6533b854fe1ef96bd12ae1dd

RESEARCH PRODUCT

Selective laser ionization of radioactive Ni-isotopes

A.-h. EvensenN. TrautmanJacques LettryA. WöhrH. L. RavnS. KohlerV. N. FedoseyevN. ErdmannA. JokinenY. JadingE. KuglerKarl KratzP. Van DuppenV. I. MishinV. I. Tikhonov

subject

Nuclear and High Energy PhysicsChemical ionizationMatrix-assisted laser desorption electrospray ionizationChemistryRadiochemistryAnalytical chemistryThermal ionizationIon sourceAtmospheric-pressure laser ionizationIonizationPhysics::Atomic PhysicsNuclear ExperimentInstrumentationElectron ionizationAmbient ionization

description

Abstract A chemically selective laser ion source based on resonance ionization of atoms in a hot cavity has been applied in the study of Ni-isotopes at the CERN-ISOLDE on-line isotope separator. Laser ionization enhanced the yields of long-lived Ni-isotopes almost four orders of magnitude when compared to the yields obtained with the surface ionization mode of the source. As a result, high yields of long-lived Ni-isotopes were obtained. Separation efficiencies of 0.3 and 0.8% were obtained for Ni produced in uranium-carbide, produced from uranium-di-pthalocyanine, and Ta-foil targets, respectively. Ni was found to be released very slowly from the present target and ion source combination.

https://doi.org/10.1016/s0168-583x(97)01078-1