The nuclear spins and moments, as well as the observed inversion of the odd-even staggering for218–222Rn, can be associated with the effects of octupole instability around N=134.