0000000000007512
AUTHOR
V. N. Fedoseyev
Frequency tripling for resonance ionization spectroscopy (RIS) of Cd
To explore the nucleosynthesis of heavy elements in the rapid neutron-capture process, investigations on short- lived, very neutron-rich Cd isotopes are planned that require pure samples. These will be produced at the CERN-ISOLDE on-line mass separator in combination with a chemically se- lective laser ion source. The excitation scheme for resonance ionization of Cd was tested in Mainz with a copper-vapor- pumped dye laser system. Due to the high ionization potential of Cd, frequency tripling was required for the first excita- tion step.1D 228: 8n m/. Laser light with an average power of 2m Wwas obtained after frequency tripling and was suc- cessfully used for RIS test measurements on cadmi…
On-line yields obtained with the ISOLDE RILIS
The ISOLDE resonance ionization laser ion source (RILIS) allows to ionize efficiently and selectively many metallic elements. In recent yield surveys and on-line experiments with the ISOLDE RILIS we observed 23–34 Mg, 26–34 Al, 98–132 Cd, 149 Tb, 155–177 Yb, 179–200 Tl, 183–215 Pb and 188–218 Bi. The obtained yields are presented together with measured release parameters which allow to extrapolate the release efficiency towards more exotic (short-lived) nuclides of the same elements. 2002 Elsevier Science B.V. All rights reserved.
New information on β-delayed neutron emission from Be-12, Be-14
17 pages, 3 tables, 5 figures, 1 appendix.-- PACS nrs.: 23.40.Hc; 27.20.+n.
Selective laser ionization of N≥82 indium isotopes: The new r-process nuclide 135In
Production yields and beta-decay half-lives of very neutron-rich indium isotopes were determined at CERN/ISOLDE using isobaric selectivity of a resonance-ionization laser ion-source. Beta-delayed neutron multiscaling measurements have yielded improved half-lives for 206(6)~ms $^{132}$In, 165(3)~ms $^{133}$In and 141(5)~ms $^{134}$In. With 92(10)~ms $^{135}$In, a new r-process nuclide has been identified which acts as an important `waiting-point' in the In isotopic chain for neutron densities in the range n$_n \simeq 10^{24}$--10$^{26}$ n/cm$^3$, where the r-matter flow has already passed the ${\rm A} \simeq 130$ abundance-peak region.
Structure And Decay Of Neutron-Rich Nuclides In The 115 ≤ A ≤ 138 Mass Range And r-Process Nucleosynthesis
The structure and decay of neutron‐rich r‐process nuclides has been studied by a variety of means that take advantage of enhanced selectivity to permit identification of exotic nuclides. New level structures are presented for 134,135Sb along with data for Ag isomers and Cd yrast structures. Some of the properties measured play an important role in calculations of the yields of elements and isotopes produced in r‐process nucleosynthesis that takes place at high temperature in the presence of large densities of neutrons.
Light exotic isotopes: recent beam developments and physics applications at ISOLDE
This paper is divided in three parts: (i) the measurement of yields and decay losses of Li and Be isotopes released from a thin foil tantalum target at the CERN/ISOLDE PS-Booster; (ii) results from beta-decay experiments on Be-12 and Be-14, an improved half-life of 21.49(3) ms has been obtained for Be-12; (iii) the beta-decay of C-9. An outline of the analysis procedure to determine the branching at high excitation energies is given. The ground-state branch has been determined to 54.1(15)%.
Study of short-lived tin isotopes with a laser ion source
A chemically selective laser ion source based on resonance ionization of atoms in a hot cavity has been applied for the study of short-lived silver isotopes at CERN/ ISOLDE. Silver atoms were ionized by two resonant excitations and final laser ionization into the continuum. Decay properties of the neutron-rich isotopes121–127Ag were studied with a neutron long-counter and aβ-detector.
Production of radioactive Ag ion beams with a chemically selective laser ion source
Abstract We have developed a chemically selective laser ion source at the CERN-ISOLDE facility in order to study neutron-rich Ag nuclides. A pulsed laser system with high repetition rate has been used based on high-power coppe-vapour pump lasers and dye lasers. With this source significant reductions of the isobaric background has been achieved.
β−decay of the neutron-rich isotope215Pb
This Brief Report reports on the first observation of the β--delayed γ decay of 215Pb, feeding states in 215Bi. The 215Pb beam was produced using resonant laser ionization and mass separated at the ISOLDE-CERN on-line mass separator. This ensured clean identification of the γ rays as belonging to the decay of 215Pb or its β-decay daughters. A half-life of 147(12) s was measured for the 215Pb β decay and a level scheme for the daughter nucleus 215Bi is proposed, resulting in an extended systematics of the excited states of the neutron-rich Bi isotopes.
Selective laser ionization of very neutron-rich cadmium isotopes: Decay properties of131Cd83and132Cd84
A chemically selective laser ion source has been applied in a decay study of the very neutron-rich isotopes ${}^{131}\mathrm{Cd}$ and ${}^{132}\mathrm{Cd}$ at CERN/ISOLDE. For the ${\ensuremath{\beta}}^{\ensuremath{-}}$ decay of the $N=83$ nuclide ${}^{131}\mathrm{Cd}$ a surprisingly short half-life of $(68\ifmmode\pm\else\textpm\fi{}3)$ ms and a weak delayed-neutron branch of ${P}_{n}=(3.5\ifmmode\pm\else\textpm\fi{}1.0)%$ were observed. For the $N=84$ nuclide ${}^{132}\mathrm{Cd}$ a half-life of $(97\ifmmode\pm\else\textpm\fi{}10)$ ms and a ${P}_{n}$ value of $(60\ifmmode\pm\else\textpm\fi{}15)%$ were obtained. Schematic features of both decay schemes are developed. We find that our new d…
$\beta$ - decay of the M$_{T}$=-1 nucleus $^{58}$Zn studied by selective laser ionization
$\beta$ - decay of $^{58}$Zn has been studied for the first time. A new laser ion-source concept has been used to produce mass-separated sources for $\beta$ and $\gamma$ - spectroscopy. The half-life of $^{58}$Zn was determined to be 86(18) ms. Comparisons are made with previous data from charge-exchange reactions. Our Gamow-Teller strength to the 1$^{+}$ state at 1051 keV excitation in $^{58}$Cu agrees well with the value extracted from a recent ($^{3}$He, t) study. Extensive shell-model calculations are presented.
Selective laser ionization of radioactive Ni-isotopes
Abstract A chemically selective laser ion source based on resonance ionization of atoms in a hot cavity has been applied in the study of Ni-isotopes at the CERN-ISOLDE on-line isotope separator. Laser ionization enhanced the yields of long-lived Ni-isotopes almost four orders of magnitude when compared to the yields obtained with the surface ionization mode of the source. As a result, high yields of long-lived Ni-isotopes were obtained. Separation efficiencies of 0.3 and 0.8% were obtained for Ni produced in uranium-carbide, produced from uranium-di-pthalocyanine, and Ta-foil targets, respectively. Ni was found to be released very slowly from the present target and ion source combination.
Progress in ISOL target–ion source systems
The heart of every ISOL (isotope separation on-line) facility is its target and ion source system. Its efficiency, selectivity and rapidity is decisive for the production of intense and pure ion beams of short-lived isotopes. Recent progress in ISOL target and ion source technology is discussed at the examples of radioactive ion beams of exotic zinc and tin isotopes that were purified by isothermal chromatography and molecular sideband separation respectively. An outlook is given to which other elements these purification methods are applicable.
Decay of Neutron-Rich Mn Nuclides and Deformation of Heavy Fe Isotopes
The use of chemically selective laser ionization combined with beta-delayed neutron counting at CERN/ISOLDE has permitted identification and half-life measurements for 623-ms Mn-61 up through 14-ms Mn-69. The measured half-lives are found to be significantly longer near N=40 than the values calculated with a QRPA shell model using ground-state deformations from the FRDM and ETFSI models. Gamma-ray singles and coincidence spectroscopy has been performed for Mn-64 and Mn-66 decays to levels of Fe-64 and Fe-66, revealing a significant drop in the energy of the first 2+ state in these nuclides that suggests an unanticipated increase in collectivity near N=40.
Beta decay of the new isotope101Sn
The very neutron-deficient isotope 101Sn was produced in a 50Cr(58Ni, 2p5n) reaction and its decay properties were determined for the first time. By using chemically selective ion sources of an on-line mass separator, the energy spectrum and the half-life (3 ± 1 s) of beta-delayed protons of 101Sn were measured. These results are compared to theoretical predictions.
First observation of the β-decay of neutron-rich 215Pb and 218Bi by the pulsed-release technique and resonant laser ionisation
The neutron-rich Tl, Pb and Bi isotopes are of exceptional interest to trace the evolution of single-particle levels away from the doubly magic 208Pb towards the neutron-rich side of the nuclear chart. While 208Pb is well understood in terms of the shell model, experimental data on the heavier isotopes is very scarce and it is far from clear to what extent the shell model is upheld [1]. Furthermore, large branchings ratios for β-delayed neutron emission are expected in this mass region, adding astrophysical interest to the subject [2].
Ground-state spin of 59Mn
Beta decay of $^{59}$Mn has been studied at PSB-ISOLDE, CERN. The intense and pure Mn beam was produced using the Resonance Ionization Laser Ion Source (RILIS). Based on the measured $\beta$-decay rates the ground-state spin and parity are proposed to be $J^{\pi}$ = 5/2$^{-}$. This result is consistent with the systematic trend of the odd-A Mn nuclei and extends the systematics one step further towards the neutron drip line.
Charge radius change in the heavy tin isotopes until A = 132 from laser spectroscopy
Laser spectroscopy measurements have been carried out on the very neutron-rich tin isotopes with the COMPLIS experimental setup. Using the 5s 25p 23P 0 → 5s 25p6s 3P 1 optical transition, hyperfine spectra of 126-132Sn and 125m, 127m, 129m-131mSn where recorded for the first time. The variation of the mean-square charge radius ( δ〈r 2〉) between these nuclei and nuclear moments of the isomers and the odd isotopes were thus measured. An odd-even staggering which inverts at A = 130 is clearly observed. This indicates a small appearance of a plateau on the δ〈r 2〉 which has to be confirmed by measuring the isotope shift beyond A = 132.
Measurement of the Magnetic Moment of the One-Neutron Halo NucleusB11e
The magnetic moment of ${}^{11}\mathrm{Be}$ ( ${T}_{1/2}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}13.8\phantom{\rule{0ex}{0ex}}\mathrm{s}$) was measured by detecting nuclear magnetic resonance signals in a beryllium crystal lattice. The experimental technique applied to a ${}^{11}{\mathrm{Be}}^{+}$ ion beam from a laser ion source includes in-beam optical polarization, implantation into a metallic single crystal, and observation of rf resonances in the asymmetric angular distribution of the $\ensuremath{\beta}$ decay ( $\ensuremath{\beta}$-NMR). The nuclear magnetic moment $\ensuremath{\mu}{(}^{11}\mathrm{Be})\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}\ensuremath{-}1.6816(8…
Charge radii of odd-A 191–211Po isotopes
Isotope shifts have been measured for the odd-A polonium isotopes 191–211Po and changes in the nuclear mean square charge radii δr2 have been deduced. The measurements were performed at CERN-ISOLDE using the in-source resonance-ionization spectroscopy technique. The combined analysis of these data and our recent results for even-A polonium isotopes indicates an onset of deformation already at 197,198Po, when going away from stability. This is significantly earlier than was suggested by previous theoretical and experimental studies of the polonium isotopes. Moreover and in contrast to the mercury isotopes, where a strong odd–even staggering of the charge radii of the ground states was observ…
β-decay studies of135–137Snusing selective resonance laser ionization techniques
The decays of the very neutron rich Sn isotopes Sn135-137 were studied at CERN/ISOLDE using isotopic and isobaric selectivity achieved by the use of a resonance ionization laser ion source and mass spectroscopy, respectively. Neutron decay rates, gamma-ray singles, and gamma-gamma coincidence data were collected as a function of time. The half-life (T-1/2) and delayed neutron emission probability (P-n) values of 135 Sn were measured to be 530(20) ms and 21(3)%, respectively. For Sn-136, a T-1/2 of 250(30) ms was determined along with a P-n value of 30(5)%. For Sn-137, a T-1/2 of 190(60) ms and a P-n value of 58(15)% were deduced. Identification of low-energy transitions in Sb-135 was made p…